Huamin Wang, Wenjing Niu, Min Wei, Ying Xiao, Ying-Wu Lin
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引用次数: 0
摘要
碳二亚胺阴离子是由n -氰基- n -芳基-对甲苯磺酰胺(NCTS)在碱的存在下原位生成的,参与了迄今为止报道较少的环。在此,我们首次在无过渡金属的条件下,开发了cf3取代的杂1,3-二烯与NCTS的高效环保[4 + 2]环化反应,以高效合成cf3取代的4h -1,3-恶嗪和2-氨基嘧啶。该方法具有底物易得、操作简单、官能团耐受性好、底物范围广等优点,为合成结构多样的cf3取代支架提供了一条有前景的途径。经过简单转化的产物为TAS2R14激动剂类似物提供了一条便捷的途径。
Direct Access to CF3-Containing 4H-1,3-Oxazines and 2-Aminopyrimidines Via a [4 + 2] Annulation Using In Situ Generated Carbodiimide Anions
The carbodiimide anions which were generated in situ from N-cyano-N-aryl-p-toluenesulfonamides (NCTS) in the presence of the base participated in annulations that remain less reported to date. Herein, we have developed for the first time an efficient and environmentally friendly [4 + 2] annulation reaction of CF3-substituted hetero-1,3-dienes with NCTS for the efficient synthesis of CF3-substituted 4H-1,3-oxazines and 2-aminopyrimidines under transition-metal-free conditions. The methodology demonstrates the advantages of readily available substrates, simple operation, good functional group tolerance, and broad substrate scope, providing a promising route to the synthesis of structurally diverse CF3-substituted scaffolds. The products followed by simple transformations provide a facile route to TAS2R14 agonist analogues.
期刊介绍:
Organic Letters invites original reports of fundamental research in all branches of the theory and practice of organic, physical organic, organometallic,medicinal, and bioorganic chemistry. Organic Letters provides rapid disclosure of the key elements of significant studies that are of interest to a large portion of the organic community. In selecting manuscripts for publication, the Editors place emphasis on the originality, quality and wide interest of the work. Authors should provide enough background information to place the new disclosure in context and to justify the rapid publication format. Back-to-back Letters will be considered. Full details should be reserved for an Article, which should appear in due course.