Julian Max Salchegger, Rajdeep Adhikari, Bogdan Faina, Jelena Pešić, Alberta Bonanni
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{"title":"狄拉克半金属铂硒2中的负纵向磁阻：近藤效应和表面自旋动力学","authors":"Julian Max Salchegger, Rajdeep Adhikari, Bogdan Faina, Jelena Pešić, Alberta Bonanni","doi":"10.1103/physrevb.110.205403","DOIUrl":null,"url":null,"abstract":"The emergence of negative longitudinal magnetoresistance in the topologically nontrivial transition-metal dichalcogenide <mjx-container ctxtmenu_counter=\"58\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(2 0 1)\"><mjx-mrow><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-role=\"unknown\" data-semantic-speech=\"PtSe Subscript 2\" data-semantic-type=\"subscript\"><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"text\" style='font-family: MJX-STX-ZERO, \"Helvetica Neue\", Helvetica, Roboto, Arial, sans-serif;'><mjx-utext style=\"font-size: 90.6%; padding: 0.828em 0px 0.221em; width: 27px;\" variant=\"-explicitFont\">PtSe</mjx-utext></mjx-mtext><mjx-script style=\"vertical-align: -0.235em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>2</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mspace style=\"width: 0.16em;\"></mjx-mspace></mjx-mrow></mjx-math></mjx-container>is studied. Low-<mjx-container ctxtmenu_counter=\"59\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-role=\"latinletter\" data-semantic-speech=\"upper T\" data-semantic-type=\"identifier\"><mjx-c>𝑇</mjx-c></mjx-mi></mjx-math></mjx-container>, high-<mjx-container ctxtmenu_counter=\"60\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(5 (2 0 1) 4 3)\"><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"2,3\" data-semantic-content=\"4\" data-semantic- data-semantic-owns=\"2 4 3\" data-semantic-role=\"implicit\" data-semantic-speech=\"mu 0 upper H\" data-semantic-type=\"infixop\"><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-parent=\"5\" data-semantic-role=\"greekletter\" data-semantic-type=\"subscript\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"greekletter\" data-semantic-type=\"identifier\"><mjx-c>𝜇</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>0</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"5\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\"><mjx-c>𝐻</mjx-c></mjx-mi></mjx-mrow></mjx-math></mjx-container> transport is performed for arbitrary field directions, and an analytical framework is established. The source of the negative longitudinal magnetoresistance is identified as the Kondo effect stemming from Pt vacancies contributing an uncompensated spin exclusively at the sample surface. The concentration of vacancies and the sample thickness are identified as tuning parameters. The findings are substantiated by density functional theory, which corroborates the proposed Pt-vacancy model.","PeriodicalId":20082,"journal":{"name":"Physical Review B","volume":null,"pages":null},"PeriodicalIF":3.7000,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Negative longitudinal magnetoresistance in the Dirac semimetalPtSe2: Kondo effect and surface spin dynamics\",\"authors\":\"Julian Max Salchegger, Rajdeep Adhikari, Bogdan Faina, Jelena Pešić, Alberta Bonanni\",\"doi\":\"10.1103/physrevb.110.205403\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The emergence of negative longitudinal magnetoresistance in the topologically nontrivial transition-metal dichalcogenide <mjx-container ctxtmenu_counter=\\\"58\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" overflow=\\\"linebreak\\\" role=\\\"tree\\\" sre-explorer- style=\\\"font-size: 100.7%;\\\" tabindex=\\\"0\\\"><mjx-math data-semantic-structure=\\\"(2 0 1)\\\"><mjx-mrow><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-owns=\\\"0 1\\\" data-semantic-role=\\\"unknown\\\" data-semantic-speech=\\\"PtSe Subscript 2\\\" data-semantic-type=\\\"subscript\\\"><mjx-mtext data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"unknown\\\" data-semantic-type=\\\"text\\\" style='font-family: MJX-STX-ZERO, \\\"Helvetica Neue\\\", Helvetica, Roboto, Arial, sans-serif;'><mjx-utext style=\\\"font-size: 90.6%; padding: 0.828em 0px 0.221em; width: 27px;\\\" variant=\\\"-explicitFont\\\">PtSe</mjx-utext></mjx-mtext><mjx-script style=\\\"vertical-align: -0.235em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c>2</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mspace style=\\\"width: 0.16em;\\\"></mjx-mspace></mjx-mrow></mjx-math></mjx-container>is studied. Low-<mjx-container ctxtmenu_counter=\\\"59\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" overflow=\\\"linebreak\\\" role=\\\"tree\\\" sre-explorer- style=\\\"font-size: 100.7%;\\\" tabindex=\\\"0\\\"><mjx-math data-semantic-structure=\\\"0\\\"><mjx-mi data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"italic\\\" data-semantic- data-semantic-role=\\\"latinletter\\\" data-semantic-speech=\\\"upper T\\\" data-semantic-type=\\\"identifier\\\"><mjx-c>𝑇</mjx-c></mjx-mi></mjx-math></mjx-container>, high-<mjx-container ctxtmenu_counter=\\\"60\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" overflow=\\\"linebreak\\\" role=\\\"tree\\\" sre-explorer- style=\\\"font-size: 100.7%;\\\" tabindex=\\\"0\\\"><mjx-math data-semantic-structure=\\\"(5 (2 0 1) 4 3)\\\"><mjx-mrow data-semantic-annotation=\\\"clearspeak:unit\\\" data-semantic-children=\\\"2,3\\\" data-semantic-content=\\\"4\\\" data-semantic- data-semantic-owns=\\\"2 4 3\\\" data-semantic-role=\\\"implicit\\\" data-semantic-speech=\\\"mu 0 upper H\\\" data-semantic-type=\\\"infixop\\\"><mjx-msub data-semantic-children=\\\"0,1\\\" data-semantic- data-semantic-owns=\\\"0 1\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"greekletter\\\" data-semantic-type=\\\"subscript\\\"><mjx-mi data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"italic\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"greekletter\\\" data-semantic-type=\\\"identifier\\\"><mjx-c>𝜇</mjx-c></mjx-mi><mjx-script style=\\\"vertical-align: -0.15em;\\\"><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"2\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\" size=\\\"s\\\"><mjx-c>0</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\\\"true\\\" data-semantic- data-semantic-operator=\\\"infixop,\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"multiplication\\\" data-semantic-type=\\\"operator\\\"><mjx-c></mjx-c></mjx-mo><mjx-mi data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"italic\\\" data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"latinletter\\\" data-semantic-type=\\\"identifier\\\"><mjx-c>𝐻</mjx-c></mjx-mi></mjx-mrow></mjx-math></mjx-container> transport is performed for arbitrary field directions, and an analytical framework is established. The source of the negative longitudinal magnetoresistance is identified as the Kondo effect stemming from Pt vacancies contributing an uncompensated spin exclusively at the sample surface. The concentration of vacancies and the sample thickness are identified as tuning parameters. The findings are substantiated by density functional theory, which corroborates the proposed Pt-vacancy model.\",\"PeriodicalId\":20082,\"journal\":{\"name\":\"Physical Review B\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.7000,\"publicationDate\":\"2024-11-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Review B\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/physrevb.110.205403\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"Physics and Astronomy\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review B","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physrevb.110.205403","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Physics and Astronomy","Score":null,"Total":0}
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