Moiz I. Butt , Abdullah G. Weiss , Erik J. Pavlina , Thomas J. Nizolek , Michael A. Hahn , Caitlin A. Kohnert , Sean M. McDeavitt , Erik P. Luther
{"title":"900 K时氢浓度对氢化物中子缓和的影响","authors":"Moiz I. Butt , Abdullah G. Weiss , Erik J. Pavlina , Thomas J. Nizolek , Michael A. Hahn , Caitlin A. Kohnert , Sean M. McDeavitt , Erik P. Luther","doi":"10.1016/j.anucene.2025.111852","DOIUrl":null,"url":null,"abstract":"<div><div>The neutron attenuation and permeation characteristics of several metal hydrides were studied to determine the efficacy of metal hydrides as neutron moderators and shields. These metal hydrides comprised yttrium, zirconium, and yttrium-chromium-based hydrides and deuterides. Neutron attenuation coefficients (<span><math><msub><mi>μ</mi><mi>n</mi></msub></math></span>) and neutron permeation coefficients (<span><math><msub><mi>ξ</mi><mi>n</mi></msub></math></span>) of these hydrides were determined using Monte Carlo N-Particle (MCNP) transport simulations. The effect of impurities on the moderating efficacy of specific hydrides was evaluated by comparing ideal, or pure, hydride compositions with hydrides of metals containing impurity levels typical of commercially available metal alloys. The analysis showed that metal alloy hydrides, particularly those of a yttrium-5 wt% chromium and other impurity containing yttrium materials do not significantly decrease the moderating capability of the moderator when compared to pure yttrium. The analysis also compared the difference in moderating capabilities between the different hydrides of yttrium and zirconium, where zirconium performs better for neutron attenuation, but yttrium performs better with respect to neutron permeation over the range of energies investigated.</div></div>","PeriodicalId":8006,"journal":{"name":"Annals of Nuclear Energy","volume":"226 ","pages":"Article 111852"},"PeriodicalIF":2.3000,"publicationDate":"2025-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Effect of hydrogen concentration on neutron moderation of hydrides at 900 K\",\"authors\":\"Moiz I. Butt , Abdullah G. Weiss , Erik J. Pavlina , Thomas J. Nizolek , Michael A. Hahn , Caitlin A. Kohnert , Sean M. McDeavitt , Erik P. Luther\",\"doi\":\"10.1016/j.anucene.2025.111852\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The neutron attenuation and permeation characteristics of several metal hydrides were studied to determine the efficacy of metal hydrides as neutron moderators and shields. These metal hydrides comprised yttrium, zirconium, and yttrium-chromium-based hydrides and deuterides. Neutron attenuation coefficients (<span><math><msub><mi>μ</mi><mi>n</mi></msub></math></span>) and neutron permeation coefficients (<span><math><msub><mi>ξ</mi><mi>n</mi></msub></math></span>) of these hydrides were determined using Monte Carlo N-Particle (MCNP) transport simulations. The effect of impurities on the moderating efficacy of specific hydrides was evaluated by comparing ideal, or pure, hydride compositions with hydrides of metals containing impurity levels typical of commercially available metal alloys. The analysis showed that metal alloy hydrides, particularly those of a yttrium-5 wt% chromium and other impurity containing yttrium materials do not significantly decrease the moderating capability of the moderator when compared to pure yttrium. The analysis also compared the difference in moderating capabilities between the different hydrides of yttrium and zirconium, where zirconium performs better for neutron attenuation, but yttrium performs better with respect to neutron permeation over the range of energies investigated.</div></div>\",\"PeriodicalId\":8006,\"journal\":{\"name\":\"Annals of Nuclear Energy\",\"volume\":\"226 \",\"pages\":\"Article 111852\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2025-09-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Annals of Nuclear Energy\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0306454925006693\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"NUCLEAR SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Annals of Nuclear Energy","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0306454925006693","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Effect of hydrogen concentration on neutron moderation of hydrides at 900 K
The neutron attenuation and permeation characteristics of several metal hydrides were studied to determine the efficacy of metal hydrides as neutron moderators and shields. These metal hydrides comprised yttrium, zirconium, and yttrium-chromium-based hydrides and deuterides. Neutron attenuation coefficients () and neutron permeation coefficients () of these hydrides were determined using Monte Carlo N-Particle (MCNP) transport simulations. The effect of impurities on the moderating efficacy of specific hydrides was evaluated by comparing ideal, or pure, hydride compositions with hydrides of metals containing impurity levels typical of commercially available metal alloys. The analysis showed that metal alloy hydrides, particularly those of a yttrium-5 wt% chromium and other impurity containing yttrium materials do not significantly decrease the moderating capability of the moderator when compared to pure yttrium. The analysis also compared the difference in moderating capabilities between the different hydrides of yttrium and zirconium, where zirconium performs better for neutron attenuation, but yttrium performs better with respect to neutron permeation over the range of energies investigated.
期刊介绍:
Annals of Nuclear Energy provides an international medium for the communication of original research, ideas and developments in all areas of the field of nuclear energy science and technology. Its scope embraces nuclear fuel reserves, fuel cycles and cost, materials, processing, system and component technology (fission only), design and optimization, direct conversion of nuclear energy sources, environmental control, reactor physics, heat transfer and fluid dynamics, structural analysis, fuel management, future developments, nuclear fuel and safety, nuclear aerosol, neutron physics, computer technology (both software and hardware), risk assessment, radioactive waste disposal and reactor thermal hydraulics. Papers submitted to Annals need to demonstrate a clear link to nuclear power generation/nuclear engineering. Papers which deal with pure nuclear physics, pure health physics, imaging, or attenuation and shielding properties of concretes and various geological materials are not within the scope of the journal. Also, papers that deal with policy or economics are not within the scope of the journal.