Spatiotemporal Mapping of Ultrafine Particle Fluxes in an Office HVAC System with a Diffusion Charger Sensor Array.

Commercial HVAC systems intended to mitigate indoor air pollution are operated based on standards that exclude aerosols with smaller diameters, such as ultrafine particles (UFPs, D_p ≤ 100 nm), which dominate a large proportion of indoor and outdoor number-based particle size distributions. UFPs generated from occupant activities or infiltrating from the outdoors can be recirculated and accumulate indoors when they are not successfully filtered by an air handling unit. Monitoring UFPs in real occupied environments is vital to understanding these source and mitigation dynamics, but capturing their rapid transience across multiple locations can be challenging due to high-cost instrumentation. This 9-month field measurement campaign pairs four medium-cost diffusion charger sensors with volumetric airflow rates modulated and monitored in a cloud-based building automation system of an open-plan living laboratory office and dedicated air handling unit to evaluate spatiotemporal particle number and surface area concentrations and migration trends. Particle number flux rates reveal that an estimated daily median of 8 × 10¹³ UFPs enter the air handling unit from the outdoors. Switching from a MERV14 to a HEPA filter reduces the number of UFPs supplied to the room by tens of trillions of UFPs daily, increasing the median filtration efficiency from 40% to 96%. These results demonstrate the efficacy of an optimal air handling unit's performance to improve indoor air quality, while highlighting UFP dynamics that are not accounted for in current filtration standards nor in occupant-centered HVAC control. Scalable sensor development can popularize UFP monitoring and allow for future UFP integration within building control and automation platforms. The framework established for this campaign can be used to evaluate particle fluxes considering different analytes.