高性能碱金属电池用无机固态电解质的纳米级界面工程

IF 9.4 1区 化学 Q1 CHEMISTRY, PHYSICAL
Ronghao Wang , Kaiwen Sun , Yuhao Zhang , Bingqin Li , Chengfei Qian , Jingfa Li , Fangyang Liu , Weizhai Bao
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引用次数: 10

摘要

全固态金属电池(assmb)因其超高的比容量和最低的氧化还原电位而被认为是下一代高能储能系统的理想候选者。然而,循环过程中不可控的化学反应性直接决定了金属枝晶的生长行为,低库仑效率和安全问题严重限制了它们的实际应用。基于固态电解质(ssi)的晶体学优化为抑制金属阳极枝晶生长提供了原子尺度上的基本解决方案,已引起广泛关注。从这一角度出发,总结了近年来各类固态电解质晶体学优化的研究进展。我们重点介绍了新一代全固态电池(包括锂离子电池、钠离子电池、镁离子电池)晶体学优化的最新实验发现,旨在对assmb中的晶体学反应有更深入的了解。讨论了晶体学优化在未来设计和工程中的挑战和前景,为进一步研究晶体学优化以提高可充电电池的性能提供了思路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Nanoscale interface engineering of inorganic Solid-State electrolytes for High-Performance alkali metal batteries

Nanoscale interface engineering of inorganic Solid-State electrolytes for High-Performance alkali metal batteries

All-solid-state metal batteries (ASSMBs) have been regarded as the ideal candidate for the next-generation high-energy storage system due to their ultrahigh specific capacity and the lowest redox potential. However, the uncontrollable chemical reactivity during cycling which directly determines the growth behaviour of metal dendrites, the low coulombic efficiency and the safety concerns severely limit their real-world applications.. Crystallographic optimization based on solid-state electrolytes (SSEs) provides an atomic-scale and fundamental solution for the inhibition of dendrite growth in metal anodes, which has attracted widespread attentions. From this perspective, we summarize the recent advance of the crystallographic optimization for various classes of solid-state electrolytes. We highlight the recent experimental findings of crystallographic optimization for a new generation of all-solid-state batteries, including lithium-ion batteries, sodium-ion batteries, magnesium-ion batteries, with the aim of providing a deeper understanding of the crystallographic reactions in ASSMBs. The challenges and prospects for the future design and engineering of crystallographic optimization of SSEs are discussed, providing ideas for further research into crystallographic optimization to improve the performance of rechargeable batteries.

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来源期刊
CiteScore
16.10
自引率
7.10%
发文量
2568
审稿时长
2 months
期刊介绍: The Journal of Colloid and Interface Science publishes original research findings on the fundamental principles of colloid and interface science, as well as innovative applications in various fields. The criteria for publication include impact, quality, novelty, and originality. Emphasis: The journal emphasizes fundamental scientific innovation within the following categories: A.Colloidal Materials and Nanomaterials B.Soft Colloidal and Self-Assembly Systems C.Adsorption, Catalysis, and Electrochemistry D.Interfacial Processes, Capillarity, and Wetting E.Biomaterials and Nanomedicine F.Energy Conversion and Storage, and Environmental Technologies
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