Limin Yu, Ru Li, Chong Zhang, Hao Sun, Zhe Zhang, Pengfei Zhao, Pengji Zhang, Fan Yang
{"title":"评估黄海上空大气中无机氮和磷的沉积","authors":"Limin Yu, Ru Li, Chong Zhang, Hao Sun, Zhe Zhang, Pengfei Zhao, Pengji Zhang, Fan Yang","doi":"10.1016/j.rsma.2025.104261","DOIUrl":null,"url":null,"abstract":"<div><div>As an important fishery area in the world, the environmental status of fishery resources in the Yellow Sea is closely related to atmospheric deposition. Considering the differences in the distribution of atmospheric pollutants in different regions, in order to improve the accuracy of the assessment, the Yellow Sea was divided into three representative regions, and a method for assessing the deposition fluxes of inorganic nitrogen (DIN) and phosphorus (DIP) in large-scale marine atmospheres was constructed. Based on the particle size distribution of atmospheric particulate DIN and DIP in 10 subsections, the dry deposition rates of different DIN and DIP were obtained by refinement. On this basis, atmospheric deposition of DIN and DIP to the Yellow Sea were estimated by combining the collected measured data and empirical coefficient estimations. The results showed that in 2017 the dry deposition of atmospheric DIN in the Yellow Sea was equal to 1.71 × 10<sup>5</sup> t. NO<sub>3</sub><sup>-</sup>-N was the most important component in the dry deposition of DIN (74.3 %), followed by NH<sub>4</sub><sup>+</sup>-N (24.4 %). Unlike dry deposition, the wet deposition amount of NH<sub>4</sub><sup>+</sup>-N (2.55 × 10<sup>5</sup> t) was higher than that of NO<sub>3</sub><sup>-</sup>-N (2.02 × 10<sup>5</sup> t). The amounts of total deposition of NO<sub>3</sub><sup>-</sup>-N, NH<sub>4</sub><sup>+</sup>-N, NO<sub>2</sub><sup>-</sup>-N, and DIP were 3.29 × 10<sup>5</sup> t, 2.89 × 10<sup>5</sup> t, 4.94 × 10<sup>3</sup> t, and 2.93 × 10<sup>3</sup> t, respectively. In the Western Yellow Sea, the amounts of DIN inputs from the atmosphere and from rivers were comparable. The fluxes of NO<sub>3</sub><sup>-</sup>-N and DIP from rivers are significantly higher than those from atmosphere, while the opposite is true for NH<sub>4</sub><sup>+</sup>-N. So the contribution of atmospheric deposition to the input of nutrients in the Yellow Sea cannot be ignored. The total atmospheric deposition fluxes of DIN and DIP were highest in summer, which may be related to the high incidence of harmful algal blooms during the summer period.</div></div>","PeriodicalId":21070,"journal":{"name":"Regional Studies in Marine Science","volume":"89 ","pages":"Article 104261"},"PeriodicalIF":2.1000,"publicationDate":"2025-05-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Assessing the atmospheric deposition of inorganic nitrogen and phosphorus over the Yellow Sea\",\"authors\":\"Limin Yu, Ru Li, Chong Zhang, Hao Sun, Zhe Zhang, Pengfei Zhao, Pengji Zhang, Fan Yang\",\"doi\":\"10.1016/j.rsma.2025.104261\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>As an important fishery area in the world, the environmental status of fishery resources in the Yellow Sea is closely related to atmospheric deposition. Considering the differences in the distribution of atmospheric pollutants in different regions, in order to improve the accuracy of the assessment, the Yellow Sea was divided into three representative regions, and a method for assessing the deposition fluxes of inorganic nitrogen (DIN) and phosphorus (DIP) in large-scale marine atmospheres was constructed. Based on the particle size distribution of atmospheric particulate DIN and DIP in 10 subsections, the dry deposition rates of different DIN and DIP were obtained by refinement. On this basis, atmospheric deposition of DIN and DIP to the Yellow Sea were estimated by combining the collected measured data and empirical coefficient estimations. The results showed that in 2017 the dry deposition of atmospheric DIN in the Yellow Sea was equal to 1.71 × 10<sup>5</sup> t. NO<sub>3</sub><sup>-</sup>-N was the most important component in the dry deposition of DIN (74.3 %), followed by NH<sub>4</sub><sup>+</sup>-N (24.4 %). Unlike dry deposition, the wet deposition amount of NH<sub>4</sub><sup>+</sup>-N (2.55 × 10<sup>5</sup> t) was higher than that of NO<sub>3</sub><sup>-</sup>-N (2.02 × 10<sup>5</sup> t). The amounts of total deposition of NO<sub>3</sub><sup>-</sup>-N, NH<sub>4</sub><sup>+</sup>-N, NO<sub>2</sub><sup>-</sup>-N, and DIP were 3.29 × 10<sup>5</sup> t, 2.89 × 10<sup>5</sup> t, 4.94 × 10<sup>3</sup> t, and 2.93 × 10<sup>3</sup> t, respectively. In the Western Yellow Sea, the amounts of DIN inputs from the atmosphere and from rivers were comparable. The fluxes of NO<sub>3</sub><sup>-</sup>-N and DIP from rivers are significantly higher than those from atmosphere, while the opposite is true for NH<sub>4</sub><sup>+</sup>-N. So the contribution of atmospheric deposition to the input of nutrients in the Yellow Sea cannot be ignored. The total atmospheric deposition fluxes of DIN and DIP were highest in summer, which may be related to the high incidence of harmful algal blooms during the summer period.</div></div>\",\"PeriodicalId\":21070,\"journal\":{\"name\":\"Regional Studies in Marine Science\",\"volume\":\"89 \",\"pages\":\"Article 104261\"},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2025-05-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Regional Studies in Marine Science\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S235248552500252X\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ECOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Regional Studies in Marine Science","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S235248552500252X","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ECOLOGY","Score":null,"Total":0}
Assessing the atmospheric deposition of inorganic nitrogen and phosphorus over the Yellow Sea
As an important fishery area in the world, the environmental status of fishery resources in the Yellow Sea is closely related to atmospheric deposition. Considering the differences in the distribution of atmospheric pollutants in different regions, in order to improve the accuracy of the assessment, the Yellow Sea was divided into three representative regions, and a method for assessing the deposition fluxes of inorganic nitrogen (DIN) and phosphorus (DIP) in large-scale marine atmospheres was constructed. Based on the particle size distribution of atmospheric particulate DIN and DIP in 10 subsections, the dry deposition rates of different DIN and DIP were obtained by refinement. On this basis, atmospheric deposition of DIN and DIP to the Yellow Sea were estimated by combining the collected measured data and empirical coefficient estimations. The results showed that in 2017 the dry deposition of atmospheric DIN in the Yellow Sea was equal to 1.71 × 105 t. NO3--N was the most important component in the dry deposition of DIN (74.3 %), followed by NH4+-N (24.4 %). Unlike dry deposition, the wet deposition amount of NH4+-N (2.55 × 105 t) was higher than that of NO3--N (2.02 × 105 t). The amounts of total deposition of NO3--N, NH4+-N, NO2--N, and DIP were 3.29 × 105 t, 2.89 × 105 t, 4.94 × 103 t, and 2.93 × 103 t, respectively. In the Western Yellow Sea, the amounts of DIN inputs from the atmosphere and from rivers were comparable. The fluxes of NO3--N and DIP from rivers are significantly higher than those from atmosphere, while the opposite is true for NH4+-N. So the contribution of atmospheric deposition to the input of nutrients in the Yellow Sea cannot be ignored. The total atmospheric deposition fluxes of DIN and DIP were highest in summer, which may be related to the high incidence of harmful algal blooms during the summer period.
期刊介绍:
REGIONAL STUDIES IN MARINE SCIENCE will publish scientifically sound papers on regional aspects of maritime and marine resources in estuaries, coastal zones, continental shelf, the seas and oceans.