N, o -二甲基氨基甲酸酯与甲胺单体和二聚体反应的量子化学研究

IF 0.7 4区 化学 Q4 CHEMISTRY, PHYSICAL
A. Ya. Samuilov, E. P. Kozhanova, Ya. D. Samuilov
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引用次数: 0

摘要

利用量子化学方法B3LYP和M06研究了N,O -二甲基氨基甲酸酯与甲胺单体和二聚体之间的相互作用,作为聚氨酯生产的模型。考虑了一阶段的相互作用机制和两阶段的中间产物的形成,其中包含一个四配位碳原子。后一种途径是不可能的,因为中间产物的形成以平衡常数的低值为特征。甲胺二聚体参与的动力学和热力学反应更可取。与单体相比,甲胺二聚体参与反应的动力学偏好是由于其增强的供体和酸碱性质。与甲胺二聚体反应的热力学偏好是由于相对于与单体反应的转化熵更大。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Quantum Chemical Study of the Reaction between N,O-Dimethylcarbamate and the Monomer and Dimer of Methylamine

Quantum Chemical Study of the Reaction between N,O-Dimethylcarbamate and the Monomer and Dimer of Methylamine

Quantum-chemical methods B3LYP and M06 are used to study the interaction between N,O‑dimethylcarbamate and the monomer and dimer of methylamine as a model for the production of polyureas. A one-stage mechanism of interaction and a two-stage route with the formation of an intermediate containing a tetracoordinated carbon atom are both considered. The latter path is unlikely, since the formation of the intermediate is characterized by low values of the equilibrium constants. Kinetically and thermodynamically reactions with the participation of the methylamine dimer are more preferable. The kinetic preference for reactions with the participation of the methylamine dimer is due to its enhanced donor and acid-base properties, relative to the monomer. The thermodynamic preference for reactions with the methylamine dimer is due to the greater entropy of transformation, relative to the reaction with the monomer.

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来源期刊
CiteScore
1.20
自引率
14.30%
发文量
376
审稿时长
5.1 months
期刊介绍: Russian Journal of Physical Chemistry A. Focus on Chemistry (Zhurnal Fizicheskoi Khimii), founded in 1930, offers a comprehensive review of theoretical and experimental research from the Russian Academy of Sciences, leading research and academic centers from Russia and from all over the world. Articles are devoted to chemical thermodynamics and thermochemistry, biophysical chemistry, photochemistry and magnetochemistry, materials structure, quantum chemistry, physical chemistry of nanomaterials and solutions, surface phenomena and adsorption, and methods and techniques of physicochemical studies.
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