LinCong Shu, ShuLin Sha, ZhaoYing Xi, Lei Li, SuHao Yao, JiaHan Zhang, XueQiang Ji, ShaoHui Zhang, Ang Bian, MingMing Jiang, YuFeng Guo, WeiHua Tang, Zeng Liu
{"title":"通过高效热电子激发和界面注入实现表面等离子体装饰的 InGaO 深紫外光探测器阵列,用于图像传感和水质监测","authors":"LinCong Shu, ShuLin Sha, ZhaoYing Xi, Lei Li, SuHao Yao, JiaHan Zhang, XueQiang Ji, ShaoHui Zhang, Ang Bian, MingMing Jiang, YuFeng Guo, WeiHua Tang, Zeng Liu","doi":"10.1007/s11431-024-2660-1","DOIUrl":null,"url":null,"abstract":"<p>In addition to the plasmon-mediated resonant coupling mechanism, the excitation of hot electron induced by plasmon presents a promising path for developing high-performance optoelectronic devices tailored for various applications. This study introduces a sophisticated design for a solar-blind ultraviolet (UV) detector array using linear In-doped Ga<sub>2</sub>O<sub>3</sub> (InGaO) modulated by platinum (Pt) nanoparticles (PtNPs). The construction of this array involves depositing a thin film of Ga<sub>2</sub>O<sub>3</sub> through the plasmonenhanced chemical vapor deposition (PECVD) technique. Subsequently, PtNPs were synthesized via radio-frequency magnetron sputtering and annealing process. The performance of these highly uniform arrays is significantly enhanced owing to the generation of high-energy hot electrons. This process is facilitated by non-radiative decay processes induced by PtNPs. Notably, the array achieves maximum responsivity (<i>R</i>) of 353 mA/W, external quantum efficiency (<i>EQE</i>) of 173%, detectivity (<i>D</i>*) of approximately 10<sup>13</sup> Jones, and photoconductive gain of 1.58. In addition, the standard deviation for photocurrent stays below 17% for more than 80% of the array units within the array. Subsequently, the application of this array extends to photon detection in the deep-UV (DUV) range. This includes critical areas such as imaging sensing and water quality monitoring. By leveraging surface plasmon coupling, the array achieves high-performance DUV photon detection. This approach enables a broad spectrum of practical applications, underscoring the significant potential of this technology for the advancement of DUV detectors.</p>","PeriodicalId":21612,"journal":{"name":"Science China Technological Sciences","volume":"245 1","pages":""},"PeriodicalIF":4.4000,"publicationDate":"2024-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Surface plasmon decorated InGaO deep-UV photodetector array for image sensing and water quality monitoring via highly effective hot electron excitation and interfacial injection\",\"authors\":\"LinCong Shu, ShuLin Sha, ZhaoYing Xi, Lei Li, SuHao Yao, JiaHan Zhang, XueQiang Ji, ShaoHui Zhang, Ang Bian, MingMing Jiang, YuFeng Guo, WeiHua Tang, Zeng Liu\",\"doi\":\"10.1007/s11431-024-2660-1\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>In addition to the plasmon-mediated resonant coupling mechanism, the excitation of hot electron induced by plasmon presents a promising path for developing high-performance optoelectronic devices tailored for various applications. This study introduces a sophisticated design for a solar-blind ultraviolet (UV) detector array using linear In-doped Ga<sub>2</sub>O<sub>3</sub> (InGaO) modulated by platinum (Pt) nanoparticles (PtNPs). The construction of this array involves depositing a thin film of Ga<sub>2</sub>O<sub>3</sub> through the plasmonenhanced chemical vapor deposition (PECVD) technique. Subsequently, PtNPs were synthesized via radio-frequency magnetron sputtering and annealing process. The performance of these highly uniform arrays is significantly enhanced owing to the generation of high-energy hot electrons. This process is facilitated by non-radiative decay processes induced by PtNPs. Notably, the array achieves maximum responsivity (<i>R</i>) of 353 mA/W, external quantum efficiency (<i>EQE</i>) of 173%, detectivity (<i>D</i>*) of approximately 10<sup>13</sup> Jones, and photoconductive gain of 1.58. In addition, the standard deviation for photocurrent stays below 17% for more than 80% of the array units within the array. Subsequently, the application of this array extends to photon detection in the deep-UV (DUV) range. This includes critical areas such as imaging sensing and water quality monitoring. By leveraging surface plasmon coupling, the array achieves high-performance DUV photon detection. This approach enables a broad spectrum of practical applications, underscoring the significant potential of this technology for the advancement of DUV detectors.</p>\",\"PeriodicalId\":21612,\"journal\":{\"name\":\"Science China Technological Sciences\",\"volume\":\"245 1\",\"pages\":\"\"},\"PeriodicalIF\":4.4000,\"publicationDate\":\"2024-07-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Science China Technological Sciences\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1007/s11431-024-2660-1\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Science China Technological Sciences","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1007/s11431-024-2660-1","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, MULTIDISCIPLINARY","Score":null,"Total":0}
Surface plasmon decorated InGaO deep-UV photodetector array for image sensing and water quality monitoring via highly effective hot electron excitation and interfacial injection
In addition to the plasmon-mediated resonant coupling mechanism, the excitation of hot electron induced by plasmon presents a promising path for developing high-performance optoelectronic devices tailored for various applications. This study introduces a sophisticated design for a solar-blind ultraviolet (UV) detector array using linear In-doped Ga2O3 (InGaO) modulated by platinum (Pt) nanoparticles (PtNPs). The construction of this array involves depositing a thin film of Ga2O3 through the plasmonenhanced chemical vapor deposition (PECVD) technique. Subsequently, PtNPs were synthesized via radio-frequency magnetron sputtering and annealing process. The performance of these highly uniform arrays is significantly enhanced owing to the generation of high-energy hot electrons. This process is facilitated by non-radiative decay processes induced by PtNPs. Notably, the array achieves maximum responsivity (R) of 353 mA/W, external quantum efficiency (EQE) of 173%, detectivity (D*) of approximately 1013 Jones, and photoconductive gain of 1.58. In addition, the standard deviation for photocurrent stays below 17% for more than 80% of the array units within the array. Subsequently, the application of this array extends to photon detection in the deep-UV (DUV) range. This includes critical areas such as imaging sensing and water quality monitoring. By leveraging surface plasmon coupling, the array achieves high-performance DUV photon detection. This approach enables a broad spectrum of practical applications, underscoring the significant potential of this technology for the advancement of DUV detectors.
期刊介绍:
Science China Technological Sciences, an academic journal cosponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China, and published by Science China Press, is committed to publishing high-quality, original results in both basic and applied research.
Science China Technological Sciences is published in both print and electronic forms. It is indexed by Science Citation Index.
Categories of articles:
Reviews summarize representative results and achievements in a particular topic or an area, comment on the current state of research, and advise on the research directions. The author’s own opinion and related discussion is requested.
Research papers report on important original results in all areas of technological sciences.
Brief reports present short reports in a timely manner of the latest important results.