通过电子-供体-受体络合物光活化和自由基加成到亚胺试剂中的选择性C-H亚胺化。

IF 5 1区 化学 Q1 CHEMISTRY, ORGANIC
Joshua T Baxter,Adrian Hall,Michael C Willis
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引用次数: 0

摘要

芳基亚砜酰胺是一种通用的合成中间体,用于获得多种与医学相关的S(VI)功能,如磺胺和磺胺酰亚胺。在此,我们报道了一种通过蓝光促进的电子供体-受体(EDA)络合物,使噻吩使能,位点选择性的C-H亚胺化过程,以获得关键的芳基亚胺物种。这个操作简单的过程结合了位点选择性C-H磺酸盐的制备,然后是由光活性EDA配合物与现成的胺形成的单电子转移(SET)。生成的芳基自由基与亚胺试剂在温和条件下反应生成芳基亚胺。该方法显示了广泛的通用性,并且在不使用昂贵的过渡金属或光氧化还原催化剂的情况下,区域选择性地从医学相关的芳烃中构建关键的芳基亚胺,突出了其作为药物和药物发现化学的后期功能化工具的用途。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Site-Selective C-H Sulfinamidation through Electron-Donor-Acceptor Complex Photoactivation and Radical Addition into Sulfinylamine Reagents.
Aryl sulfinamides are versatile synthetic intermediates for accessing diverse and medicinally relevant S(VI) functionalities, such as sulfonamides and sulfonimidamides. Herein, we report a thianthrenium-enabled, site-selective C-H sulfinamidation procedure via a blue-light-promoted electron-donor-acceptor (EDA) complex to afford the key aryl sulfinamide species. This operationally simple procedure combines site-selective C-H sulfonium salt preparation followed by single-electron transfer (SET) from a photoactive EDA complex formed with readily available amines. The resultant aryl radicals react with sulfinylamine reagents to deliver aryl sulfinamides under mild conditions. The method displays broad generality and regioselectively constructs key aryl sulfinamides from medicinally relevant arenes without using expensive transition metal or photoredox catalysts, highlighting its use as a late-stage functionalization tool for medicinal and drug discovery chemistry.
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来源期刊
Organic Letters
Organic Letters 化学-有机化学
CiteScore
9.30
自引率
11.50%
发文量
1607
审稿时长
1.5 months
期刊介绍: Organic Letters invites original reports of fundamental research in all branches of the theory and practice of organic, physical organic, organometallic,medicinal, and bioorganic chemistry. Organic Letters provides rapid disclosure of the key elements of significant studies that are of interest to a large portion of the organic community. In selecting manuscripts for publication, the Editors place emphasis on the originality, quality and wide interest of the work. Authors should provide enough background information to place the new disclosure in context and to justify the rapid publication format. Back-to-back Letters will be considered. Full details should be reserved for an Article, which should appear in due course.
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