三角形反铁磁体K2Co(SeO3)2的万尼尔态和自旋超固体物理

IF 5.4 1区 物理与天体物理 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
M. Zhu, Leandro M. Chinellato, V. Romerio, N. Murai, S. Ohira-Kawamura, Christian Balz, Z. Yan, S. Gvasaliya, Yasuyuki Kato, C. D. Batista, A. Zheludev
{"title":"三角形反铁磁体K2Co(SeO3)2的万尼尔态和自旋超固体物理","authors":"M. Zhu, Leandro M. Chinellato, V. Romerio, N. Murai, S. Ohira-Kawamura, Christian Balz, Z. Yan, S. Gvasaliya, Yasuyuki Kato, C. D. Batista, A. Zheludev","doi":"10.1038/s41535-025-00791-2","DOIUrl":null,"url":null,"abstract":"<p>We combine ultra-high-resolution inelastic neutron scattering and quantum Monte Carlo simulations to study thermodynamics and spin excitations in the spin-supersolid phase of the triangular lattice XXZ antiferromagnet K<sub>2</sub>Co(SeO<sub>3</sub>)<sub>2</sub> under zero and non-zero magnetic field. BKT transitions signaling the onset of Ising and supersolid order are clearly identified, and the Wannier entropy is experimentally recovered just above the supersolid phase. At low temperatures, with an experimental resolution of about 23 μeV, no discrete coherent magnon modes are resolved within a broad scattering continuum. Alongside gapless excitations, a pseudo-Goldstone mode with a 0.06 meV gap is observed. A second, higher-energy continuum replaces single-spin-flip excitations of the Ising model. Under applied fields, the continuum evolves into coherent spin waves, with Goldstone and pseudo-Goldstone sectors responding differently. The experiments and simulations show excellent quantitative agreement.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":"7 1","pages":""},"PeriodicalIF":5.4000,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Wannier states and spin supersolid physics in the triangular antiferromagnet K2Co(SeO3)2\",\"authors\":\"M. Zhu, Leandro M. Chinellato, V. Romerio, N. Murai, S. Ohira-Kawamura, Christian Balz, Z. Yan, S. Gvasaliya, Yasuyuki Kato, C. D. Batista, A. Zheludev\",\"doi\":\"10.1038/s41535-025-00791-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>We combine ultra-high-resolution inelastic neutron scattering and quantum Monte Carlo simulations to study thermodynamics and spin excitations in the spin-supersolid phase of the triangular lattice XXZ antiferromagnet K<sub>2</sub>Co(SeO<sub>3</sub>)<sub>2</sub> under zero and non-zero magnetic field. BKT transitions signaling the onset of Ising and supersolid order are clearly identified, and the Wannier entropy is experimentally recovered just above the supersolid phase. At low temperatures, with an experimental resolution of about 23 μeV, no discrete coherent magnon modes are resolved within a broad scattering continuum. Alongside gapless excitations, a pseudo-Goldstone mode with a 0.06 meV gap is observed. A second, higher-energy continuum replaces single-spin-flip excitations of the Ising model. Under applied fields, the continuum evolves into coherent spin waves, with Goldstone and pseudo-Goldstone sectors responding differently. The experiments and simulations show excellent quantitative agreement.</p>\",\"PeriodicalId\":19283,\"journal\":{\"name\":\"npj Quantum Materials\",\"volume\":\"7 1\",\"pages\":\"\"},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2025-07-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"npj Quantum Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41535-025-00791-2\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"npj Quantum Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41535-025-00791-2","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

结合超高分辨率非弹性中子散射和量子蒙特卡罗模拟,研究了三角形晶格XXZ反铁磁体K2Co(SeO3)2在零磁场和非零磁场下的自旋超固相热力学和自旋激发。BKT跃迁信号表明了伊辛和超固序的开始,并且在实验中恢复了超固相上方的万尼尔熵。在低温下,实验分辨率约为23 μeV,在广泛的散射连续区内没有分离的相干磁振子模式。除了无间隙激发外,还观察到具有0.06 meV间隙的伪goldstone模式。第二种能量更高的连续体取代了伊辛模型的单自旋翻转激发。在应用领域中,连续体演变成相干自旋波,戈德斯通和伪戈德斯通扇区的响应不同。实验和模拟结果显示了极好的定量一致性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Wannier states and spin supersolid physics in the triangular antiferromagnet K2Co(SeO3)2

Wannier states and spin supersolid physics in the triangular antiferromagnet K2Co(SeO3)2

We combine ultra-high-resolution inelastic neutron scattering and quantum Monte Carlo simulations to study thermodynamics and spin excitations in the spin-supersolid phase of the triangular lattice XXZ antiferromagnet K2Co(SeO3)2 under zero and non-zero magnetic field. BKT transitions signaling the onset of Ising and supersolid order are clearly identified, and the Wannier entropy is experimentally recovered just above the supersolid phase. At low temperatures, with an experimental resolution of about 23 μeV, no discrete coherent magnon modes are resolved within a broad scattering continuum. Alongside gapless excitations, a pseudo-Goldstone mode with a 0.06 meV gap is observed. A second, higher-energy continuum replaces single-spin-flip excitations of the Ising model. Under applied fields, the continuum evolves into coherent spin waves, with Goldstone and pseudo-Goldstone sectors responding differently. The experiments and simulations show excellent quantitative agreement.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
npj Quantum Materials
npj Quantum Materials Materials Science-Electronic, Optical and Magnetic Materials
CiteScore
10.60
自引率
3.50%
发文量
107
审稿时长
6 weeks
期刊介绍: npj Quantum Materials is an open access journal that publishes works that significantly advance the understanding of quantum materials, including their fundamental properties, fabrication and applications.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信