废铅酸电池储存设施附近空气、水、土壤和农作物中重金属污染的风险评估

IF 2.7 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES
Xiaofeng Gao, Yiran Zhou, Siyan Liu, Zihan Bi, Min Jiang, Manli Zhang, Hongying Cai, Xiaoming Wang
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引用次数: 0

摘要

中国最近被公认为最大的铅酸电池生产国和消费国,这凸显了加大污染控制力度的必要性。现有的环境风险评估研究主要集中在回收过程上,往往忽视了废弃实验室的储存阶段。因此,我们采用暴露评估和健康风险评估(HRA)方法,深入研究了重庆废弃实验室储存设施附近的ERA。虽然空气、地表水和土壤中的重金属含量仍低于标准限值,但蔬菜中的铅、铬和砷含量超过了标准限值。暴露评估结果显示,儿童日均重金属暴露量是成人的1.36 ~ 1.51倍,主要通过蔬菜摄入。此外,HRA表明,在废LAB储存设施附近的环境暴露对成人和儿童都具有不可接受的非致癌和致癌风险。Cr、As和Sb是非致癌风险的主要因素,而Cr、Cd、Ni和As是不可接受的致癌风险的主要因素。与暴露评估结果相一致,蔬菜摄入是导致非致癌和致癌风险的主要暴露途径。综上所述,本研究为废LAB贮存过程中的环境风险防控提供了参考信息。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Risk assessment of heavy metal contamination in air, water, soil, and crops adjacent to a spent lead-acid battery storage facility

China’s recent recognition as the largest producer and consumer of lead-acid batteries (LABs) underscores the need for increased efforts in controlling pollution. Existing environmental risk assessment (ERA) studies are focused on recycling processes, and they often neglect the storage phase of spent LABs. Hence, we delves into ERA near a Chongqing-based storage facility for spent LABs, employing exposure assessment and health risk assessment (HRA). Although the concentrations of heavy metals in the air, surface water, and soil remained below the standard limits, those of Pb, Cr, and As in vegetables surpassed these values. The exposure assessment showed that children's total average daily exposure to heavy metals was 1.36 ~ 1.51 times higher than adults’, primarily through vegetable ingestion. Furthermore, HRA signified that environmental exposure near the spent LAB storage facility posed unacceptable noncarcinogenic and carcinogenic risks for both adults and children. Cr, As, and Sb were the main contributors to noncarcinogenic risk, whereas Cr, Cd, Ni, and As were the main contributors to unacceptable carcinogenic risks. Corroborating the exposure assessment results, vegetable ingestion was the primary exposure route leading to both noncarcinogenic and carcinogenic risks. Overall, this study provides reference information for environmental risk prevention and control during spent LAB storage.

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来源期刊
CiteScore
5.30
自引率
16.10%
发文量
205
审稿时长
4.8 months
期刊介绍: The Journal of Material Cycles and Waste Management has a twofold focus: research in technical, political, and environmental problems of material cycles and waste management; and information that contributes to the development of an interdisciplinary science of material cycles and waste management. Its aim is to develop solutions and prescriptions for material cycles. The journal publishes original articles, reviews, and invited papers from a wide range of disciplines related to material cycles and waste management. The journal is published in cooperation with the Japan Society of Material Cycles and Waste Management (JSMCWM) and the Korea Society of Waste Management (KSWM).
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