E. Pitthan , M. Fellinger , B.Burazor Domazet , P.M. Wolf , J. Shams-Latifi , F. Aumayr , D. Primetzhofer
{"title":"光离子与等离子体表面材料的相互作用:提高实验精度及其对溅射良率模拟的影响","authors":"E. Pitthan , M. Fellinger , B.Burazor Domazet , P.M. Wolf , J. Shams-Latifi , F. Aumayr , D. Primetzhofer","doi":"10.1016/j.nme.2025.101996","DOIUrl":null,"url":null,"abstract":"<div><div>This work investigates how corrections to fundamental parameters describing ion–solid interaction affect sputtering yield simulations based on the binary collision approximation. We review recent experimental assessments of electronic stopping power and short-range repulsive interatomic potentials for light plasma species (H, D, He) in plasma-facing material candidates (W, Fe, EUROFER97), and compare them to widely used semi-empirical and theoretical models. At low energies, discrepancies of up to 60% relative to SRIM-2013 and up to 210% relative to SRIM-1997 are identified for the specific energy loss, highlighting the need for improved input parameters. We assess the sensitivity of sputtering yields to these corrections using SDTrimSP simulations, and compare the results to new experimental sputter yield data obtained for re-deposited thin W, Fe, and EUROFER97 films on a high-sensitivity quartz crystal microbalance. Incorporating derived stopping powers and interatomic potentials into the simulation significantly reduces the discrepancies between experimental and simulated sputtering yields. Remaining uncertainties and model limitations, such as crystal structure effects and ion implantation, are discussed.</div></div>","PeriodicalId":56004,"journal":{"name":"Nuclear Materials and Energy","volume":"45 ","pages":"Article 101996"},"PeriodicalIF":2.7000,"publicationDate":"2025-09-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Interaction of light ions with plasma-facing materials: Improved experimental accuracy and its impact on sputter yield simulations\",\"authors\":\"E. Pitthan , M. Fellinger , B.Burazor Domazet , P.M. Wolf , J. Shams-Latifi , F. Aumayr , D. Primetzhofer\",\"doi\":\"10.1016/j.nme.2025.101996\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This work investigates how corrections to fundamental parameters describing ion–solid interaction affect sputtering yield simulations based on the binary collision approximation. We review recent experimental assessments of electronic stopping power and short-range repulsive interatomic potentials for light plasma species (H, D, He) in plasma-facing material candidates (W, Fe, EUROFER97), and compare them to widely used semi-empirical and theoretical models. At low energies, discrepancies of up to 60% relative to SRIM-2013 and up to 210% relative to SRIM-1997 are identified for the specific energy loss, highlighting the need for improved input parameters. We assess the sensitivity of sputtering yields to these corrections using SDTrimSP simulations, and compare the results to new experimental sputter yield data obtained for re-deposited thin W, Fe, and EUROFER97 films on a high-sensitivity quartz crystal microbalance. Incorporating derived stopping powers and interatomic potentials into the simulation significantly reduces the discrepancies between experimental and simulated sputtering yields. Remaining uncertainties and model limitations, such as crystal structure effects and ion implantation, are discussed.</div></div>\",\"PeriodicalId\":56004,\"journal\":{\"name\":\"Nuclear Materials and Energy\",\"volume\":\"45 \",\"pages\":\"Article 101996\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2025-09-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nuclear Materials and Energy\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2352179125001383\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"NUCLEAR SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nuclear Materials and Energy","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2352179125001383","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Interaction of light ions with plasma-facing materials: Improved experimental accuracy and its impact on sputter yield simulations
This work investigates how corrections to fundamental parameters describing ion–solid interaction affect sputtering yield simulations based on the binary collision approximation. We review recent experimental assessments of electronic stopping power and short-range repulsive interatomic potentials for light plasma species (H, D, He) in plasma-facing material candidates (W, Fe, EUROFER97), and compare them to widely used semi-empirical and theoretical models. At low energies, discrepancies of up to 60% relative to SRIM-2013 and up to 210% relative to SRIM-1997 are identified for the specific energy loss, highlighting the need for improved input parameters. We assess the sensitivity of sputtering yields to these corrections using SDTrimSP simulations, and compare the results to new experimental sputter yield data obtained for re-deposited thin W, Fe, and EUROFER97 films on a high-sensitivity quartz crystal microbalance. Incorporating derived stopping powers and interatomic potentials into the simulation significantly reduces the discrepancies between experimental and simulated sputtering yields. Remaining uncertainties and model limitations, such as crystal structure effects and ion implantation, are discussed.
期刊介绍:
The open-access journal Nuclear Materials and Energy is devoted to the growing field of research for material application in the production of nuclear energy. Nuclear Materials and Energy publishes original research articles of up to 6 pages in length.