Dian Wang, Wei Wang, Yilin Jia, Huihui Cheng, Xinran Ji, Haoru Zhang and Qiannan Wu
{"title":"基于超薄相变超材料的可调谐超宽带等离子体太赫兹吸收体","authors":"Dian Wang, Wei Wang, Yilin Jia, Huihui Cheng, Xinran Ji, Haoru Zhang and Qiannan Wu","doi":"10.1039/D4CP04836A","DOIUrl":null,"url":null,"abstract":"<p >The paper proposes an ultrathin and tunable ultrawideband plasmonic terahertz absorber based on vanadium dioxide (VO<small><sub>2</sub></small>) phase transition metamaterials, with a thickness of only 5.98 micrometers, to address the current issues of insufficient frequency tunability and limited bandwidth coverage in terahertz absorbers. The absorber features a multilayer composite structure consisting of a bottom Au metal layer, a SiO<small><sub>2</sub></small> dielectric layer, a VO<small><sub>2</sub></small> layer, an upper SiO<small><sub>2</sub></small> layer, and a patterned VO<small><sub>2</sub></small> layer on the surface. Simulation results show that the absorber achieves over 90% absorption ranging from 6 to 24 THz (a bandwidth of 18 THz), and nearly perfect absorption at 20.00 THz, covering a wide terahertz frequency range. By adjusting the phase state of VO<small><sub>2</sub></small>, the absorption characteristics are tunable, and the device is insensitive to both TE and TM polarizations. The designed absorber combines the advantages of ultrawideband, high performance, tunability, and miniaturization, making it suitable for enhancing terahertz communication technology, optimizing high-resolution imaging, and applications in high-precision sensing, providing strong support for the development of related technologies.</p>","PeriodicalId":99,"journal":{"name":"Physical Chemistry Chemical Physics","volume":" 14","pages":" 7447-7455"},"PeriodicalIF":2.9000,"publicationDate":"2025-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Tunable ultra-broadband plasmonic terahertz absorber based on ultrathin phase-change metamaterials†\",\"authors\":\"Dian Wang, Wei Wang, Yilin Jia, Huihui Cheng, Xinran Ji, Haoru Zhang and Qiannan Wu\",\"doi\":\"10.1039/D4CP04836A\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The paper proposes an ultrathin and tunable ultrawideband plasmonic terahertz absorber based on vanadium dioxide (VO<small><sub>2</sub></small>) phase transition metamaterials, with a thickness of only 5.98 micrometers, to address the current issues of insufficient frequency tunability and limited bandwidth coverage in terahertz absorbers. The absorber features a multilayer composite structure consisting of a bottom Au metal layer, a SiO<small><sub>2</sub></small> dielectric layer, a VO<small><sub>2</sub></small> layer, an upper SiO<small><sub>2</sub></small> layer, and a patterned VO<small><sub>2</sub></small> layer on the surface. Simulation results show that the absorber achieves over 90% absorption ranging from 6 to 24 THz (a bandwidth of 18 THz), and nearly perfect absorption at 20.00 THz, covering a wide terahertz frequency range. By adjusting the phase state of VO<small><sub>2</sub></small>, the absorption characteristics are tunable, and the device is insensitive to both TE and TM polarizations. The designed absorber combines the advantages of ultrawideband, high performance, tunability, and miniaturization, making it suitable for enhancing terahertz communication technology, optimizing high-resolution imaging, and applications in high-precision sensing, providing strong support for the development of related technologies.</p>\",\"PeriodicalId\":99,\"journal\":{\"name\":\"Physical Chemistry Chemical Physics\",\"volume\":\" 14\",\"pages\":\" 7447-7455\"},\"PeriodicalIF\":2.9000,\"publicationDate\":\"2025-03-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Chemistry Chemical Physics\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2025/cp/d4cp04836a\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Chemistry Chemical Physics","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/cp/d4cp04836a","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Tunable ultra-broadband plasmonic terahertz absorber based on ultrathin phase-change metamaterials†
The paper proposes an ultrathin and tunable ultrawideband plasmonic terahertz absorber based on vanadium dioxide (VO2) phase transition metamaterials, with a thickness of only 5.98 micrometers, to address the current issues of insufficient frequency tunability and limited bandwidth coverage in terahertz absorbers. The absorber features a multilayer composite structure consisting of a bottom Au metal layer, a SiO2 dielectric layer, a VO2 layer, an upper SiO2 layer, and a patterned VO2 layer on the surface. Simulation results show that the absorber achieves over 90% absorption ranging from 6 to 24 THz (a bandwidth of 18 THz), and nearly perfect absorption at 20.00 THz, covering a wide terahertz frequency range. By adjusting the phase state of VO2, the absorption characteristics are tunable, and the device is insensitive to both TE and TM polarizations. The designed absorber combines the advantages of ultrawideband, high performance, tunability, and miniaturization, making it suitable for enhancing terahertz communication technology, optimizing high-resolution imaging, and applications in high-precision sensing, providing strong support for the development of related technologies.
期刊介绍:
Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions.
The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.