{"title":"基于胶体三氧化钼纳米带阵列的环保型可见光波长光电探测器","authors":"D. S. Ivan Jebakumar, Vallabha Rao Rikka","doi":"10.1002/cptc.202400038","DOIUrl":null,"url":null,"abstract":"In an era marked by growing emphasis on sustainability and innovation, the quest for eco‐friendly energy conversion devices capable of harnessing visible light has gained paramount importance. In response to this critical demand, we demonstrate visible light‐responsive photoswitching from molybdenum trioxide nanobelt arrays in the photoconductive device fabricated using solution‐processing technique. We exploit the visible light‐driven modulation of conductivity in the reversibly switchable photochromic state of MoO3 to fabricate a photochromism‐assisted photoconductive photodetector with fast response (< 0.1 s), significant on/off ratio and excellent responsivity (41 AW‐1) at 5 V. The light harvesting strategy presented herein holds the potential for efficient energy generation by harnessing visible light, even under low‐light conditions.","PeriodicalId":10108,"journal":{"name":"ChemPhotoChem","volume":"41 1","pages":""},"PeriodicalIF":3.0000,"publicationDate":"2024-07-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Eco‐friendly Visible Wavelength PhotodetectorsBasedon Colloidal Molybdenum Trioxide Nanobelt Arrays\",\"authors\":\"D. S. Ivan Jebakumar, Vallabha Rao Rikka\",\"doi\":\"10.1002/cptc.202400038\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"In an era marked by growing emphasis on sustainability and innovation, the quest for eco‐friendly energy conversion devices capable of harnessing visible light has gained paramount importance. In response to this critical demand, we demonstrate visible light‐responsive photoswitching from molybdenum trioxide nanobelt arrays in the photoconductive device fabricated using solution‐processing technique. We exploit the visible light‐driven modulation of conductivity in the reversibly switchable photochromic state of MoO3 to fabricate a photochromism‐assisted photoconductive photodetector with fast response (< 0.1 s), significant on/off ratio and excellent responsivity (41 AW‐1) at 5 V. The light harvesting strategy presented herein holds the potential for efficient energy generation by harnessing visible light, even under low‐light conditions.\",\"PeriodicalId\":10108,\"journal\":{\"name\":\"ChemPhotoChem\",\"volume\":\"41 1\",\"pages\":\"\"},\"PeriodicalIF\":3.0000,\"publicationDate\":\"2024-07-26\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ChemPhotoChem\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1002/cptc.202400038\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ChemPhotoChem","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1002/cptc.202400038","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
摘要
在这个日益强调可持续发展和创新的时代,寻求能够利用可见光的生态友好型能源转换设备变得至关重要。为了满足这一关键需求,我们在利用溶液处理技术制造的光电导器件中展示了三氧化钼纳米带阵列的可见光响应光开关。我们利用可见光驱动的 MoO3 可逆切换光致变色态的电导率调制,制造出一种光致变色辅助光电导光电探测器,在 5 V 电压下具有快速响应(0.1 秒)、显著的开/关比和出色的响应率(41 AW-1)。本文介绍的光收集策略有望通过利用可见光实现高效能源生产,即使在弱光条件下也是如此。
In an era marked by growing emphasis on sustainability and innovation, the quest for eco‐friendly energy conversion devices capable of harnessing visible light has gained paramount importance. In response to this critical demand, we demonstrate visible light‐responsive photoswitching from molybdenum trioxide nanobelt arrays in the photoconductive device fabricated using solution‐processing technique. We exploit the visible light‐driven modulation of conductivity in the reversibly switchable photochromic state of MoO3 to fabricate a photochromism‐assisted photoconductive photodetector with fast response (< 0.1 s), significant on/off ratio and excellent responsivity (41 AW‐1) at 5 V. The light harvesting strategy presented herein holds the potential for efficient energy generation by harnessing visible light, even under low‐light conditions.