Thomas Halloran, Peter Czajka, Gicela Saucedo Salas, Corey E. Frank, Chang-Jong Kang, J. A. Rodriguez-Rivera, Jakob Lass, Daniel G. Mazzone, Marc Janoschek, Gabriel Kotliar, Nicholas P. Butch
{"title":"UTe2中f电子相关与磁激发的关系","authors":"Thomas Halloran, Peter Czajka, Gicela Saucedo Salas, Corey E. Frank, Chang-Jong Kang, J. A. Rodriguez-Rivera, Jakob Lass, Daniel G. Mazzone, Marc Janoschek, Gabriel Kotliar, Nicholas P. Butch","doi":"10.1038/s41535-024-00720-9","DOIUrl":null,"url":null,"abstract":"<p>The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe<sub>2</sub> is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry <i>Y</i> and <i>T</i> points and disperse along the crystallographic <span>\\(\\hat{b}\\)</span>-axis. In applied magnetic fields to at least <i>μ</i><sub>0</sub><i>H</i> = 11 T along the <span>\\(\\hat{c}-{\\rm{axis}}\\)</span>, the magnetism is found to be field-independent in the (<i>h</i><i>k</i>0) plane. The scattering intensity is consistent with that expected from U<sup>3+</sup>/U<sup>4+</sup> <i>f</i>-electron spins with preferential orientation along the crystallographic <span>\\(\\hat{a}\\)</span>-axis, and a fluctuating magnetic moment of <i>μ</i><sub><i>e</i><i>f</i><i>f</i></sub>=1.7(5) <i>μ</i><sub><i>B</i></sub>. We propose interband spin excitons arising from <i>f</i>-electron hybridization as a possible origin of the magnetic excitations in UTe<sub>2</sub>.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":"66 1","pages":""},"PeriodicalIF":5.4000,"publicationDate":"2025-01-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Connection between f-electron correlations and magnetic excitations in UTe2\",\"authors\":\"Thomas Halloran, Peter Czajka, Gicela Saucedo Salas, Corey E. Frank, Chang-Jong Kang, J. A. Rodriguez-Rivera, Jakob Lass, Daniel G. Mazzone, Marc Janoschek, Gabriel Kotliar, Nicholas P. Butch\",\"doi\":\"10.1038/s41535-024-00720-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe<sub>2</sub> is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry <i>Y</i> and <i>T</i> points and disperse along the crystallographic <span>\\\\(\\\\hat{b}\\\\)</span>-axis. In applied magnetic fields to at least <i>μ</i><sub>0</sub><i>H</i> = 11 T along the <span>\\\\(\\\\hat{c}-{\\\\rm{axis}}\\\\)</span>, the magnetism is found to be field-independent in the (<i>h</i><i>k</i>0) plane. The scattering intensity is consistent with that expected from U<sup>3+</sup>/U<sup>4+</sup> <i>f</i>-electron spins with preferential orientation along the crystallographic <span>\\\\(\\\\hat{a}\\\\)</span>-axis, and a fluctuating magnetic moment of <i>μ</i><sub><i>e</i><i>f</i><i>f</i></sub>=1.7(5) <i>μ</i><sub><i>B</i></sub>. We propose interband spin excitons arising from <i>f</i>-electron hybridization as a possible origin of the magnetic excitations in UTe<sub>2</sub>.</p>\",\"PeriodicalId\":19283,\"journal\":{\"name\":\"npj Quantum Materials\",\"volume\":\"66 1\",\"pages\":\"\"},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2025-01-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"npj Quantum Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41535-024-00720-9\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"npj Quantum Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41535-024-00720-9","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Connection between f-electron correlations and magnetic excitations in UTe2
The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe2 is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry Y and T points and disperse along the crystallographic \(\hat{b}\)-axis. In applied magnetic fields to at least μ0H = 11 T along the \(\hat{c}-{\rm{axis}}\), the magnetism is found to be field-independent in the (hk0) plane. The scattering intensity is consistent with that expected from U3+/U4+f-electron spins with preferential orientation along the crystallographic \(\hat{a}\)-axis, and a fluctuating magnetic moment of μeff=1.7(5) μB. We propose interband spin excitons arising from f-electron hybridization as a possible origin of the magnetic excitations in UTe2.
期刊介绍:
npj Quantum Materials is an open access journal that publishes works that significantly advance the understanding of quantum materials, including their fundamental properties, fabrication and applications.