高溶剂粘度下粘弹性溶液的粒子迁移逆转

IF 2.7 2区 工程技术 Q2 MECHANICS
Xavier Salas-Barzola , Guillaume Maîtrejean , Clément de Loubens , Antoine Naillon , Enric Santanach Carreras , Hugues Bodiguel
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引用次数: 0

摘要

在压力驱动的粘弹性流动中,颗粒周围法向应力的不平衡会诱发颗粒的横向迁移,从而为在微流体设备中操纵颗粒提供了可能性。理论预测与粒子向流动中心线迁移的实验证据一致。然而,这些论点受到了实验和数值研究的挑战,揭示了粘弹性剪切稀化流体迁移方向逆转的可能性。然而,粘弹性液体的一个重要特性在很大程度上仍未被探索,那就是溶剂粘度与溶剂和聚合物粘度之和的比值,用 β 表示。 我们利用 Oldroyd-B 构成方程计算了一个自由流动的圆柱体在二维 Poiseuille 流体中的升力系数。随着 β 值的增加,升力系数从负值(中心线迁移)过渡到正值(壁面迁移)。与惯性升力类似,升力系数的符号变化与粒子旋转速度的突然变化(尽管很小)密切相关。我们为升力系数建立了一个缩放定律,该定律与预期的魏森堡数成正比,同时也与粘弹性和牛顿情况下的旋转速度差成正比。如果粒子的旋转速度快于牛顿情况,它就会向壁面移动;反之,如果粒子的旋转速度慢于牛顿情况,它就会向通道中心线移动。最后,在微流体狭缝中进行的实验证实,高粘度比的粘弹性流体会向壁面迁移。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Reversal of particle Migration for viscoelastic solution at high solvent viscosity

The imbalance of normal stress around a particle induces its transverse migration in pressure-driven viscoelastic flow, offering possibilities for particle manipulation in microfluidic devices. Theoretical predictions align with experimental evidence of particles migrating towards the center-line of the flow. However, these arguments have been challenged by both experimental and numerical investigations, revealing the potential for a reversal in the direction of migration for viscoelastic shear-thinning fluids. Yet, a significant property of viscoelastic liquids that remains largely unexplored is the ratio of solvent viscosity to the sum of solvent and polymer viscosities, denoted as β. We computed the lift coefficients of a freely flowing cylinder in a bi-dimensional Poiseuille flow with Oldroyd-B constitutive equations. A transition from a negative (center-line migration) to a positive (wall migration) lift coefficient was demonstrated with increasing β values. Analogous to inertial lift, the changes in the sign of the lift coefficient were strongly correlated with abrupt (albeit small) variations in the rotation velocity of the particle. We established a scaling law for the lift coefficient that is proportional, as expected, to the Weissenberg number, but also to the difference in rotation velocity between the viscoelastic and Newtonian cases. If the particle rotates more rapidly than in the Newtonian case, it migrates towards the wall; conversely, if the particle rotates more slowly than in the Newtonian case, it migrates towards the center-line of the channel. Finally, experiments in microfluidic slits confirmed migration towards the wall for viscoelastic fluids with high viscosity ratio.

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来源期刊
CiteScore
5.00
自引率
19.40%
发文量
109
审稿时长
61 days
期刊介绍: The Journal of Non-Newtonian Fluid Mechanics publishes research on flowing soft matter systems. Submissions in all areas of flowing complex fluids are welcomed, including polymer melts and solutions, suspensions, colloids, surfactant solutions, biological fluids, gels, liquid crystals and granular materials. Flow problems relevant to microfluidics, lab-on-a-chip, nanofluidics, biological flows, geophysical flows, industrial processes and other applications are of interest. Subjects considered suitable for the journal include the following (not necessarily in order of importance): Theoretical, computational and experimental studies of naturally or technologically relevant flow problems where the non-Newtonian nature of the fluid is important in determining the character of the flow. We seek in particular studies that lend mechanistic insight into flow behavior in complex fluids or highlight flow phenomena unique to complex fluids. Examples include Instabilities, unsteady and turbulent or chaotic flow characteristics in non-Newtonian fluids, Multiphase flows involving complex fluids, Problems involving transport phenomena such as heat and mass transfer and mixing, to the extent that the non-Newtonian flow behavior is central to the transport phenomena, Novel flow situations that suggest the need for further theoretical study, Practical situations of flow that are in need of systematic theoretical and experimental research. Such issues and developments commonly arise, for example, in the polymer processing, petroleum, pharmaceutical, biomedical and consumer product industries.
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