Xavier Salas-Barzola , Guillaume Maîtrejean , Clément de Loubens , Antoine Naillon , Enric Santanach Carreras , Hugues Bodiguel
{"title":"高溶剂粘度下粘弹性溶液的粒子迁移逆转","authors":"Xavier Salas-Barzola , Guillaume Maîtrejean , Clément de Loubens , Antoine Naillon , Enric Santanach Carreras , Hugues Bodiguel","doi":"10.1016/j.jnnfm.2024.105234","DOIUrl":null,"url":null,"abstract":"<div><p>The imbalance of normal stress around a particle induces its transverse migration in pressure-driven viscoelastic flow, offering possibilities for particle manipulation in microfluidic devices. Theoretical predictions align with experimental evidence of particles migrating towards the center-line of the flow. However, these arguments have been challenged by both experimental and numerical investigations, revealing the potential for a reversal in the direction of migration for viscoelastic shear-thinning fluids. Yet, a significant property of viscoelastic liquids that remains largely unexplored is the ratio of solvent viscosity to the sum of solvent and polymer viscosities, denoted as <span><math><mi>β</mi></math></span>. We computed the lift coefficients of a freely flowing cylinder in a bi-dimensional Poiseuille flow with Oldroyd-B constitutive equations. A transition from a negative (center-line migration) to a positive (wall migration) lift coefficient was demonstrated with increasing <span><math><mi>β</mi></math></span> values. Analogous to inertial lift, the changes in the sign of the lift coefficient were strongly correlated with abrupt (albeit small) variations in the rotation velocity of the particle. We established a scaling law for the lift coefficient that is proportional, as expected, to the Weissenberg number, but also to the difference in rotation velocity between the viscoelastic and Newtonian cases. If the particle rotates more rapidly than in the Newtonian case, it migrates towards the wall; conversely, if the particle rotates more slowly than in the Newtonian case, it migrates towards the center-line of the channel. Finally, experiments in microfluidic slits confirmed migration towards the wall for viscoelastic fluids with high viscosity ratio.</p></div>","PeriodicalId":54782,"journal":{"name":"Journal of Non-Newtonian Fluid Mechanics","volume":"329 ","pages":"Article 105234"},"PeriodicalIF":2.7000,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Reversal of particle Migration for viscoelastic solution at high solvent viscosity\",\"authors\":\"Xavier Salas-Barzola , Guillaume Maîtrejean , Clément de Loubens , Antoine Naillon , Enric Santanach Carreras , Hugues Bodiguel\",\"doi\":\"10.1016/j.jnnfm.2024.105234\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The imbalance of normal stress around a particle induces its transverse migration in pressure-driven viscoelastic flow, offering possibilities for particle manipulation in microfluidic devices. Theoretical predictions align with experimental evidence of particles migrating towards the center-line of the flow. However, these arguments have been challenged by both experimental and numerical investigations, revealing the potential for a reversal in the direction of migration for viscoelastic shear-thinning fluids. Yet, a significant property of viscoelastic liquids that remains largely unexplored is the ratio of solvent viscosity to the sum of solvent and polymer viscosities, denoted as <span><math><mi>β</mi></math></span>. We computed the lift coefficients of a freely flowing cylinder in a bi-dimensional Poiseuille flow with Oldroyd-B constitutive equations. A transition from a negative (center-line migration) to a positive (wall migration) lift coefficient was demonstrated with increasing <span><math><mi>β</mi></math></span> values. Analogous to inertial lift, the changes in the sign of the lift coefficient were strongly correlated with abrupt (albeit small) variations in the rotation velocity of the particle. We established a scaling law for the lift coefficient that is proportional, as expected, to the Weissenberg number, but also to the difference in rotation velocity between the viscoelastic and Newtonian cases. If the particle rotates more rapidly than in the Newtonian case, it migrates towards the wall; conversely, if the particle rotates more slowly than in the Newtonian case, it migrates towards the center-line of the channel. Finally, experiments in microfluidic slits confirmed migration towards the wall for viscoelastic fluids with high viscosity ratio.</p></div>\",\"PeriodicalId\":54782,\"journal\":{\"name\":\"Journal of Non-Newtonian Fluid Mechanics\",\"volume\":\"329 \",\"pages\":\"Article 105234\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2024-03-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Non-Newtonian Fluid Mechanics\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0377025724000508\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MECHANICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Non-Newtonian Fluid Mechanics","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0377025724000508","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MECHANICS","Score":null,"Total":0}
Reversal of particle Migration for viscoelastic solution at high solvent viscosity
The imbalance of normal stress around a particle induces its transverse migration in pressure-driven viscoelastic flow, offering possibilities for particle manipulation in microfluidic devices. Theoretical predictions align with experimental evidence of particles migrating towards the center-line of the flow. However, these arguments have been challenged by both experimental and numerical investigations, revealing the potential for a reversal in the direction of migration for viscoelastic shear-thinning fluids. Yet, a significant property of viscoelastic liquids that remains largely unexplored is the ratio of solvent viscosity to the sum of solvent and polymer viscosities, denoted as . We computed the lift coefficients of a freely flowing cylinder in a bi-dimensional Poiseuille flow with Oldroyd-B constitutive equations. A transition from a negative (center-line migration) to a positive (wall migration) lift coefficient was demonstrated with increasing values. Analogous to inertial lift, the changes in the sign of the lift coefficient were strongly correlated with abrupt (albeit small) variations in the rotation velocity of the particle. We established a scaling law for the lift coefficient that is proportional, as expected, to the Weissenberg number, but also to the difference in rotation velocity between the viscoelastic and Newtonian cases. If the particle rotates more rapidly than in the Newtonian case, it migrates towards the wall; conversely, if the particle rotates more slowly than in the Newtonian case, it migrates towards the center-line of the channel. Finally, experiments in microfluidic slits confirmed migration towards the wall for viscoelastic fluids with high viscosity ratio.
期刊介绍:
The Journal of Non-Newtonian Fluid Mechanics publishes research on flowing soft matter systems. Submissions in all areas of flowing complex fluids are welcomed, including polymer melts and solutions, suspensions, colloids, surfactant solutions, biological fluids, gels, liquid crystals and granular materials. Flow problems relevant to microfluidics, lab-on-a-chip, nanofluidics, biological flows, geophysical flows, industrial processes and other applications are of interest.
Subjects considered suitable for the journal include the following (not necessarily in order of importance):
Theoretical, computational and experimental studies of naturally or technologically relevant flow problems where the non-Newtonian nature of the fluid is important in determining the character of the flow. We seek in particular studies that lend mechanistic insight into flow behavior in complex fluids or highlight flow phenomena unique to complex fluids. Examples include
Instabilities, unsteady and turbulent or chaotic flow characteristics in non-Newtonian fluids,
Multiphase flows involving complex fluids,
Problems involving transport phenomena such as heat and mass transfer and mixing, to the extent that the non-Newtonian flow behavior is central to the transport phenomena,
Novel flow situations that suggest the need for further theoretical study,
Practical situations of flow that are in need of systematic theoretical and experimental research. Such issues and developments commonly arise, for example, in the polymer processing, petroleum, pharmaceutical, biomedical and consumer product industries.