非均匀弹性系统的反常态密度与均匀热化的准局域振动。

Cunyuan Jiang
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引用次数: 0

摘要

由于缺乏平移对称性,非晶固体表现出动态不均匀性,导致与结晶固体相比具有不同的振动特性。这些包括异常低频振动态密度(VDOS)和相关的低温热行为偏差。虽然粒子水平的研究进展迅速,但基于物理定律对这些现象的基本解释仍然不发达。在这项工作中,我们从准平衡条件开始,它要求弹性势能在长时间尺度上均匀分布在非均匀弹性固体中。分析结果表明,当弹性非均匀体系施加准平衡时,会出现低频异常VDOS标度\(D(\omega) \propto \omega^4\)。在更高的频率下,超越了由非均匀性长度尺度决定的交叉,VDOS转变为\(D(\omega) \propto \omega^2\),与晶体的德拜定律一致。这些发现与最近的粒子水平研究一致,表明非晶固体中普遍的低频异常是由均匀热化引起的。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The anomalous density of states and quasi-localized vibration through homogeneous thermalization of an inhomogeneous elastic system.

Amorphous solids exhibit dynamic inhomogeneity due to their lack of translational symmetry, leading to distinct vibrational properties compared to crystalline solids. These include anomalous low-frequency vibrational density of states (VDOS) and associated deviations in low-temperature thermal behavior. While particle-level investigations have advanced rapidly, a fundamental interpretation of these phenomena based on physical laws remains underdeveloped. In this work, we begin with the quasi-equilibrium condition, which mandates a homogeneous distribution of elastic potential energy in an inhomogeneous elastic solid over long timescales. The analytical results suggest that the anomalous low-frequency VDOS scalingD(ω)∝ω4emerges when quasi-equilibrium is imposed on an elastically inhomogeneous system. At higher frequencies, beyond a crossover dictated by the length scale of inhomogeneity, the VDOS transitions toD(ω)∝ω2, consistent with Debye's law for crystals. These findings align with recent particle-level studies and suggests that the universal low-frequency anomaly in amorphous solids arises from homogeneous thermalization.

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