{"title":"作为纳米结构近场随机传送带的负载脂双分子层","authors":"Yazgan Tuna, Vahid Sandoghdar","doi":"10.1021/acs.jpcc.4c06908","DOIUrl":null,"url":null,"abstract":"Placement of nanoscopic entities in the optical near field of a structure such as a plasmonic nanoantenna or the aperture of a scanning near-field optical microscopy (SNOM) remains a nontrivial task, which often requires sophisticated nanofabrication techniques. Here, we show that the fluidity and diffusion of lipid molecules in bilayer geometries can be exploited for facile delivery of nano-objects such as organic dye molecules, semiconductor quantum dots, and gold nanoparticles to the near field of well-defined surface structures. We demonstrate this in three different scenarios with substantial plasmonic enhancement of fluorescence.","PeriodicalId":61,"journal":{"name":"The Journal of Physical Chemistry C","volume":"13 1","pages":""},"PeriodicalIF":3.3000,"publicationDate":"2024-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Supported Lipid Bilayers as Stochastic Conveyor Belt for Delivery to the Near Field of Nanoscopic Structures\",\"authors\":\"Yazgan Tuna, Vahid Sandoghdar\",\"doi\":\"10.1021/acs.jpcc.4c06908\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Placement of nanoscopic entities in the optical near field of a structure such as a plasmonic nanoantenna or the aperture of a scanning near-field optical microscopy (SNOM) remains a nontrivial task, which often requires sophisticated nanofabrication techniques. Here, we show that the fluidity and diffusion of lipid molecules in bilayer geometries can be exploited for facile delivery of nano-objects such as organic dye molecules, semiconductor quantum dots, and gold nanoparticles to the near field of well-defined surface structures. We demonstrate this in three different scenarios with substantial plasmonic enhancement of fluorescence.\",\"PeriodicalId\":61,\"journal\":{\"name\":\"The Journal of Physical Chemistry C\",\"volume\":\"13 1\",\"pages\":\"\"},\"PeriodicalIF\":3.3000,\"publicationDate\":\"2024-12-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"The Journal of Physical Chemistry C\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.jpcc.4c06908\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"The Journal of Physical Chemistry C","FirstCategoryId":"1","ListUrlMain":"https://doi.org/10.1021/acs.jpcc.4c06908","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Supported Lipid Bilayers as Stochastic Conveyor Belt for Delivery to the Near Field of Nanoscopic Structures
Placement of nanoscopic entities in the optical near field of a structure such as a plasmonic nanoantenna or the aperture of a scanning near-field optical microscopy (SNOM) remains a nontrivial task, which often requires sophisticated nanofabrication techniques. Here, we show that the fluidity and diffusion of lipid molecules in bilayer geometries can be exploited for facile delivery of nano-objects such as organic dye molecules, semiconductor quantum dots, and gold nanoparticles to the near field of well-defined surface structures. We demonstrate this in three different scenarios with substantial plasmonic enhancement of fluorescence.
期刊介绍:
The Journal of Physical Chemistry A/B/C is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, and chemical physicists.