用磁性 Fe3O4@Au@m-ABS 纳米粒子提高有机太阳能电池的功率转换效率

Nanomaterials Pub Date : 2024-07-10 DOI:10.3390/nano14141175
Pradeep Kumar, Shih-Han Huang, Chia-Yi Hsu, Ssu-Yung Chung, H. Cha, Chih-Min Chuang, Kuen-Lin Chen, Yu-Ching Huang
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摘要

有机-无机纳米复合材料因其生态友好性、合适的带隙和高稳定性而具有应用于光伏材料的潜力。在这项工作中,我们将金和 Fe3O4 磁性纳米粒子与聚间氨基苯磺酸(m-ABS)结合在一起,合成了 Fe3O4@Au@聚(间氨基苯磺酸)(Fe3O4@Au@m-ABS)磁光电纳米粒子(MPNPs),以提高有机光伏(OPV)的性能。这些 MPNPs 具有宽泛的紫外可见吸收和 2.878 eV 的低带隙,因此更适合光伏应用。为了研究 MPNPs 对 OPV 功率转换效率(PCE)的影响,我们在 ZnO 电子传输层(ETL)和活性层中引入了 MPNPs。当在 ETL 中加入 0.1 vol% 的 MPNPs 时,OPV 的 PCE 为 14.24%,填充因子 (FF) 为 69.10%。另一方面,在活性层中加入 0.1 Vol% 的 MPNPs 时,OPV 的 PCE 为 14.11%,FF 为 68.83%。然而,没有加入 MPNPs 的 OPV 的 PCE 只有 13.15%,FF 为 63.69%。加入 MPNPs 后,OPV 器件的 PCE 增加了 8.3%。这些研究结果表明,Fe3O4@Au@m-ABS MPNPs 是一种很有前途的纳米复合材料,可用于提高 OPV 的性能。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Enhancing Power Conversion Efficiency of Organic Solar Cells with Magnetoplasmonic Fe3O4@Au@m-ABS Nanoparticles
Organic–inorganic nanocomposites have the potential to be used in photovoltaic materials due to their eco-friendliness, suitable band gaps, and high stability. In this work, we integrated gold and Fe3O4 magnetic nanoparticles with poly-m-amino benzene sulfonic (m-ABS) to synthesize Fe3O4@Au@poly-(m-aminobenzenesulfonic acid) (Fe3O4@Au@m-ABS) magneto-plasmonic nanoparticles (MPNPs) to enhance the performance of the organic photovoltaic (OPV). These MPNPs exhibit broad UV-Vis absorption and a low band gap of 2.878 eV, enhancing their suitability for photovoltaic applications. The MPNPs were introduced into the ZnO electron transporting layer (ETL) and active layer to investigate the influence of MPNPs on the power conversion efficiency (PCE) of the OPVs. When 0.1 vol% MPNPs were incorporated in the ETL, the OPVs achieved a PCE of 14.24% and a fill factor (FF) of 69.10%. On the other hand, when 0.1 vol% MPNPs were incorporated in the active layer, the OPVs showed a PCE of 14.11% and an FF of 68.83%. However, the OPVs without MPNPs only possessed a PCE of 13.15% and an FF of 63.69%. The incorporation of MPNPs increased the PCE by 8.3% in the OPV device. These findings suggest that Fe3O4@Au@m-ABS MPNPs are promising nanocomposite materials for enhancing the performance of OPVs.
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