Antonio Cobarrubia, Sancia M. Tauro, Joshua R. Hendrickson and Sanjay K. Behura*,
{"title":"六方氮化硼量子发射极SLH张量网络的表征","authors":"Antonio Cobarrubia, Sancia M. Tauro, Joshua R. Hendrickson and Sanjay K. Behura*, ","doi":"10.1021/acs.jpcc.5c02502","DOIUrl":null,"url":null,"abstract":"<p >Defect-based quantum emitters in hexagonal boron nitride (hBN) are promising for the development of photonic qubits. However, the quantum emission based on spin-optical properties of defects has yet to be fully understood at room temperature due to the multienvironmental interactions. In this work, we utilize a quantum input–output network framework to develop a tensor network state, that describes the photon emission in the boron vacancy quantum defect, <i>V</i><sub><i>B</i></sub><sup>–</sup>, as an SLH triple, <i>G</i><sub>hBN</sub>. We showcase a time-evolving block decimation algorithm to simulate the spin-optical properties, which incorporate multitime scale of slow and fast state transitions with their bond dimensions that grow to a polynomial order. We investigated the effects of a coherent state stimulating the radiative port of <i>G</i><sub>hBN</sub>, highlighting the output photon emission of characteristic slow and fast radiative decay rates. Our results and methodology demonstrate that defect-based quantum emission in hBN is influenced by the time scale of the radiative lifetime and the influx of photons at the input port of <i>G</i><sub>hBN</sub>.</p>","PeriodicalId":61,"journal":{"name":"The Journal of Physical Chemistry C","volume":"129 32","pages":"14430–14439"},"PeriodicalIF":3.2000,"publicationDate":"2025-08-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Characterization of Hexagonal Boron Nitride Quantum Emitter as an SLH Tensor Network\",\"authors\":\"Antonio Cobarrubia, Sancia M. Tauro, Joshua R. Hendrickson and Sanjay K. Behura*, \",\"doi\":\"10.1021/acs.jpcc.5c02502\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Defect-based quantum emitters in hexagonal boron nitride (hBN) are promising for the development of photonic qubits. However, the quantum emission based on spin-optical properties of defects has yet to be fully understood at room temperature due to the multienvironmental interactions. In this work, we utilize a quantum input–output network framework to develop a tensor network state, that describes the photon emission in the boron vacancy quantum defect, <i>V</i><sub><i>B</i></sub><sup>–</sup>, as an SLH triple, <i>G</i><sub>hBN</sub>. We showcase a time-evolving block decimation algorithm to simulate the spin-optical properties, which incorporate multitime scale of slow and fast state transitions with their bond dimensions that grow to a polynomial order. We investigated the effects of a coherent state stimulating the radiative port of <i>G</i><sub>hBN</sub>, highlighting the output photon emission of characteristic slow and fast radiative decay rates. Our results and methodology demonstrate that defect-based quantum emission in hBN is influenced by the time scale of the radiative lifetime and the influx of photons at the input port of <i>G</i><sub>hBN</sub>.</p>\",\"PeriodicalId\":61,\"journal\":{\"name\":\"The Journal of Physical Chemistry C\",\"volume\":\"129 32\",\"pages\":\"14430–14439\"},\"PeriodicalIF\":3.2000,\"publicationDate\":\"2025-08-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"The Journal of Physical Chemistry C\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.jpcc.5c02502\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"The Journal of Physical Chemistry C","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.jpcc.5c02502","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Characterization of Hexagonal Boron Nitride Quantum Emitter as an SLH Tensor Network
Defect-based quantum emitters in hexagonal boron nitride (hBN) are promising for the development of photonic qubits. However, the quantum emission based on spin-optical properties of defects has yet to be fully understood at room temperature due to the multienvironmental interactions. In this work, we utilize a quantum input–output network framework to develop a tensor network state, that describes the photon emission in the boron vacancy quantum defect, VB–, as an SLH triple, GhBN. We showcase a time-evolving block decimation algorithm to simulate the spin-optical properties, which incorporate multitime scale of slow and fast state transitions with their bond dimensions that grow to a polynomial order. We investigated the effects of a coherent state stimulating the radiative port of GhBN, highlighting the output photon emission of characteristic slow and fast radiative decay rates. Our results and methodology demonstrate that defect-based quantum emission in hBN is influenced by the time scale of the radiative lifetime and the influx of photons at the input port of GhBN.
期刊介绍:
The Journal of Physical Chemistry A/B/C is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, and chemical physicists.