分数态下磁场与自旋子的相互作用

IF 6.2 1区 物理与天体物理 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Yu Zhang, Hengdi Zhao, Tristan R. Cao, Rahul Nandkishore, Pedro Schlottmann, Lance De Long, Gang Cao
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引用次数: 0

摘要

四维电子三聚体晶格Ba₄Nb₁₃ₓRu₃₊ₓO₁₂表现为量子自旋液体(QSL)或重费米子奇异金属(HFSM)相,具体取决于Nb含量。在QSL状态下,流动的自旋子作为有效的热载体,增强了导热性。引人注目的是,施加高达14 T的磁场会导致热容量在150 mK以下突然增加高达5000%,从而破坏了两相典型的线性温度依赖性。同时,交流电阻率和电阻率几乎保持不变,而导热系数在4 K以下下降了40%。这些结果表明,尽管自旋子是电荷中性的,但在低温下对磁场高度敏感。我们提出磁场可以诱导自旋子的安德森局域化,从而产生导致热容类似肖特基异常的非磁性双能级系统。这些发现指出了一个以前未被探索的自旋子动力学机制,可能由场诱导的局部化控制,与传统的磁性或输运特征不同。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Interaction of magnetic fields with spinons in a fractionalized state

Interaction of magnetic fields with spinons in a fractionalized state

The 4d-electron trimer lattice Ba₄Nb₁₋Ru₃₊O₁₂ exhibits either a quantum spin liquid (QSL) or a heavy-fermion strange metal (HFSM) phase, depending on Nb content. In the QSL state, itinerant spinons act as effective heat carriers, enhancing thermal conductivity. Strikingly, applying a magnetic field up to 14 T causes an abrupt, up-to-5000% increase in heat capacity below 150 mK, disrupting the linear temperature dependence typical of both phases. Meanwhile, AC susceptibility and electrical resistivity remain nearly unchanged, while thermal conductivity drops by up to 40% below 4 K. These results suggest spinons, despite being charge-neutral, are highly sensitive to magnetic fields at low temperatures. We propose that the magnetic field could induce Anderson localization of spinons, creating emergent non-magnetic two-level systems responsible for the Schottky-like anomaly in heat capacity. These findings point to a previously unexplored regime of spinon dynamics, potentially governed by field-induced localization and distinct from conventional magnetic or transport signatures.

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来源期刊
npj Quantum Materials
npj Quantum Materials Materials Science-Electronic, Optical and Magnetic Materials
CiteScore
10.60
自引率
3.50%
发文量
107
审稿时长
6 weeks
期刊介绍: npj Quantum Materials is an open access journal that publishes works that significantly advance the understanding of quantum materials, including their fundamental properties, fabrication and applications.
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