{"title":"第 IX 章.非等温链式过程的动力学规律","authors":"V. V. Azatyan","doi":"10.1134/S0023158424601335","DOIUrl":null,"url":null,"abstract":"<p>The rarely considered fundamental difference between the temperature dependences of the reaction rate and the rate constant is emphasized. The small change in the rate of reactions with high activation energies, contrary to existing ideas, is illustrated. It was shown that the main reason for the deviation between the calculated and experimental rates is the neglect of the temperature dependence of the reagent concentrations during the reaction. It has been shown that the main reason for the deviation between the calculated and experimental rate values is the neglect of the temperature dependence of the reactant concentrations in the course the reaction. The concept of the temperature rate constant is introduced: the change in the rate with a unit change in temperature, i.e., the temperature derivative of the rate constant. It is shown that this characteristic determines the competition between the stages of a complex process under nonisothermal conditions. The law of temperature dependence of the chain process was discovered, and its agreement with experiment was verified. The difference between the self-acceleration of a reaction from an increase in temperature and from the multiplication of active particles is explained. An experimental illustration is provided. The difference between the temperature dependences of the reaction rates in a gas heated from outside before and after the onset of ignition is explained. Based on experimental data, the determining role of the hydrogen atom concentrations in the combustion rate at hundredths of atmospheric pressure and at atmospheric pressure is quantitatively demonstrated. This demonstrates the determining role in combustion of the conversion of a significant part of the enthalpy of the initial reagents into the free-valence energy.</p>","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Chapter IX. Laws of Kinetics of Nonisothermal Chain Processes\",\"authors\":\"V. V. Azatyan\",\"doi\":\"10.1134/S0023158424601335\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The rarely considered fundamental difference between the temperature dependences of the reaction rate and the rate constant is emphasized. The small change in the rate of reactions with high activation energies, contrary to existing ideas, is illustrated. It was shown that the main reason for the deviation between the calculated and experimental rates is the neglect of the temperature dependence of the reagent concentrations during the reaction. It has been shown that the main reason for the deviation between the calculated and experimental rate values is the neglect of the temperature dependence of the reactant concentrations in the course the reaction. The concept of the temperature rate constant is introduced: the change in the rate with a unit change in temperature, i.e., the temperature derivative of the rate constant. It is shown that this characteristic determines the competition between the stages of a complex process under nonisothermal conditions. The law of temperature dependence of the chain process was discovered, and its agreement with experiment was verified. The difference between the self-acceleration of a reaction from an increase in temperature and from the multiplication of active particles is explained. An experimental illustration is provided. The difference between the temperature dependences of the reaction rates in a gas heated from outside before and after the onset of ignition is explained. Based on experimental data, the determining role of the hydrogen atom concentrations in the combustion rate at hundredths of atmospheric pressure and at atmospheric pressure is quantitatively demonstrated. This demonstrates the determining role in combustion of the conversion of a significant part of the enthalpy of the initial reagents into the free-valence energy.</p>\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2024-08-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://link.springer.com/article/10.1134/S0023158424601335\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1134/S0023158424601335","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Chapter IX. Laws of Kinetics of Nonisothermal Chain Processes
The rarely considered fundamental difference between the temperature dependences of the reaction rate and the rate constant is emphasized. The small change in the rate of reactions with high activation energies, contrary to existing ideas, is illustrated. It was shown that the main reason for the deviation between the calculated and experimental rates is the neglect of the temperature dependence of the reagent concentrations during the reaction. It has been shown that the main reason for the deviation between the calculated and experimental rate values is the neglect of the temperature dependence of the reactant concentrations in the course the reaction. The concept of the temperature rate constant is introduced: the change in the rate with a unit change in temperature, i.e., the temperature derivative of the rate constant. It is shown that this characteristic determines the competition between the stages of a complex process under nonisothermal conditions. The law of temperature dependence of the chain process was discovered, and its agreement with experiment was verified. The difference between the self-acceleration of a reaction from an increase in temperature and from the multiplication of active particles is explained. An experimental illustration is provided. The difference between the temperature dependences of the reaction rates in a gas heated from outside before and after the onset of ignition is explained. Based on experimental data, the determining role of the hydrogen atom concentrations in the combustion rate at hundredths of atmospheric pressure and at atmospheric pressure is quantitatively demonstrated. This demonstrates the determining role in combustion of the conversion of a significant part of the enthalpy of the initial reagents into the free-valence energy.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.