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引用次数: 0
摘要
微液滴形成已广泛应用于三维打印、增材制造、化学合成等领域。全面了解微滴的形成对于上述领域的工艺优化非常必要。本文基于 OpenFOAM,采用 Giesekus(GK)模型模拟 T 型微通道中粘弹性液滴的形成。通过改变分散相的弛豫时间、聚合物粘度和通道壁接触角,研究了液相弹性、粘度和通道壁润湿性对粘弹性液滴形成的影响。比较了不同操作条件下的压力特性、液滴最终长度和脱离时间。模拟结果以压力的形式描述了流体参数对液滴形成的影响,用来补充现有应力实验的不足。结果表明,在拉伸阶段,弹性会阻碍液滴破裂。随着聚合物粘度的增加,液滴的弹性会显著增加,从而阻止液滴丝的拉伸和断裂,导致液滴形成的频率变慢。此外,还观察了壁面接触角和流体流速对 T 型微通道中粘弹性液滴形成的影响。研究发现,壁面接触角对最终液滴长度的影响也不容忽视。
Simulation of viscoelastic droplet formation in T-type microchannels using OpenFOAM
Microdroplet formation has been widely used in 3D printing, additive manufacturing, chemical synthesis and other fields. Comprehensive understanding for the microdroplet formation is necessary for process optimization of the above-mentioned fields. In this paper, the Giesekus (GK) model is used to simulate the formation of viscoelastic droplet in T-type microchannels based on OpenFOAM. The effects of liquid phase elasticity, viscosity and channel wall wettability on the formation of viscoelastic droplet were investigated by changing the relaxation time of the dispersed phase, polymer viscosity and wall contact angle. The pressure characteristics, droplet final lengths and detachment time were compared under different operating conditions. The simulation results describe the effect of fluid parameters on droplet formation in the form of pressure, which is used to supplement the shortcomings of existing experiments in stress. The results show that the elasticity hinders droplet breakup during the stretching stage. As the polymer viscosity increases, there is a significant increase in the elasticity of the droplet, which prevents the droplet filaments from stretching and breaking, resulting in a slower frequency of droplet formation. Moreover, the influence of wall contact angle and fluid flow rate on the formation of viscoelastic droplets in T-shaped microchannel is also observed. It is found that the wall contact angle also has an impact on the final droplet length, which cannot be ignored.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.