赣州某离子吸附稀土矿区土壤、水和蔬菜中稀土元素污染及健康风险评价

IF 3.2 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL
Liye Zhu, Jinyu Huang, GongHua Hu, Qi Wang, Hui Huang, Sihui Wang, Chunmei Wu, Ziyue Sun, Yi Fang, Ming Hao, Liang Xiong
{"title":"赣州某离子吸附稀土矿区土壤、水和蔬菜中稀土元素污染及健康风险评价","authors":"Liye Zhu, Jinyu Huang, GongHua Hu, Qi Wang, Hui Huang, Sihui Wang, Chunmei Wu, Ziyue Sun, Yi Fang, Ming Hao, Liang Xiong","doi":"10.1007/s10653-025-02426-8","DOIUrl":null,"url":null,"abstract":"<p><p>Rare earth elements (REEs) are increasingly recognized as significant environmental pollutants due to their environmental persistence, bioaccumulation, and chronic toxicity. This study assessed REEs pollution in soil, water, and vegetables in an ion-adsorption rare earth mining area in Ganzhou, and evaluated the associated health risks to the local population. Results indicated that the REEs content in soil ranged from 168.58 to 1915.68 mg/kg, with an average of 546.71 mg/kg, substantially surpassing the background level for Jiangxi Province (243.4 mg/kg) and the national average (197.3 mg/kg). Vegetables displayed an average REEs content of 23.17 mg/kg in fresh weight, far exceeding the hygiene standard of 0.7 mg/kg. Water samples contained REEs at a concentration of 4.09 μg/L. The estimated daily intake (EDI) of REEs from vegetables exceeded the threshold for subclinical damage, posing potential health risks, particularly for children and adolescents. Further analysis of the adjusted average daily intake (ADI) and non-carcinogenic risk suggested that while most vegetable consumption remains within safe threshold, the intake of REEs from high-risk vegetables such as pakchoi should be limited. Overall, carcinogenic risks associated with lifetime cancer risk (LCR) model for REEs exposure through vegetables and water were found to be low in this area.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 4","pages":"116"},"PeriodicalIF":3.2000,"publicationDate":"2025-03-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Pollution and health risk assessment of rare earth elements in soil, water and vegetables from an ion-adsorption rare earth mining area in Ganzhou, China.\",\"authors\":\"Liye Zhu, Jinyu Huang, GongHua Hu, Qi Wang, Hui Huang, Sihui Wang, Chunmei Wu, Ziyue Sun, Yi Fang, Ming Hao, Liang Xiong\",\"doi\":\"10.1007/s10653-025-02426-8\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Rare earth elements (REEs) are increasingly recognized as significant environmental pollutants due to their environmental persistence, bioaccumulation, and chronic toxicity. This study assessed REEs pollution in soil, water, and vegetables in an ion-adsorption rare earth mining area in Ganzhou, and evaluated the associated health risks to the local population. Results indicated that the REEs content in soil ranged from 168.58 to 1915.68 mg/kg, with an average of 546.71 mg/kg, substantially surpassing the background level for Jiangxi Province (243.4 mg/kg) and the national average (197.3 mg/kg). Vegetables displayed an average REEs content of 23.17 mg/kg in fresh weight, far exceeding the hygiene standard of 0.7 mg/kg. Water samples contained REEs at a concentration of 4.09 μg/L. The estimated daily intake (EDI) of REEs from vegetables exceeded the threshold for subclinical damage, posing potential health risks, particularly for children and adolescents. Further analysis of the adjusted average daily intake (ADI) and non-carcinogenic risk suggested that while most vegetable consumption remains within safe threshold, the intake of REEs from high-risk vegetables such as pakchoi should be limited. Overall, carcinogenic risks associated with lifetime cancer risk (LCR) model for REEs exposure through vegetables and water were found to be low in this area.</p>\",\"PeriodicalId\":11759,\"journal\":{\"name\":\"Environmental Geochemistry and Health\",\"volume\":\"47 4\",\"pages\":\"116\"},\"PeriodicalIF\":3.2000,\"publicationDate\":\"2025-03-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Geochemistry and Health\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1007/s10653-025-02426-8\",\"RegionNum\":3,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Geochemistry and Health","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1007/s10653-025-02426-8","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

摘要

稀土元素(ree)由于其环境持久性、生物蓄积性和慢性毒性而日益被认为是重要的环境污染物。本研究对赣州某离子吸附稀土矿区土壤、水体和蔬菜中稀土元素的污染状况进行了评价,并对当地居民的健康风险进行了评价。结果表明:土壤中稀土元素含量为168.58 ~ 1915.68 mg/kg,平均值为546.71 mg/kg,大大超过江西省背景水平(243.4 mg/kg)和全国平均水平(197.3 mg/kg)。蔬菜鲜重平均稀土含量为23.17 mg/kg,远远超过0.7 mg/kg的卫生标准。水样中稀土元素含量为4.09 μg/L。估计每日从蔬菜中摄取的稀土元素超过了亚临床损害的阈值,对健康构成潜在风险,特别是对儿童和青少年。对调整后的每日平均摄入量和非致癌风险的进一步分析表明,虽然大多数蔬菜的摄入量仍在安全范围内,但应限制从小白菜等高风险蔬菜中摄入稀土元素。总体而言,该地区通过蔬菜和水接触稀土元素的终生癌症风险(LCR)模型相关的致癌风险较低。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Pollution and health risk assessment of rare earth elements in soil, water and vegetables from an ion-adsorption rare earth mining area in Ganzhou, China.

Rare earth elements (REEs) are increasingly recognized as significant environmental pollutants due to their environmental persistence, bioaccumulation, and chronic toxicity. This study assessed REEs pollution in soil, water, and vegetables in an ion-adsorption rare earth mining area in Ganzhou, and evaluated the associated health risks to the local population. Results indicated that the REEs content in soil ranged from 168.58 to 1915.68 mg/kg, with an average of 546.71 mg/kg, substantially surpassing the background level for Jiangxi Province (243.4 mg/kg) and the national average (197.3 mg/kg). Vegetables displayed an average REEs content of 23.17 mg/kg in fresh weight, far exceeding the hygiene standard of 0.7 mg/kg. Water samples contained REEs at a concentration of 4.09 μg/L. The estimated daily intake (EDI) of REEs from vegetables exceeded the threshold for subclinical damage, posing potential health risks, particularly for children and adolescents. Further analysis of the adjusted average daily intake (ADI) and non-carcinogenic risk suggested that while most vegetable consumption remains within safe threshold, the intake of REEs from high-risk vegetables such as pakchoi should be limited. Overall, carcinogenic risks associated with lifetime cancer risk (LCR) model for REEs exposure through vegetables and water were found to be low in this area.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信