F A M Leermakers, L Ruiz-Martínez, S D Stoyanov, J van der Gucht
{"title":"分离性葡聚糖-聚乙二醇水溶液的自一致场分析:(2)吸附和润湿。","authors":"F A M Leermakers, L Ruiz-Martínez, S D Stoyanov, J van der Gucht","doi":"10.1021/acs.jpcb.5c04279","DOIUrl":null,"url":null,"abstract":"<p><p>Aqueous two-phase systems (ATPS), with dextran-water-poly(ethylene glycol) (PEG) as the main example, are water-continuous polymer segregated systems. How such ATPS behaves near solid interfaces is studied using the Scheutjens Fleer self-consistent field (SF-SCF) theory. We have analyzed the adsorption isotherms of the minority (wetting) component PEG at either a fixed solvent- or a fixed dextran bulk volume fraction and focused on wetting and polymer displacement transitions. When the driving force for segregative phase behavior is sufficiently strong (repulsive interactions between dextran and PEG: the major driving force), a jump-like transition displacing adsorbed dextran by PEG may take the form of a prewetting transition when the PEG-rich phase wets the surface. Interestingly, the first-order displacement transition manifests as a pure surface phase transition at supercritical conditions. This explains why the wetting transition is robust first order. Only when the segregative phase behavior is triggered by a solvent quality disparity (minor driving force), one may find isotherms with two consecutive transitions, that is, a smooth displacement transition followed by a jump-like prewetting transition. Explained by the low interfacial tension between the PEG-rich and dextran-rich phases, the parameter window for partial wetting is small. Remarkably, for an experimentally realistic ATPS and carefully tuned adsorption parameters, it is possible that upon a change of the solvent content there is a sequence of two wetting transitions (going from partial wet to wet and back to partial wet) followed by a drying transition.</p>","PeriodicalId":60,"journal":{"name":"The Journal of Physical Chemistry B","volume":" ","pages":""},"PeriodicalIF":2.9000,"publicationDate":"2025-10-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Self-Consistent Field Analysis of Segregative Aqueous Dextran-Polyethylene Glycol Solutions: (2) Adsorption and Wetting.\",\"authors\":\"F A M Leermakers, L Ruiz-Martínez, S D Stoyanov, J van der Gucht\",\"doi\":\"10.1021/acs.jpcb.5c04279\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Aqueous two-phase systems (ATPS), with dextran-water-poly(ethylene glycol) (PEG) as the main example, are water-continuous polymer segregated systems. How such ATPS behaves near solid interfaces is studied using the Scheutjens Fleer self-consistent field (SF-SCF) theory. We have analyzed the adsorption isotherms of the minority (wetting) component PEG at either a fixed solvent- or a fixed dextran bulk volume fraction and focused on wetting and polymer displacement transitions. When the driving force for segregative phase behavior is sufficiently strong (repulsive interactions between dextran and PEG: the major driving force), a jump-like transition displacing adsorbed dextran by PEG may take the form of a prewetting transition when the PEG-rich phase wets the surface. Interestingly, the first-order displacement transition manifests as a pure surface phase transition at supercritical conditions. This explains why the wetting transition is robust first order. Only when the segregative phase behavior is triggered by a solvent quality disparity (minor driving force), one may find isotherms with two consecutive transitions, that is, a smooth displacement transition followed by a jump-like prewetting transition. Explained by the low interfacial tension between the PEG-rich and dextran-rich phases, the parameter window for partial wetting is small. Remarkably, for an experimentally realistic ATPS and carefully tuned adsorption parameters, it is possible that upon a change of the solvent content there is a sequence of two wetting transitions (going from partial wet to wet and back to partial wet) followed by a drying transition.</p>\",\"PeriodicalId\":60,\"journal\":{\"name\":\"The Journal of Physical Chemistry B\",\"volume\":\" \",\"pages\":\"\"},\"PeriodicalIF\":2.9000,\"publicationDate\":\"2025-10-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"The Journal of Physical Chemistry B\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.jpcb.5c04279\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"The Journal of Physical Chemistry B","FirstCategoryId":"1","ListUrlMain":"https://doi.org/10.1021/acs.jpcb.5c04279","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Self-Consistent Field Analysis of Segregative Aqueous Dextran-Polyethylene Glycol Solutions: (2) Adsorption and Wetting.
Aqueous two-phase systems (ATPS), with dextran-water-poly(ethylene glycol) (PEG) as the main example, are water-continuous polymer segregated systems. How such ATPS behaves near solid interfaces is studied using the Scheutjens Fleer self-consistent field (SF-SCF) theory. We have analyzed the adsorption isotherms of the minority (wetting) component PEG at either a fixed solvent- or a fixed dextran bulk volume fraction and focused on wetting and polymer displacement transitions. When the driving force for segregative phase behavior is sufficiently strong (repulsive interactions between dextran and PEG: the major driving force), a jump-like transition displacing adsorbed dextran by PEG may take the form of a prewetting transition when the PEG-rich phase wets the surface. Interestingly, the first-order displacement transition manifests as a pure surface phase transition at supercritical conditions. This explains why the wetting transition is robust first order. Only when the segregative phase behavior is triggered by a solvent quality disparity (minor driving force), one may find isotherms with two consecutive transitions, that is, a smooth displacement transition followed by a jump-like prewetting transition. Explained by the low interfacial tension between the PEG-rich and dextran-rich phases, the parameter window for partial wetting is small. Remarkably, for an experimentally realistic ATPS and carefully tuned adsorption parameters, it is possible that upon a change of the solvent content there is a sequence of two wetting transitions (going from partial wet to wet and back to partial wet) followed by a drying transition.
期刊介绍:
An essential criterion for acceptance of research articles in the journal is that they provide new physical insight. Please refer to the New Physical Insights virtual issue on what constitutes new physical insight. Manuscripts that are essentially reporting data or applications of data are, in general, not suitable for publication in JPC B.