基于[2.2]副环环烷的铰链状机械致色团。

Shohei Shimizu, Jess M Clough, Christoph Weder, Yoshimitsu Sagara
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引用次数: 0

摘要

提出了一种基于[2.2]副环烷核和两个准分子形成的1,6-二(苯基乙炔)芘发光基团的铰链状超分子机械基团。每个发光团与[2.2]副环环烷共享一个苯基,导致刚性和张力结构,迫使两个发光团靠近。因此,机械团在THF溶液和含有新基元的聚氨酯固体膜中的光致发光主要是准分子发射。拉伸聚合物薄膜会导致从亮黄色准分子到蓝绿色单体为主的明显变化。准分子与单体发射强度之比可以跟踪聚合物井的非线性应力-应变曲线,是宏观施力的良好指标。机械反应的可逆性、理论分析和类似的机械基团(发射体和[2.2]副环环烷核心通过柔性连接体连接)的参考实验支持这样的结论,即机械激活是由分子扭曲成弯曲的、更开放的构象而不是共价键的断裂引起的。通过研究基于[2.2]副环烷核心和1,4-双(苯乙基)苯发射体的第二种铰链状机械基团,进一步证实了该工作原理。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Hinge-Like Mechanochromic Mechanophores Based on [2.2]Paracyclophane.

A hinge-like supramolecular mechanophore based on a [2.2]paracyclophane core and two excimer-forming 1,6-bis(phenylethynyl)pyrene luminophores is presented. Each luminophore shares one phenyl group with the [2.2]paracyclophane, resulting in a rigid and strained structure that forces the two luminophores into close proximity. As a consequence, the photoluminescence of the mechanophore in THF solution and in solid films of a polyurethane containing the new motif is dominated by excimer emission. Stretching the polymer films causes an easily discernible change from bright yellow excimer to blue-green monomer-dominated emission. The ratio of excimer to monomer emission intensities traces the nonlinear stress-strain curves of the polymer well and is a good indicator for the macroscopically applied force. The reversibility of the mechanoresponse, theoretical analyses, and reference experiments with a similar mechanophore in which the emitters and the [2.2]paracyclophane core are connected by flexible linkers support the conclusion that the mechanoactivation is caused by distorting the molecule into a bent, more open conformation and not the scission of covalent bonds. The operating principle was further confirmed by investigating a second hinge-like mechanophore based on a [2.2]paracyclophane core and 1,4-bis(phenylethynyl)benzene emitters.

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