{"title":"揭示基于 Ag2S 的全无机柔性热电器件在温度传感器方面的潜力","authors":"","doi":"10.1016/j.solidstatesciences.2024.107632","DOIUrl":null,"url":null,"abstract":"<div><p>Thermoelectric sensors, which are capable to convert temperature gradients into electrical signals, hold promise for use in wearable body-temperature monitors and self-powered electronic devices. However, traditional flexible thermoelectric devices constructed with organic materials have been hampered by their low energy conversion efficiency, largely stemming from the lack of ideal materials and optimized device geometry. In this study, we utilize state-of-the-art Ag<sub>2</sub>S-based inorganic materials and fine-tune the geometric parameters of full-inorganic flexible thermoelectric devices through finite element simulation. Our research reveal that these geometric parameters significantly impact the output performance of the flexible thermoelectric device. With the temperature difference set up as 25 K, the optimized device demonstrates a notable performance enhancement, particularly in terms of power density, which is 84 % higher compared to the pre-optimization state. This work introduces a novel approach for enhancing the performance of full-inorganic flexible thermoelectric devices, and also delves into the potential application of this technology in the realm of respiratory monitoring, underscoring its significance and promising prospects.</p></div>","PeriodicalId":432,"journal":{"name":"Solid State Sciences","volume":null,"pages":null},"PeriodicalIF":3.4000,"publicationDate":"2024-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Unveiling the potential of Ag2S-based full-inorganic flexible thermoelectric devices for temperature sensors\",\"authors\":\"\",\"doi\":\"10.1016/j.solidstatesciences.2024.107632\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Thermoelectric sensors, which are capable to convert temperature gradients into electrical signals, hold promise for use in wearable body-temperature monitors and self-powered electronic devices. However, traditional flexible thermoelectric devices constructed with organic materials have been hampered by their low energy conversion efficiency, largely stemming from the lack of ideal materials and optimized device geometry. In this study, we utilize state-of-the-art Ag<sub>2</sub>S-based inorganic materials and fine-tune the geometric parameters of full-inorganic flexible thermoelectric devices through finite element simulation. Our research reveal that these geometric parameters significantly impact the output performance of the flexible thermoelectric device. With the temperature difference set up as 25 K, the optimized device demonstrates a notable performance enhancement, particularly in terms of power density, which is 84 % higher compared to the pre-optimization state. This work introduces a novel approach for enhancing the performance of full-inorganic flexible thermoelectric devices, and also delves into the potential application of this technology in the realm of respiratory monitoring, underscoring its significance and promising prospects.</p></div>\",\"PeriodicalId\":432,\"journal\":{\"name\":\"Solid State Sciences\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":3.4000,\"publicationDate\":\"2024-07-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Solid State Sciences\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1293255824001973\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, INORGANIC & NUCLEAR\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Solid State Sciences","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1293255824001973","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
引用次数: 0
摘要
热电传感器能够将温度梯度转换为电信号,有望用于可穿戴体温监测器和自供电电子设备。然而,由于缺乏理想的材料和优化的器件几何形状,传统的有机材料柔性热电器件一直受到能量转换效率低的阻碍。在这项研究中,我们采用了最先进的 AgS 无机材料,并通过有限元模拟微调了全无机柔性热电器件的几何参数。我们的研究发现,这些几何参数对柔性热电器件的输出性能有重大影响。当温差设定为 25 K 时,优化后的器件表现出明显的性能提升,尤其是功率密度,与优化前相比提高了 84%。这项工作介绍了一种提高全无机柔性热电器件性能的新方法,还深入探讨了该技术在呼吸监测领域的潜在应用,凸显了其重要意义和广阔前景。
Unveiling the potential of Ag2S-based full-inorganic flexible thermoelectric devices for temperature sensors
Thermoelectric sensors, which are capable to convert temperature gradients into electrical signals, hold promise for use in wearable body-temperature monitors and self-powered electronic devices. However, traditional flexible thermoelectric devices constructed with organic materials have been hampered by their low energy conversion efficiency, largely stemming from the lack of ideal materials and optimized device geometry. In this study, we utilize state-of-the-art Ag2S-based inorganic materials and fine-tune the geometric parameters of full-inorganic flexible thermoelectric devices through finite element simulation. Our research reveal that these geometric parameters significantly impact the output performance of the flexible thermoelectric device. With the temperature difference set up as 25 K, the optimized device demonstrates a notable performance enhancement, particularly in terms of power density, which is 84 % higher compared to the pre-optimization state. This work introduces a novel approach for enhancing the performance of full-inorganic flexible thermoelectric devices, and also delves into the potential application of this technology in the realm of respiratory monitoring, underscoring its significance and promising prospects.
期刊介绍:
Solid State Sciences is the journal for researchers from the broad solid state chemistry and physics community. It publishes key articles on all aspects of solid state synthesis, structure-property relationships, theory and functionalities, in relation with experiments.
Key topics for stand-alone papers and special issues:
-Novel ways of synthesis, inorganic functional materials, including porous and glassy materials, hybrid organic-inorganic compounds and nanomaterials
-Physical properties, emphasizing but not limited to the electrical, magnetical and optical features
-Materials related to information technology and energy and environmental sciences.
The journal publishes feature articles from experts in the field upon invitation.
Solid State Sciences - your gateway to energy-related materials.