流动反应器中化学过程的稳定性分析

IF 0.7 4区 工程技术 Q4 ENGINEERING, CHEMICAL
A. A. Belyaev, A. V. Arutyunov, V. S. Arutyunov
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引用次数: 0

摘要

分析了在具有空间不均匀性的流动反应器中的化学过程中出现振荡条件的可能性。反应器的数学动态模型考虑了分子和对流的传热和传质过程。该问题在单步化学反应条件下以一维近似方式求解。在扩散系数和温度传导系数相等的条件下,得到了稳态条件稳定性标准的分析表达式。在确定系统稳定性的临界条件时,显示了行动顺序。进行了一系列数值实验,以验证在与反应器实际条件相对应的不同参数值下是否会出现振荡状态。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The Stability Analysis of a Chemical Process in a Flow Reactor

The possibility of emergence of oscillatory conditions during a chemical process in a flow reactor with spatial inhomogeneity is analyzed. The mathematical dynamic model of the reactor takes into account molecular and convective heat- and mass-transfer processes. The problem is solved in a one-dimensional approximation under single-step chemical-reaction conditions. An analytical expression for the stability criterion of the steady-state conditions is obtained provided that the diffusion and temperature conductivity coefficients are equal. The sequence of actions upon determining the critical conditions for the stability of the system is shown. A series of numerical experiments is performed to verify the emergence of oscillatory regimes at different parameter values corresponding to real conditions in the reactor.

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来源期刊
CiteScore
1.20
自引率
25.00%
发文量
70
审稿时长
24 months
期刊介绍: Theoretical Foundations of Chemical Engineering is a comprehensive journal covering all aspects of theoretical and applied research in chemical engineering, including transport phenomena; surface phenomena; processes of mixture separation; theory and methods of chemical reactor design; combined processes and multifunctional reactors; hydromechanic, thermal, diffusion, and chemical processes and apparatus, membrane processes and reactors; biotechnology; dispersed systems; nanotechnologies; process intensification; information modeling and analysis; energy- and resource-saving processes; environmentally clean processes and technologies.
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