利用同步衰变曲线分析法研究天然铂上α粒子诱导反应的异构体产生,最高可达29兆电子伏

Naohiko Otuka, Sandor Takacs, Masayuki Aikawa, Shuichiro Ebata, Hiromitsu Haba
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引用次数: 0

摘要

利用标准叠箔活化技术和伽马射线光谱法,对天然铂上α粒子诱导反应产生的^{198}$Au、^{197}$Hg和^{195}$Hg的同分异构体比率进行了实验研究,结果表明,在29 MeV以下,α粒子诱导反应产生的^{198}$Au、^{197}$Hg和^{195}$Hg的同分异构体比率与冷却时间有很大关系。根据传统活化截面公式确定的 $^{197}$Hg 和 $^{195}$Hg 的异构体比率显示出强烈的冷却时间依赖性。利用同步衰变曲线分析框架调整了这两种同位素的异构转变分支比,从而解决了时间依赖性问题。我们的分析表明,^{197m}$Hg(24 小时)和^{195m}$Hg(42 小时)的异构转变分支比分别为 94.5% 和 48.9%。我们还利用这些修正后的异构转变支化比测量了$^{198}$Au、$^{197}$Hg、$^{195}$Hg和其他一些汞、金和铂同位素的低至6 MeV的异构转变支化比和独立产生截面,并与TALYS-2.0统计模型和前平衡模型的预测进行了比较,以讨论参数依赖性。我们发现,如果将自旋切参数减小到用刚体惯性矩估算的参数的一半或更小,则测得的异构比预测结果会更好。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Isomer production studied with simultaneous decay curve analysis for alpha-particle induced reactions on natural platinum up to 29 MeV
The isomeric ratios of $^{198}$Au, $^{197}$Hg and $^{195}$Hg produced by $\alpha$-particle induced reactions on natural platinum were investigated experimentally up to 29 MeV by using the standard stacked foil activation technique and $\gamma$-ray spectrometry. The isomeric ratios of $^{197}$Hg and $^{195}$Hg determined by the conventional activation cross section formula showed strong cooling time dependence. The time dependence was resolved by adjusting the isomeric transition branching ratios for the two isotopes within a simultaneous decay curve analysis framework. Our analysis suggests 94.5$\pm$0.7% and 48.9$\pm$1.8% as the isomeric transition branching ratios of $^{197m}$Hg (24 h) and $^{195m}$Hg (42 h), respectively. The isomeric ratios and independent production cross sections of $^{198}$Au, $^{197}$Hg, $^{195}$Hg and some other Hg, Au and Pt isotopes were also measured down to 6 MeV with these corrected isomeric transition branching ratios, and compared with predictions of statistical and pre-equilibrium models by TALYS-2.0 to discuss spin cuto? parameter dependence. We found the measured isomeric ratios are better predicted if we reduce the spin cuto? parameter to half or less from that estimated with the rigid body moment of inertia.
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