反铁磁拓扑金属 NdGaSi 中的巨型各向异性反常霍尔效应

Anyesh Saraswati, Sudipta Chatterjee, Nitesh Kumar
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引用次数: 0

摘要

磁性材料中的磁性和强电子相关性之间的相互作用产生了各种有趣的拓扑特征。在此,我们对掺镓硅单晶的磁性、热力学和电传输特性进行了系统研究。磁性测量揭示了低于 T_N(11 K)的磁有序性,自旋在平面内与铁磁性(FM)排列,在平面外与铁磁性(FM)排列。纵向电阻率数据和热容量因 TN 处的磁有序而显示出明显的异常。磁阻研究表明,沿任一方向测量时都会出现明显不同的行为,这是由于磁性结构的复杂性造成的,其中一个方向的磁矩完全饱和,而另一个方向的磁矩则随之发生自旋翻转。值得注意的是,我们还注意到一种不寻常的各向异性反常霍尔响应。我们观察到,在 2 K 时,B//[001] 和 B //[100] 的巨反常霍尔电导率(AHC)分别为 1730 欧姆-1 厘米-1 和 490 欧姆-1 厘米-1。我们对 AHC 的比例分析表明,所研究化合物中的反常霍尔效应是由贝里相驱动的内在机制主导的。钕镓硅中的这些惊人发现为稀土基金属间化合物中的反铁磁自旋电子学开辟了新的可能性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Giant anisotropic anomalous Hall effect in antiferromagnetic topological metal NdGaSi
The interplay between magnetism and strong electron correlation in magnetic materials discerns a variety of intriguing topological features. Here, we report a systematic investigation of the magnetic, thermodynamic, and electrical transport properties in NdGaSi single crystals. The magnetic measurements reveal a magnetic ordering below T_N (11 K), with spins aligning antiferromagnetically in-plane, and it orders ferromagnetically (FM) out-of-plane. The longitudinal resistivity data and heat capacity exhibit a significant anomaly as a consequence of the magnetic ordering at TN. The magnetoresistance study shows significantly different behavior when measured along either direction, resulting from the complex nature of the magnetic structure, stemming from complete saturation of moments in one direction and subsequent spin flop transitions in the other. Remarkably, we have also noticed an unusual anisotropic anomalous Hall response. We have observed a giant anomalous Hall conductivity (AHC) of 1730 ohm-1 cm-1 and 490 ohm-1 cm-1 at 2 K, with B // [001] and B // [100], respectively. Our scaling analysis of AHC reveals that the anomalous Hall effect in the studied compound is dominated by the Berry phase-driven intrinsic mechanism. These astonishing findings in NdGaSi open up new possibilities for antiferromagnetic spintronics in rare-earth-based intermetallic compounds.
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