超冷液体弹塑性模型玻璃化动力学的均方场分析

IF 1.8 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY
EPL Pub Date : 2024-05-14 DOI:10.1209/0295-5075/ad3b35
J. W. Baron and G. Biroli
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引用次数: 0

摘要

我们提出了超冷液体粗粒度模型的均场理论,在该模型中,弛豫是通过局部塑性重排发生的。局部弛豫可以由热波动或其他重排的长程弹性后果引起。我们提取了弛豫时间和动态关联长度尺度的温度依赖性。我们发现了两种动力学状态。首先,在临界温度 Tc 时,特征时间和长度尺度以幂律发散。这种状态是通过忽略活化弛豫通道的近似方法发现的,可以解释为类似于玻璃的模耦合转变。实际上,在 Tc 时只发生了一次交叉。残余塑性活动导致了第二种情况,其特征是低于 Tc 时的阿伦尼乌斯定律。在这种情况下,我们发现支配动态相关性的长度尺度以幂律的形式发散,与弛豫时间成对数关系。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Mean-field analysis of the glassy dynamics of an elastoplastic model of super-cooled liquids
We present a mean-field theory of a coarse-grained model of a super-cooled liquid in which relaxation occurs via local plastic rearrangements. Local relaxation can be induced by thermal fluctuations or by the long-range elastic consequences of other rearrangements. We extract the temperature dependence of both the relaxation time and the length scale of dynamical correlations. We find two dynamical regimes. First, a regime in which the characteristic time and length scales diverge as a power law at a critical temperature Tc. This regime is found by an approximation that neglects activated relaxation channels, which can be interpreted as akin to the one found by the mode-coupling transition of glasses. In reality, only a crossover takes place at Tc. The residual plastic activity leads to a second regime characterised by an Arrhenius law below Tc. In this case, we show that the length scale governing dynamical correlations diverges as a power law as , and is logarithmically related to the relaxation time.
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来源期刊
EPL
EPL 物理-物理:综合
CiteScore
3.30
自引率
5.60%
发文量
332
审稿时长
1.9 months
期刊介绍: General physics – physics of elementary particles and fields – nuclear physics – atomic, molecular and optical physics – classical areas of phenomenology – physics of gases, plasmas and electrical discharges – condensed matter – cross-disciplinary physics and related areas of science and technology. Letters submitted to EPL should contain new results, ideas, concepts, experimental methods, theoretical treatments, including those with application potential and be of broad interest and importance to one or several sections of the physics community. The presentation should satisfy the specialist, yet remain understandable to the researchers in other fields through a suitable, clearly written introduction and conclusion (if appropriate). EPL also publishes Comments on Letters previously published in the Journal.
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