{"title":"基于材料信息学逆设计的强非互易宽带热辐射","authors":"Zihe Chen, Run Hu","doi":"10.1002/adom.202501219","DOIUrl":null,"url":null,"abstract":"<p>Through magneto-optical materials or spatiotemporal metamaterials, the reciprocity relation between thermal emission and absorption can be broken, achieving the more flexible nonreciprocal thermal radiation (NTR) to even approach the ultimate thermodynamic limit, such as the Landsberg limit. However, most NTR emitters only cover a narrow band, which is unwanted for thermal energy utilization. Here, a material-informatics framework with a Bayesian optimization (BO) kernel is proposed for designing NTR emitters, which consists of multilayer epsilon-near-zero (ENZ) magneto-optical films on a metal bottom. The optimal structural parameters can be obtained within only 0.5% of all possible structures, demonstrating super-efficient optimization capability. Additionally, compared to the design method based on the Fresnel formula, the broadband nonreciprocity can be significantly enhanced, with the wavelength-averaged nonreciprocity improved by 80.4%, which can be attributed to the unequal electromagnetic power dissipation density and mismatched effective impedance at opposite angles. Furthermore, the effects of the dielectric layer, different incident angles, number of layers, and magnetic fields on BO-based nonreciprocal thermal emitters have been investigated. This study can further promote the development of broadband NTR and can be extended to multilayer structures containing magnetic Weyl semimetals.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":"13 28","pages":""},"PeriodicalIF":7.2000,"publicationDate":"2025-08-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Strong Nonreciprocal Broadband Thermal Radiation via Materials Informatics Inverse Design\",\"authors\":\"Zihe Chen, Run Hu\",\"doi\":\"10.1002/adom.202501219\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Through magneto-optical materials or spatiotemporal metamaterials, the reciprocity relation between thermal emission and absorption can be broken, achieving the more flexible nonreciprocal thermal radiation (NTR) to even approach the ultimate thermodynamic limit, such as the Landsberg limit. However, most NTR emitters only cover a narrow band, which is unwanted for thermal energy utilization. Here, a material-informatics framework with a Bayesian optimization (BO) kernel is proposed for designing NTR emitters, which consists of multilayer epsilon-near-zero (ENZ) magneto-optical films on a metal bottom. The optimal structural parameters can be obtained within only 0.5% of all possible structures, demonstrating super-efficient optimization capability. Additionally, compared to the design method based on the Fresnel formula, the broadband nonreciprocity can be significantly enhanced, with the wavelength-averaged nonreciprocity improved by 80.4%, which can be attributed to the unequal electromagnetic power dissipation density and mismatched effective impedance at opposite angles. Furthermore, the effects of the dielectric layer, different incident angles, number of layers, and magnetic fields on BO-based nonreciprocal thermal emitters have been investigated. This study can further promote the development of broadband NTR and can be extended to multilayer structures containing magnetic Weyl semimetals.</p>\",\"PeriodicalId\":116,\"journal\":{\"name\":\"Advanced Optical Materials\",\"volume\":\"13 28\",\"pages\":\"\"},\"PeriodicalIF\":7.2000,\"publicationDate\":\"2025-08-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Optical Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://advanced.onlinelibrary.wiley.com/doi/10.1002/adom.202501219\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Optical Materials","FirstCategoryId":"88","ListUrlMain":"https://advanced.onlinelibrary.wiley.com/doi/10.1002/adom.202501219","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Strong Nonreciprocal Broadband Thermal Radiation via Materials Informatics Inverse Design
Through magneto-optical materials or spatiotemporal metamaterials, the reciprocity relation between thermal emission and absorption can be broken, achieving the more flexible nonreciprocal thermal radiation (NTR) to even approach the ultimate thermodynamic limit, such as the Landsberg limit. However, most NTR emitters only cover a narrow band, which is unwanted for thermal energy utilization. Here, a material-informatics framework with a Bayesian optimization (BO) kernel is proposed for designing NTR emitters, which consists of multilayer epsilon-near-zero (ENZ) magneto-optical films on a metal bottom. The optimal structural parameters can be obtained within only 0.5% of all possible structures, demonstrating super-efficient optimization capability. Additionally, compared to the design method based on the Fresnel formula, the broadband nonreciprocity can be significantly enhanced, with the wavelength-averaged nonreciprocity improved by 80.4%, which can be attributed to the unequal electromagnetic power dissipation density and mismatched effective impedance at opposite angles. Furthermore, the effects of the dielectric layer, different incident angles, number of layers, and magnetic fields on BO-based nonreciprocal thermal emitters have been investigated. This study can further promote the development of broadband NTR and can be extended to multilayer structures containing magnetic Weyl semimetals.
期刊介绍:
Advanced Optical Materials, part of the esteemed Advanced portfolio, is a unique materials science journal concentrating on all facets of light-matter interactions. For over a decade, it has been the preferred optical materials journal for significant discoveries in photonics, plasmonics, metamaterials, and more. The Advanced portfolio from Wiley is a collection of globally respected, high-impact journals that disseminate the best science from established and emerging researchers, aiding them in fulfilling their mission and amplifying the reach of their scientific discoveries.