Y Alexanian, A de la Torre, S McKeown Walker, M Straub, G Gatti, A Hunter, S Mandloi, E Cappelli, S Riccò, F Y Bruno, M Radovic, N C Plumb, M Shi, J Osiecki, C Polley, T K Kim, P Dudin, M Hoesch, R S Perry, A Tamai, F Baumberger
{"title":"高掺杂Sr2IrO4的费米表面和赝隙。","authors":"Y Alexanian, A de la Torre, S McKeown Walker, M Straub, G Gatti, A Hunter, S Mandloi, E Cappelli, S Riccò, F Y Bruno, M Radovic, N C Plumb, M Shi, J Osiecki, C Polley, T K Kim, P Dudin, M Hoesch, R S Perry, A Tamai, F Baumberger","doi":"10.1038/s41535-025-00817-9","DOIUrl":null,"url":null,"abstract":"<p><p>The fate of the Fermi surface in bulk electron-doped Sr<sub>2</sub>IrO<sub>4</sub> remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate the electronic structure of Sr<sub>2-<i>x</i></sub> La <sub><i>x</i></sub> IrO<sub>4</sub> up to <i>x</i> = 0.2, a factor of two higher than in previous work. We find that the antinodal pseudogap persists up to the highest doping level, and thus beyond the sharp increase in Hall carrier density to ≃ 1 + <i>x</i> recently observed above <i>x</i>* ≃ 0.16<sup>1</sup>. This suggests that doped iridates host a unique phase of matter in which a large Hall density coexists with an anisotropic pseudogap, breaking up the Fermi surface into disconnected arcs. The temperature boundary of the pseudogap is <i>T</i>* ≃ 200 K for <i>x</i> = 0.2, comparable to cuprates and to the energy scale of short range antiferromagnetic correlations in cuprates and iridates.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":"10 1","pages":"100"},"PeriodicalIF":6.2000,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12494496/pdf/","citationCount":"0","resultStr":"{\"title\":\"Fermi surface and pseudogap in highly doped Sr<sub>2</sub>IrO<sub>4</sub>.\",\"authors\":\"Y Alexanian, A de la Torre, S McKeown Walker, M Straub, G Gatti, A Hunter, S Mandloi, E Cappelli, S Riccò, F Y Bruno, M Radovic, N C Plumb, M Shi, J Osiecki, C Polley, T K Kim, P Dudin, M Hoesch, R S Perry, A Tamai, F Baumberger\",\"doi\":\"10.1038/s41535-025-00817-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>The fate of the Fermi surface in bulk electron-doped Sr<sub>2</sub>IrO<sub>4</sub> remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate the electronic structure of Sr<sub>2-<i>x</i></sub> La <sub><i>x</i></sub> IrO<sub>4</sub> up to <i>x</i> = 0.2, a factor of two higher than in previous work. We find that the antinodal pseudogap persists up to the highest doping level, and thus beyond the sharp increase in Hall carrier density to ≃ 1 + <i>x</i> recently observed above <i>x</i>* ≃ 0.16<sup>1</sup>. This suggests that doped iridates host a unique phase of matter in which a large Hall density coexists with an anisotropic pseudogap, breaking up the Fermi surface into disconnected arcs. The temperature boundary of the pseudogap is <i>T</i>* ≃ 200 K for <i>x</i> = 0.2, comparable to cuprates and to the energy scale of short range antiferromagnetic correlations in cuprates and iridates.</p>\",\"PeriodicalId\":19283,\"journal\":{\"name\":\"npj Quantum Materials\",\"volume\":\"10 1\",\"pages\":\"100\"},\"PeriodicalIF\":6.2000,\"publicationDate\":\"2025-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12494496/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"npj Quantum Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41535-025-00817-9\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"2025/10/3 0:00:00\",\"PubModel\":\"Epub\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"npj Quantum Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41535-025-00817-9","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/10/3 0:00:00","PubModel":"Epub","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
在块体电子掺杂的Sr2IrO4中,费米表面的命运仍然是难以捉摸的,它的赝隙相的起源和扩展也是如此。在这里,我们使用高分辨率角分辨光电子能谱(ARPES)来研究Sr2-x La x IrO4高达x = 0.2的电子结构,比以前的工作高两倍。我们发现,当霍尔载流子密度急剧增加到x*以上的1 + x时,反晶格赝隙持续存在到最高掺杂水平,从而达到≃0.161。这表明,掺杂的铱酸盐拥有一种独特的物质相,其中大霍尔密度与各向异性赝隙共存,将费米表面分解成不相连的弧。当x = 0.2时,赝隙的温度边界为T*≃200 K,与铜酸盐和铱酸盐的短程反铁磁相关的能量尺度相当。
Fermi surface and pseudogap in highly doped Sr2IrO4.
The fate of the Fermi surface in bulk electron-doped Sr2IrO4 remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate the electronic structure of Sr2-x La x IrO4 up to x = 0.2, a factor of two higher than in previous work. We find that the antinodal pseudogap persists up to the highest doping level, and thus beyond the sharp increase in Hall carrier density to ≃ 1 + x recently observed above x* ≃ 0.161. This suggests that doped iridates host a unique phase of matter in which a large Hall density coexists with an anisotropic pseudogap, breaking up the Fermi surface into disconnected arcs. The temperature boundary of the pseudogap is T* ≃ 200 K for x = 0.2, comparable to cuprates and to the energy scale of short range antiferromagnetic correlations in cuprates and iridates.
期刊介绍:
npj Quantum Materials is an open access journal that publishes works that significantly advance the understanding of quantum materials, including their fundamental properties, fabrication and applications.