卡戈梅反铁磁体九分之一高原附近费米子行为的热力学证据

Guoxin Zheng, Dechen Zhang, Yuan Zhu, Kuan-Wen Chen, Aaron Chan, Kaila Jenkins, Byungmin Kang, Zhenyuan Zeng, Aini Xu, D. Ratkovski, Joanna Blawat, Ali Bangura, John Singleton, Patrick A. Lee, Shiliang Li, Lu Li
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引用次数: 0

摘要

自旋-1/2卡戈梅海森堡反铁磁体被认为蕴藏着奇异的量子纠缠态。最近,在卡戈梅反铁磁体YCu$_3$(OH)$_6$Br$_2$[Br$_x$(OH)$_{1-x}$](YCOB)中发现的1/9磁化高原和磁振荡现象使这种材料成为实验实现量子自旋液体态的理想候选材料。在这里,我们展示了 YCOB 在高磁场(高达 41.5 特斯拉)中低至 0.46 开尔文的比热 $C_p$的测量结果,并且证实了 1/9 高原特征。此外,在 1/9 高原区附近,$C_p/T$ 的温度依赖性可以通过一个以 $T$ 为单位的线性项和一个常数项来拟合,前者表明了狄拉克谱的存在,后者表明了由其他费米面贡献的有限状态密度(DOS)。令人惊讶的是,常数项在磁场方向上高度各向异性。此外,我们还在 1/9 高原上方 30$~T 附近观察到双峰特征,这是费米子激发比热的另一个标志。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Thermodynamic evidence of fermionic behavior in the vicinity of one-ninth plateau in a kagome antiferromagnet
The spin-1/2 kagome Heisenberg antiferromagnets are believed to host exotic quantum entangled states. Recently, the report of 1/9 magnetization plateau and magnetic oscillations in a kagome antiferromagnet YCu$_3$(OH)$_6$Br$_2$[Br$_x$(OH)$_{1-x}$] (YCOB) have made this material a promising candidate for experimentally realizing quantum spin liquid states. Here we present measurements of the specific heat $C_p$ in YCOB in high magnetic fields (up to 41.5 Tesla) down to 0.46 Kelvin, and the 1/9 plateau feature has been confirmed. Moreover, the temperature dependence of $C_p/T$ in the vicinity of 1/9 plateau region can be fitted by a linear in $T$ term which indicates the presence of a Dirac spectrum, together with a constant term, which indicates a finite density of states (DOS) contributed by other Fermi surfaces. Surprisingly the constant term is highly anisotropic in the direction of the magnetic field. Additionally, we observe a double-peak feature near $30$~T above the 1/9 plateau which is another hallmark of fermionic excitations in the specific heat.
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