光对二氧化钛表面吸附和解吸过程对有效CO2光还原的影响

IF 2.9 3区化学 Q3 CHEMISTRY, PHYSICAL

Physical Chemistry Chemical Physics Pub Date : 2025-03-19 DOI:10.1039/D4CP04279D

Pawel Naliwajko, Nikolaos G. Moustakas, Marcus Klahn, Tim Peppel and Jennifer Strunk

引用次数: 0

摘要

这项工作解决了经常被忽视的光诱导CO2在粉末TiO2表面的吸附行为的影响，作为光催化CO2活化的潜在第一步。这些研究将有助于更详细地了解CO2在TiO2上的光致化学反应，最终揭示CO2光还原机制。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Influence of light on ad- and desorption processes on titanium dioxide surfaces towards efficient CO2 photoreduction†

查看原文本刊更多论文

Influence of light on ad- and desorption processes on titanium dioxide surfaces towards efficient CO2 photoreduction†

This work addresses the often-overlooked effect of light-induced sorption behavior of CO₂ on powder TiO₂ surfaces, as potential first step to photocatalytic CO₂ activation. These investigations will lead to a more detailed understanding of the light-induced chemistry of CO₂ on TiO₂, to eventually unravel the CO₂ photoreduction mechanism.

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来源期刊

Physical Chemistry Chemical Physics 化学-物理：原子、分子和化学物理

CiteScore

5.50

自引率

9.10%

发文量

2675

审稿时长

2.0 months

期刊介绍： Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.