铁催化的乙醚和吡咯烷衍生物与磺酰氯的α-C(sp3)磺化反应

IF 4.7 1区 化学 Q1 CHEMISTRY, ORGANIC
Mingyu Jiang,Fuqi Li,Bei Lei,Wen-Ya Zheng,Junshan Lai
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引用次数: 0

摘要

选择性α-C(sp3)磺化醚和氮杂环提供了原子经济和阶梯经济的途径获得脂肪族砜,脂肪族砜是药物和精细化学品中普遍存在的组成部分。有机电合成和铁催化为自由基C-S键的形成提供了可持续的合成平台,但它们在脂肪族α-C(sp3)磺酰化中的结合仍未得到充分的研究。本文报道了一种未分裂细胞铁催化的乙醚和n保护吡咯烷与磺酰氯的电化学α-磺化反应。该方法得益于无迹电氧化还原等价物、廉价的地球丰富的催化剂和广泛的官能团兼容性。克级反应和产品衍生化证明了其合成的实用性。该电驱动方案利用阳极Fe(III)/Fe(II)氧化还原穿梭产生醚和吡啶衍生物作为底物衍生的自由基阳离子中间体,其中磺酰自由基来自磺酰氯的直接阴极还原。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Iron-Catalyzed Electrochemical α-C(sp3) Sulfonylation of Ethers and Pyrrolidine Derivatives with Sulfonyl Chlorides

Iron-Catalyzed Electrochemical α-C(sp3) Sulfonylation of Ethers and Pyrrolidine Derivatives with Sulfonyl Chlorides
Selective α-C(sp3) sulfonylation of ethers and nitrogen heterocycles provides atom- and step-economical access to aliphatic sulfones, which are prevalent building blocks in pharmaceuticals and fine chemicals. Organic electrosynthesis and iron catalysis represent sustainable synthetic platforms for radical C–S bond formation, yet their combination for aliphatic α-C(sp3) sulfonylation remains underexplored. Herein, an undivided-cell iron-catalyzed electrochemical α-sulfonylation of ethers and N-protected pyrrolidines with sulfonyl chlorides is reported. The method benefits from traceless electrical redox equivalents, a cheap earth-abundant catalyst, and broad functional group compatibility. Gram-scale reactions and product derivatizations demonstrate its synthetic practicability. This electro-driven protocol leverages an anodic Fe(III)/Fe(II) redox shuttle to generate ethers and pyrrolidine derivatives as substrate-derived radical cation intermediates, with sulfonyl radicals originating from direct cathodic reduction of sulfonyl chlorides.
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来源期刊
Organic Letters
Organic Letters 化学-有机化学
CiteScore
9.30
自引率
11.50%
发文量
1607
审稿时长
1.5 months
期刊介绍: Organic Letters invites original reports of fundamental research in all branches of the theory and practice of organic, physical organic, organometallic,medicinal, and bioorganic chemistry. Organic Letters provides rapid disclosure of the key elements of significant studies that are of interest to a large portion of the organic community. In selecting manuscripts for publication, the Editors place emphasis on the originality, quality and wide interest of the work. Authors should provide enough background information to place the new disclosure in context and to justify the rapid publication format. Back-to-back Letters will be considered. Full details should be reserved for an Article, which should appear in due course.
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