二维克拉默斯半金属铟碲中独特的 LA Phonon 模式诱发的强量子化电子-Phonon 耦合

IF 3.3 3区 化学 Q2 CHEMISTRY, PHYSICAL
Juntao Kong, Zhengxin Yan, Wei Song, Weili Li, Zhaoqi Wang
{"title":"二维克拉默斯半金属铟碲中独特的 LA Phonon 模式诱发的强量子化电子-Phonon 耦合","authors":"Juntao Kong, Zhengxin Yan, Wei Song, Weili Li, Zhaoqi Wang","doi":"10.1021/acs.jpcc.4c04708","DOIUrl":null,"url":null,"abstract":"Two-dimensional topological materials with flat bands and van Hove singularities in their electronic band structures are common, and these features may lead to superconductivity due to the strong condensation of electronic states. However, the electron–phonon coupling between flat bands and single longitudinal acoustic (LA) phonons has not been extensively studied or reported. In this work, using group theory, symmetry analysis, and first-principles calculations, we investigate flat electron bands, phonon spectra, and electron–phonon coupling in a two-dimensional metallic InTe monolayer. Our study reveals that the electron–phonon interaction in the intrinsic Kramers nodal line, with a van Hove singularity near the Fermi level, primarily involves a single LA phonon mode that couples strongly with the flat band electrons. This interaction leads to a slightly anisotropic superconducting gap function. Our findings provide new insights into the role of phonon-mediated electron interactions in superconductors with flat bands.","PeriodicalId":61,"journal":{"name":"The Journal of Physical Chemistry C","volume":null,"pages":null},"PeriodicalIF":3.3000,"publicationDate":"2024-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Strong Quantized Electron–Phonon Coupling Induced by the Unique LA Phonon Mode in 2D Kramers Semimetal InTe\",\"authors\":\"Juntao Kong, Zhengxin Yan, Wei Song, Weili Li, Zhaoqi Wang\",\"doi\":\"10.1021/acs.jpcc.4c04708\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Two-dimensional topological materials with flat bands and van Hove singularities in their electronic band structures are common, and these features may lead to superconductivity due to the strong condensation of electronic states. However, the electron–phonon coupling between flat bands and single longitudinal acoustic (LA) phonons has not been extensively studied or reported. In this work, using group theory, symmetry analysis, and first-principles calculations, we investigate flat electron bands, phonon spectra, and electron–phonon coupling in a two-dimensional metallic InTe monolayer. Our study reveals that the electron–phonon interaction in the intrinsic Kramers nodal line, with a van Hove singularity near the Fermi level, primarily involves a single LA phonon mode that couples strongly with the flat band electrons. This interaction leads to a slightly anisotropic superconducting gap function. Our findings provide new insights into the role of phonon-mediated electron interactions in superconductors with flat bands.\",\"PeriodicalId\":61,\"journal\":{\"name\":\"The Journal of Physical Chemistry C\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.3000,\"publicationDate\":\"2024-10-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"The Journal of Physical Chemistry C\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.jpcc.4c04708\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"The Journal of Physical Chemistry C","FirstCategoryId":"1","ListUrlMain":"https://doi.org/10.1021/acs.jpcc.4c04708","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

摘要

二维拓扑材料的电子带结构中具有平坦带和范霍夫奇点的现象很常见,这些特征可能会由于电子态的强烈凝聚而导致超导。然而,平带与单一纵向声子(LA)之间的电子-声子耦合尚未得到广泛研究和报道。在这项研究中,我们利用群论、对称性分析和第一性原理计算,研究了二维金属铟碲单层中的平坦电子带、声子谱和电子-声子耦合。我们的研究发现,在费米水平附近具有范霍夫奇点的本征克拉默结线中,电子与声子的相互作用主要涉及与平坦带电子强烈耦合的单个 LA 声子模式。这种相互作用导致了轻微的各向异性超导间隙函数。我们的发现为了解声子介导的电子相互作用在平带超导体中的作用提供了新的视角。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Strong Quantized Electron–Phonon Coupling Induced by the Unique LA Phonon Mode in 2D Kramers Semimetal InTe

Strong Quantized Electron–Phonon Coupling Induced by the Unique LA Phonon Mode in 2D Kramers Semimetal InTe
Two-dimensional topological materials with flat bands and van Hove singularities in their electronic band structures are common, and these features may lead to superconductivity due to the strong condensation of electronic states. However, the electron–phonon coupling between flat bands and single longitudinal acoustic (LA) phonons has not been extensively studied or reported. In this work, using group theory, symmetry analysis, and first-principles calculations, we investigate flat electron bands, phonon spectra, and electron–phonon coupling in a two-dimensional metallic InTe monolayer. Our study reveals that the electron–phonon interaction in the intrinsic Kramers nodal line, with a van Hove singularity near the Fermi level, primarily involves a single LA phonon mode that couples strongly with the flat band electrons. This interaction leads to a slightly anisotropic superconducting gap function. Our findings provide new insights into the role of phonon-mediated electron interactions in superconductors with flat bands.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
The Journal of Physical Chemistry C
The Journal of Physical Chemistry C 化学-材料科学:综合
CiteScore
6.50
自引率
8.10%
发文量
2047
审稿时长
1.8 months
期刊介绍: The Journal of Physical Chemistry A/B/C is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, and chemical physicists.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信