基于多指标加权有机污染物优先度评分系统的煤矿土壤有机污染物优先度排序。

IF 3.8 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL
Wenhan Liu, Shuhao Zhang, Wenxiu Xue, Xiufeng Cao, Jia Liu, Xiaowei Cui, Zhaojie Cui
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引用次数: 0

摘要

土壤中有机污染物的积累和多样性表明迫切需要一种系统的优先排序方法。本研究建立了优先有机污染物评分系统(POPSS),对煤矿土壤中有机磷进行了优先排序。POPSS采用加权综合评分系统,综合考虑浓度、毒性、环境行为和管理可行性四个方面。根据政府文件、调查报告和其他材料,将63类潜在OPs列为潜在OPs列表。然后对项目进行优先排序,并将其列为详细的项目清单。苯(B)、多氯联苯169 (PCB 169)、总石油烃(TPH)、苯并[a]芘(BaP)、多氯二苯并对二恶英和多氯二苯并呋喃(PCDD/Fs)占据前5位,被列为突出的OPs列表。从OP类别来看,多氯联苯、多环芳烃(PAHs)、TPH和PCDD/Fs因其等级明显较高而成为值得关注的OP。分析了多环芳烃不同指标的特征,揭示了多环芳烃在煤矿土壤中的广泛存在,多氯联苯具有较高的生物蓄积潜力和持久性,钛酸类化合物的毒性值得注意。本研究开发的POPSS可用于评价不同类型土壤环境中有机磷的优先度,并可为不同应用场景下的政府政策和环境立法提供参考。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Prioritization of organic contaminants in coal mine soils based on a proposed priority organic pollutant scoring system with multi-criterion weighting.

The accumulation and diversity of organic pollutants (OPs) in soil underscore the urgent need for a systematic prioritization method. This study developed a priority organic pollutant scoring system (POPSS) and conducted prioritization of OPs in coal mine soil. The POPSS utilized a weighted integrated scoring system, considering four aspects covering concentration, toxicity, environmental behavior and management feasibility. Sixty-three (63) classes of potential OPs were listed as potential OPs list, based on government documents, investigation reports, and other materials. The OPs were then prioritized and ranked as detailed OPs list. Benzene (B), poly-chlorinated biphenyl 169 (PCB 169), total petroleum hydrocarbon (TPH), Benzo[a]pyrene (BaP), and polychlorinated dibenzo-p-dioxins and Polychlorinated dibenzofurans (PCDD/Fs) occupied the top five scores and were listed as prominent OPs list. From the perspective of OP categories, PCBs, polycyclic aromatic hydrocarbons (PAHs), TPH and PCDD/Fs emerge as noteworthy OPs due to their significantly higher ratings. The characteristics of different indicators of OPs have also been analyzed, revealing the widespread presence of PAHs in coal mine soil, the high bio-accumulation potential and persistence of PCBs, and the noteworthy toxicity of titanate compounds. The POPSS developed in this study can be applied to evaluate the priority of OPs in various types of soil environments and can be used as a reference for governmental policies and environmental legislation in various application scenarios.

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来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
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