Xin Yang, Yankuan Tian, Rong Zhou, Feng Xia, Yifei Gong, Chengming Zhang, Feng Ji, Liu Liu, Faxue Li, Ruiyun Zhang, Jianyong Yu, Tingting Gao
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引用次数: 0
摘要
在常温下实现重油的高效清洁是一项世界性挑战。针对高粘度油类泄漏的传统清理方法吸收效率较低,并且存在严重的实际操作限制。在此,我们从小叶女贞(Salvinia cucullata)的被动传输过程中汲取灵感,利用可扩展的静电植绒技术,开发出一种基于太阳能加热和焦耳热的纺织品吸收剂。得益于高效的光热和电热转换效应,这种纺织吸收剂具有亲油性和排列整齐的通道,有利于热传导,从而提高重油吸收率。这种吸收器对有机溶剂(氯仿和二氯甲烷)和低粘度油(硅油、汽油和柴油)具有很高的吸收效率。在一个太阳光照射(或 5 V 电压)下,纺织吸收器的表面温度在 120 秒(240 秒)内迅速升至 92 ℃(114 ℃),导致重油粘度急剧下降,然后达到超高吸收率(2647 kg h-1 m-2)和快速平衡时间(25 秒)。快速吸收率大大减少了溢油清理时间和溢油扩散面积,从而尽可能减轻溢油对环境造成的危害。所提出的具有对齐通道的太阳能加热和焦耳热纺织品吸收器显示出高效吸收重油的巨大潜力。 图文摘要
Bioinspired Design of Textile-Based Absorbers: Photothermal and Electrothermal Synergistic Conversion for Efficient Clean-Up of Heavy Oil
It is a worldwide challenge to achieve an efficient cleaning of heavy oil at ambient temperature. Conventional cleanup methods for high-viscosity oil spills exhibit low absorption efficiency and have severe practical operating limits. Herein, inspired by the passive transport process in the Salvinia cucullata, a solar-heated and joule-heated textile-based absorber using the scalable electrostatic flocking technique. Benefiting from the efficient photothermal and electrothermal conversion effects, the textile-based absorber, with oleophilic and aligned channels, facilitates thermal conduction and hence enhances heavy oil absorption. The absorber is highly efficient for organic solvents (chloroform and dichloromethane) and low-viscosity oils (silicone oil, gasoline, and diesel oil). The surface temperature of the textile absorber rises rapidly to 92 °C (114 °C) in 120 s (240 s) under one sun irradiation (or 5 V voltage), resulting in a sharp drop in the viscosity of the heavy oil and then achieving an ultrahigh absorption rate (2647 kg h−1 m−2) and fast equilibrium time (25 s). Rapid absorption rate significantly reduces spill cleanup time and spill spreading area, hence alleviating the environmental harm caused by oil spills as much as possible. The proposed solar-heated and joule-heated textile-based absorbers with aligned channels show great potential for efficient heavy oil absorption.
期刊介绍:
Advanced Fiber Materials is a hybrid, peer-reviewed, international and interdisciplinary research journal which aims to publish the most important papers in fibers and fiber-related devices as well as their applications.Indexed by SCIE, EI, Scopus et al.
Publishing on fiber or fiber-related materials, technology, engineering and application.