共振非弹性x射线散射探测扩展相关系统中电子-声子相互作用理论

IF 11.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY
Jinu Thomas, Debshikha Banerjee, Alberto Nocera, Steven Johnston
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引用次数: 0

摘要

共振非弹性x射线散射(RIXS)的一个新兴应用是研究量子材料中的晶格激发和电子-声子(e-ph)相互作用。尽管这一领域的研究越来越重要,但学界对RIXS过程如何激发晶格以及这些激发如何编码有关e-ph相互作用的信息缺乏完整的理解。在这里,我们详细研究了扩展一维晶格上定义的hubard - holstein模型的RIXS光谱。利用密度矩阵重整化群方法,我们计算了RIXS响应,同时平等地处理了电子迁移率、多体相互作用和核心-空穴相互作用。预测光谱与通常采用的Lang-Firsov模型得到的结果有显著差异,这对分析过去和未来的实验具有重要意义。我们的结果提供了对RIXS如何探测e-ph相互作用的更深入理解,并为未来实验的更现实分析奠定了基础。2025年由美国物理学会出版
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Theory of Electron-Phonon Interactions in Extended Correlated Systems Probed by Resonant Inelastic X-Ray Scattering
An emerging application of resonant inelastic x-ray scattering (RIXS) is the study of lattice excitations and electron-phonon (e-ph) interactions in quantum materials. Despite the growing importance of this area of research, the community lacks a complete understanding of how the RIXS process excites the lattice and how these excitations encode information about the e-ph interactions. Here, we present a detailed study of the RIXS spectra of the Hubbard-Holstein model defined on extended one-dimensional lattices. Using the density matrix renormalization group method, we compute the RIXS response while treating the electron mobility, many-body interactions, and core-hole interactions on an equal footing. The predicted spectra exhibit notable differences from those obtained using the commonly adopted Lang-Firsov models, with important implications for analyzing past and future experiments. Our results provide a deeper understanding of how RIXS probes e-ph interactions and set the stage for a more realistic analysis of future experiments. Published by the American Physical Society 2025
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来源期刊
Physical Review X
Physical Review X PHYSICS, MULTIDISCIPLINARY-
CiteScore
24.60
自引率
1.60%
发文量
197
审稿时长
3 months
期刊介绍: Physical Review X (PRX) stands as an exclusively online, fully open-access journal, emphasizing innovation, quality, and enduring impact in the scientific content it disseminates. Devoted to showcasing a curated selection of papers from pure, applied, and interdisciplinary physics, PRX aims to feature work with the potential to shape current and future research while leaving a lasting and profound impact in their respective fields. Encompassing the entire spectrum of physics subject areas, PRX places a special focus on groundbreaking interdisciplinary research with broad-reaching influence.
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