{"title":"铒离子注入铌酸锂薄膜的强光致发光及其与晶格缺陷的相互作用","authors":"Liangling Wang, Sören Lerner, Houbin Zhu, Xiaojun Cui, Binge Zeng, Fengkai Wei, Elke Wendler, Carsten Ronning","doi":"10.1002/adom.202502568","DOIUrl":null,"url":null,"abstract":"<p>Erbium-doped lithium niobate on insulator (Er-LNOI) has attracted significant attention for its potential in integrated photonics and quantum applications due to its efficient 1540 nm emission in the telecom band. In this work, the lattice damage and infrared photoluminescence of Er-LNOI fabricated via Er ion implantation and subsequent thermal annealing is investigated. Damage profiles are analyzed using Rutherford backscattering spectrometry in channeling mode (RBS/C), revealing the formation of an amorphous layer during ion implantation. However, re-crystallization into an Er-doped LNOI single crystal occurs with some remaining dislocation loops after annealing. Photoluminescence measurements at room temperature demonstrate intense infrared emission with no evidence of Er clustering and concentration quenching up to an Er fluence of 2.63 × 10<sup>1</sup>⁵ ions cm<sup>2</sup>. Power- and temperature-dependent PL spectra suggest stable emission and distinct thermal quenching mechanisms for the two Stark-split transitions. The results confirm the effective optical activation of single crystalline Er-LNOI and highlight its promise for on-chip light sources and active photonic devices.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 29","pages":""},"PeriodicalIF":7.2000,"publicationDate":"2025-08-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202502568","citationCount":"0","resultStr":"{\"title\":\"Intense Photoluminescence in Erbium-Ion-Implanted Lithium Niobate Thin Films and Its Interplay with Lattice Defects\",\"authors\":\"Liangling Wang, Sören Lerner, Houbin Zhu, Xiaojun Cui, Binge Zeng, Fengkai Wei, Elke Wendler, Carsten Ronning\",\"doi\":\"10.1002/adom.202502568\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Erbium-doped lithium niobate on insulator (Er-LNOI) has attracted significant attention for its potential in integrated photonics and quantum applications due to its efficient 1540 nm emission in the telecom band. In this work, the lattice damage and infrared photoluminescence of Er-LNOI fabricated via Er ion implantation and subsequent thermal annealing is investigated. Damage profiles are analyzed using Rutherford backscattering spectrometry in channeling mode (RBS/C), revealing the formation of an amorphous layer during ion implantation. However, re-crystallization into an Er-doped LNOI single crystal occurs with some remaining dislocation loops after annealing. Photoluminescence measurements at room temperature demonstrate intense infrared emission with no evidence of Er clustering and concentration quenching up to an Er fluence of 2.63 × 10<sup>1</sup>⁵ ions cm<sup>2</sup>. Power- and temperature-dependent PL spectra suggest stable emission and distinct thermal quenching mechanisms for the two Stark-split transitions. The results confirm the effective optical activation of single crystalline Er-LNOI and highlight its promise for on-chip light sources and active photonic devices.</p>\",\"PeriodicalId\":116,\"journal\":{\"name\":\"Advanced Optical Materials\",\"volume\":\"13 29\",\"pages\":\"\"},\"PeriodicalIF\":7.2000,\"publicationDate\":\"2025-08-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/adom.202502568\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Optical Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://advanced.onlinelibrary.wiley.com/doi/10.1002/adom.202502568\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Optical Materials","FirstCategoryId":"88","ListUrlMain":"https://advanced.onlinelibrary.wiley.com/doi/10.1002/adom.202502568","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Intense Photoluminescence in Erbium-Ion-Implanted Lithium Niobate Thin Films and Its Interplay with Lattice Defects
Erbium-doped lithium niobate on insulator (Er-LNOI) has attracted significant attention for its potential in integrated photonics and quantum applications due to its efficient 1540 nm emission in the telecom band. In this work, the lattice damage and infrared photoluminescence of Er-LNOI fabricated via Er ion implantation and subsequent thermal annealing is investigated. Damage profiles are analyzed using Rutherford backscattering spectrometry in channeling mode (RBS/C), revealing the formation of an amorphous layer during ion implantation. However, re-crystallization into an Er-doped LNOI single crystal occurs with some remaining dislocation loops after annealing. Photoluminescence measurements at room temperature demonstrate intense infrared emission with no evidence of Er clustering and concentration quenching up to an Er fluence of 2.63 × 101⁵ ions cm2. Power- and temperature-dependent PL spectra suggest stable emission and distinct thermal quenching mechanisms for the two Stark-split transitions. The results confirm the effective optical activation of single crystalline Er-LNOI and highlight its promise for on-chip light sources and active photonic devices.
期刊介绍:
Advanced Optical Materials, part of the esteemed Advanced portfolio, is a unique materials science journal concentrating on all facets of light-matter interactions. For over a decade, it has been the preferred optical materials journal for significant discoveries in photonics, plasmonics, metamaterials, and more. The Advanced portfolio from Wiley is a collection of globally respected, high-impact journals that disseminate the best science from established and emerging researchers, aiding them in fulfilling their mission and amplifying the reach of their scientific discoveries.