开封市公园土壤重金属污染特征及健康风险

IF 3.8 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL
Jing Li, Haijing Duan, Jiaheng Li, Yue Liu, Wenjing Huang
{"title":"开封市公园土壤重金属污染特征及健康风险","authors":"Jing Li, Haijing Duan, Jiaheng Li, Yue Liu, Wenjing Huang","doi":"10.1007/s10653-025-02762-9","DOIUrl":null,"url":null,"abstract":"<p><p>To investigate the impact of urban park soils on ecological quality and human health, representative parks with high visitor traffic were selected for this study. A total of 89 soil samples were collected, and the concentrations of seven heavy metals (Cr, Ni, Cu, Zn, Cd, Pb, and Mn) were determined using ICP-MS. Their contamination levels, ecological risks, and human health risks were assessed, and pollution sources were qualitatively identified. The results showed that the average concentrations of ω(Cr), ω(Ni), ω(Cu), ω(Zn), ω(Cd), ω(Pb), and ω(Mn) were 60.33, 30.38, 24.77, 88.51, 0.22, 56.81, and 692.74 mg/kg, respectively, all of which exceeded the local background values. The average order of Igeo for the heavy metals was as follows: Pb (0.86) > Cd (0.65) > Ni (- 0.32) > Mn (- 0.39) > Cr (- 0.45) > Cu (- 0.52) > Zn (- 0.60). The average pollution load index (PLI) was 1.83, with parks P4, P10, and P2 classified as moderately contaminated. Ecological risk assessment indicated that Cd posed the highest single-element risk, and parks P10 and P4 exhibited relatively high ecological risks, while the overall study area maintained a moderate risk level. Health risk assessment revealed that the hazard index (HI) values for both adults and children were below 1, suggesting no significant non-carcinogenic risk. However, the total carcinogenic risk (TCR) for children was more than ten times higher than that for adults. Chromium (Cr) was identified as the major contributing factor, and oral ingestion was determined as the primary exposure route. Monte Carlo simulation further highlighted that children faced higher cumulative non-carcinogenic risks than adults, with key influencing factors being ingestion rate (Ing) for children and dermal contact (SL) for adults. Both groups were within acceptable carcinogenic risk levels, with exposure duration (ED) being the most sensitive parameter.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 10","pages":"451"},"PeriodicalIF":3.8000,"publicationDate":"2025-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Characteristics and health risks of heavy metal pollution in the soil of parks in Kaifeng City.\",\"authors\":\"Jing Li, Haijing Duan, Jiaheng Li, Yue Liu, Wenjing Huang\",\"doi\":\"10.1007/s10653-025-02762-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>To investigate the impact of urban park soils on ecological quality and human health, representative parks with high visitor traffic were selected for this study. A total of 89 soil samples were collected, and the concentrations of seven heavy metals (Cr, Ni, Cu, Zn, Cd, Pb, and Mn) were determined using ICP-MS. Their contamination levels, ecological risks, and human health risks were assessed, and pollution sources were qualitatively identified. The results showed that the average concentrations of ω(Cr), ω(Ni), ω(Cu), ω(Zn), ω(Cd), ω(Pb), and ω(Mn) were 60.33, 30.38, 24.77, 88.51, 0.22, 56.81, and 692.74 mg/kg, respectively, all of which exceeded the local background values. The average order of Igeo for the heavy metals was as follows: Pb (0.86) > Cd (0.65) > Ni (- 0.32) > Mn (- 0.39) > Cr (- 0.45) > Cu (- 0.52) > Zn (- 0.60). The average pollution load index (PLI) was 1.83, with parks P4, P10, and P2 classified as moderately contaminated. Ecological risk assessment indicated that Cd posed the highest single-element risk, and parks P10 and P4 exhibited relatively high ecological risks, while the overall study area maintained a moderate risk level. Health risk assessment revealed that the hazard index (HI) values for both adults and children were below 1, suggesting no significant non-carcinogenic risk. However, the total carcinogenic risk (TCR) for children was more than ten times higher than that for adults. Chromium (Cr) was identified as the major contributing factor, and oral ingestion was determined as the primary exposure route. Monte Carlo simulation further highlighted that children faced higher cumulative non-carcinogenic risks than adults, with key influencing factors being ingestion rate (Ing) for children and dermal contact (SL) for adults. Both groups were within acceptable carcinogenic risk levels, with exposure duration (ED) being the most sensitive parameter.</p>\",\"PeriodicalId\":11759,\"journal\":{\"name\":\"Environmental Geochemistry and Health\",\"volume\":\"47 10\",\"pages\":\"451\"},\"PeriodicalIF\":3.8000,\"publicationDate\":\"2025-09-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Geochemistry and Health\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1007/s10653-025-02762-9\",\"RegionNum\":3,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Geochemistry and Health","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1007/s10653-025-02762-9","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

摘要

为了研究城市公园土壤对生态质量和人类健康的影响,本研究选择了具有代表性的高客流量公园作为研究对象。共采集89份土壤样品,采用ICP-MS法测定了土壤中7种重金属(Cr、Ni、Cu、Zn、Cd、Pb、Mn)的浓度。对其污染程度、生态风险和人类健康风险进行了评估,并定性地确定了污染源。结果表明,该地区ω(Cr)、ω(Ni)、ω(Cu)、ω(Zn)、ω(Cd)、ω(Pb)和ω(Mn)的平均浓度分别为60.33、30.38、24.77、88.51、0.22、56.81和692.74 mg/kg,均超过当地背景值。重金属的平均订单Igeo是如下:Pb(0.86)(0.65) >镍> Cd(- 0.32) >锰(- 0.39)> Cr(- 0.45) >铜(- 0.52)>锌(- 0.60)。平均污染负荷指数(PLI)为1.83,P4、P10和P2公园为中度污染。生态风险评价结果表明,Cd是单要素风险最高的公园,P10和P4公园的生态风险相对较高,而研究区总体处于中等风险水平。健康风险评估显示,成人和儿童的危害指数(HI)值均低于1,表明没有显著的非致癌风险。然而,儿童的总致癌风险(TCR)比成人高出十倍以上。铬(Cr)被确定为主要影响因素,口服摄入被确定为主要暴露途径。蒙特卡罗模拟进一步强调,儿童面临的累积非致癌风险高于成人,关键影响因素是儿童的摄入率(Ing)和成人的皮肤接触率(SL)。两组都在可接受的致癌风险水平内,暴露时间(ED)是最敏感的参数。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Characteristics and health risks of heavy metal pollution in the soil of parks in Kaifeng City.

To investigate the impact of urban park soils on ecological quality and human health, representative parks with high visitor traffic were selected for this study. A total of 89 soil samples were collected, and the concentrations of seven heavy metals (Cr, Ni, Cu, Zn, Cd, Pb, and Mn) were determined using ICP-MS. Their contamination levels, ecological risks, and human health risks were assessed, and pollution sources were qualitatively identified. The results showed that the average concentrations of ω(Cr), ω(Ni), ω(Cu), ω(Zn), ω(Cd), ω(Pb), and ω(Mn) were 60.33, 30.38, 24.77, 88.51, 0.22, 56.81, and 692.74 mg/kg, respectively, all of which exceeded the local background values. The average order of Igeo for the heavy metals was as follows: Pb (0.86) > Cd (0.65) > Ni (- 0.32) > Mn (- 0.39) > Cr (- 0.45) > Cu (- 0.52) > Zn (- 0.60). The average pollution load index (PLI) was 1.83, with parks P4, P10, and P2 classified as moderately contaminated. Ecological risk assessment indicated that Cd posed the highest single-element risk, and parks P10 and P4 exhibited relatively high ecological risks, while the overall study area maintained a moderate risk level. Health risk assessment revealed that the hazard index (HI) values for both adults and children were below 1, suggesting no significant non-carcinogenic risk. However, the total carcinogenic risk (TCR) for children was more than ten times higher than that for adults. Chromium (Cr) was identified as the major contributing factor, and oral ingestion was determined as the primary exposure route. Monte Carlo simulation further highlighted that children faced higher cumulative non-carcinogenic risks than adults, with key influencing factors being ingestion rate (Ing) for children and dermal contact (SL) for adults. Both groups were within acceptable carcinogenic risk levels, with exposure duration (ED) being the most sensitive parameter.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信