Zi-Lun Li , Liang Zheng , Li-Hua Wang , Yi-Qian Wei , Hai-Long Liao , Guang-Wen Chu , Yong Luo , Jian-Feng Chen
{"title":"绿色化工用内循环旋转填料床:提液器结构优化","authors":"Zi-Lun Li , Liang Zheng , Li-Hua Wang , Yi-Qian Wei , Hai-Long Liao , Guang-Wen Chu , Yong Luo , Jian-Feng Chen","doi":"10.1016/j.gce.2025.05.008","DOIUrl":null,"url":null,"abstract":"<div><div>The internal circulation rotating packed beds (IN-RPBs) have been widely used in multiphase systems. However, its key component's liquid lifter suffers from the liquid lifting rate (<em>Q</em><sub>L</sub>), limiting the micro-mixing and mass transfer efficiency. In this study, the fluid motion inside the conventional lifter was theoretically analyzed. Based on the above theoretical analysis, a new impeller-equipped lifter was innovatively designed for the IN-RPB to enhance <em>Q</em><sub>L</sub>. Experiment results showed that <em>Q</em><sub>L</sub> was increased by 100% at 1400 r/min within the impeller-equipped lifter. Numerical simulations demonstrated that the flow field was altered in the impeller-equipped lifter, promoting the generation of vortices, thereby increasing the <em>Q</em><sub>L</sub>. Mass transfer experiments demonstrated that the structure optimization of the lifter led to a 60% increase in the gas-liquid volumetric mass transfer coefficient (<em>k</em><sub>L</sub><em>a</em>). This study provides a basis for the industrialization of the IN-RPB with an impeller-equipped lifter.</div></div>","PeriodicalId":66474,"journal":{"name":"Green Chemical Engineering","volume":"6 4","pages":"Pages 551-561"},"PeriodicalIF":7.6000,"publicationDate":"2025-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"An internal circulation rotating packed bed for green chemical engineering: structure optimization of liquid lifter\",\"authors\":\"Zi-Lun Li , Liang Zheng , Li-Hua Wang , Yi-Qian Wei , Hai-Long Liao , Guang-Wen Chu , Yong Luo , Jian-Feng Chen\",\"doi\":\"10.1016/j.gce.2025.05.008\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The internal circulation rotating packed beds (IN-RPBs) have been widely used in multiphase systems. However, its key component's liquid lifter suffers from the liquid lifting rate (<em>Q</em><sub>L</sub>), limiting the micro-mixing and mass transfer efficiency. In this study, the fluid motion inside the conventional lifter was theoretically analyzed. Based on the above theoretical analysis, a new impeller-equipped lifter was innovatively designed for the IN-RPB to enhance <em>Q</em><sub>L</sub>. Experiment results showed that <em>Q</em><sub>L</sub> was increased by 100% at 1400 r/min within the impeller-equipped lifter. Numerical simulations demonstrated that the flow field was altered in the impeller-equipped lifter, promoting the generation of vortices, thereby increasing the <em>Q</em><sub>L</sub>. Mass transfer experiments demonstrated that the structure optimization of the lifter led to a 60% increase in the gas-liquid volumetric mass transfer coefficient (<em>k</em><sub>L</sub><em>a</em>). This study provides a basis for the industrialization of the IN-RPB with an impeller-equipped lifter.</div></div>\",\"PeriodicalId\":66474,\"journal\":{\"name\":\"Green Chemical Engineering\",\"volume\":\"6 4\",\"pages\":\"Pages 551-561\"},\"PeriodicalIF\":7.6000,\"publicationDate\":\"2025-05-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Green Chemical Engineering\",\"FirstCategoryId\":\"1089\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2666952825000457\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Green Chemical Engineering","FirstCategoryId":"1089","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2666952825000457","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
An internal circulation rotating packed bed for green chemical engineering: structure optimization of liquid lifter
The internal circulation rotating packed beds (IN-RPBs) have been widely used in multiphase systems. However, its key component's liquid lifter suffers from the liquid lifting rate (QL), limiting the micro-mixing and mass transfer efficiency. In this study, the fluid motion inside the conventional lifter was theoretically analyzed. Based on the above theoretical analysis, a new impeller-equipped lifter was innovatively designed for the IN-RPB to enhance QL. Experiment results showed that QL was increased by 100% at 1400 r/min within the impeller-equipped lifter. Numerical simulations demonstrated that the flow field was altered in the impeller-equipped lifter, promoting the generation of vortices, thereby increasing the QL. Mass transfer experiments demonstrated that the structure optimization of the lifter led to a 60% increase in the gas-liquid volumetric mass transfer coefficient (kLa). This study provides a basis for the industrialization of the IN-RPB with an impeller-equipped lifter.