Yang Nan, Chenxing Liu, Hongchao Zhai, Siyu Wu, Zhengyuan Wu, Pengfei Tian, Daoyou Guo, Weihua Tang and Zhilai Fang
{"title":"具有可调谐多波段探测能力的高响应β-Ga2O3/GaN异质结紫外光电探测器†","authors":"Yang Nan, Chenxing Liu, Hongchao Zhai, Siyu Wu, Zhengyuan Wu, Pengfei Tian, Daoyou Guo, Weihua Tang and Zhilai Fang","doi":"10.1039/D4CE01101E","DOIUrl":null,"url":null,"abstract":"<p >The detection of ultraviolet (UV) radiation is of paramount importance, and has expanding applications in industrial, scientific, environmental, and biomedical fields. Using heterojunctions to fabricate UV photodetectors (PDs) is an effective approach for achieving multi-band detection. This study reports on high-responsivity β-Ga<small><sub>2</sub></small>O<small><sub>3</sub></small>/GaN heterojunction UV PDs, featuring tunable multi-band detection capabilities. The as-fabricated PDs demonstrate an exceptional photoresponsivity of 91.2 mA W<small><sup>−1</sup></small> under 250 nm illumination at zero bias. Furthermore, the spectral response of the Ga<small><sub>2</sub></small>O<small><sub>3</sub></small>/GaN heterojunction PDs can be precisely modulated by varying the applied bias voltage, facilitating distinct UVC-dominated and broadband UVA/UVC detection modes with enhanced detectivity. The underlying mechanism responsible for the tunable spectral responses is elucidated. This research not only introduces a straightforward and practical approach for developing multi-band UV PDs regulated by bias voltage, but also provides a comprehensive understanding of the physical mechanisms driving the photoelectric response. These advancements address the increasing demand for UV PDs, and provide guidance for the optimization of device performance and the discussion of intrinsic physical mechanisms in this field.</p>","PeriodicalId":70,"journal":{"name":"CrystEngComm","volume":" 4","pages":" 538-546"},"PeriodicalIF":2.6000,"publicationDate":"2024-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High-responsivity β-Ga2O3/GaN heterojunction UV photodetectors with tunable multi-band detection capability†\",\"authors\":\"Yang Nan, Chenxing Liu, Hongchao Zhai, Siyu Wu, Zhengyuan Wu, Pengfei Tian, Daoyou Guo, Weihua Tang and Zhilai Fang\",\"doi\":\"10.1039/D4CE01101E\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The detection of ultraviolet (UV) radiation is of paramount importance, and has expanding applications in industrial, scientific, environmental, and biomedical fields. Using heterojunctions to fabricate UV photodetectors (PDs) is an effective approach for achieving multi-band detection. This study reports on high-responsivity β-Ga<small><sub>2</sub></small>O<small><sub>3</sub></small>/GaN heterojunction UV PDs, featuring tunable multi-band detection capabilities. The as-fabricated PDs demonstrate an exceptional photoresponsivity of 91.2 mA W<small><sup>−1</sup></small> under 250 nm illumination at zero bias. Furthermore, the spectral response of the Ga<small><sub>2</sub></small>O<small><sub>3</sub></small>/GaN heterojunction PDs can be precisely modulated by varying the applied bias voltage, facilitating distinct UVC-dominated and broadband UVA/UVC detection modes with enhanced detectivity. The underlying mechanism responsible for the tunable spectral responses is elucidated. This research not only introduces a straightforward and practical approach for developing multi-band UV PDs regulated by bias voltage, but also provides a comprehensive understanding of the physical mechanisms driving the photoelectric response. These advancements address the increasing demand for UV PDs, and provide guidance for the optimization of device performance and the discussion of intrinsic physical mechanisms in this field.</p>\",\"PeriodicalId\":70,\"journal\":{\"name\":\"CrystEngComm\",\"volume\":\" 4\",\"pages\":\" 538-546\"},\"PeriodicalIF\":2.6000,\"publicationDate\":\"2024-12-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"CrystEngComm\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2025/ce/d4ce01101e\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"CrystEngComm","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/ce/d4ce01101e","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
紫外线(UV)辐射的检测是至关重要的,在工业、科学、环境和生物医学领域有着越来越广泛的应用。利用异质结制备紫外光电探测器是实现多波段探测的有效途径。本研究报道了高响应β-Ga2O3/GaN异质结UV pd,具有可调谐的多波段检测能力。在250 nm的零偏置照明下,制备的pd具有91.2 mA W−1的特殊光响应性。此外,通过改变施加的偏置电压,可以精确地调制Ga2O3/GaN异质结pd的光谱响应,从而实现不同的UVC主导和宽带UVA/UVC检测模式,提高了探测率。阐明了可调谐光谱响应的基本机制。该研究不仅为开发由偏置电压调节的多波段紫外二极管提供了一种简单实用的方法,而且还提供了对驱动光电响应的物理机制的全面理解。这些进展解决了对UV pd日益增长的需求,并为该领域的器件性能优化和内在物理机制的讨论提供了指导。
High-responsivity β-Ga2O3/GaN heterojunction UV photodetectors with tunable multi-band detection capability†
The detection of ultraviolet (UV) radiation is of paramount importance, and has expanding applications in industrial, scientific, environmental, and biomedical fields. Using heterojunctions to fabricate UV photodetectors (PDs) is an effective approach for achieving multi-band detection. This study reports on high-responsivity β-Ga2O3/GaN heterojunction UV PDs, featuring tunable multi-band detection capabilities. The as-fabricated PDs demonstrate an exceptional photoresponsivity of 91.2 mA W−1 under 250 nm illumination at zero bias. Furthermore, the spectral response of the Ga2O3/GaN heterojunction PDs can be precisely modulated by varying the applied bias voltage, facilitating distinct UVC-dominated and broadband UVA/UVC detection modes with enhanced detectivity. The underlying mechanism responsible for the tunable spectral responses is elucidated. This research not only introduces a straightforward and practical approach for developing multi-band UV PDs regulated by bias voltage, but also provides a comprehensive understanding of the physical mechanisms driving the photoelectric response. These advancements address the increasing demand for UV PDs, and provide guidance for the optimization of device performance and the discussion of intrinsic physical mechanisms in this field.