金属纳米粒子的声子散热和纳米粒子低温冷却动力学

A. Bezuglyj, L. Davydov
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引用次数: 0

摘要

对嵌入电介质基体的金属纳米粒子电子-声子系统能量弛豫的理论分析通常基于电子和声子温度的半现象学动态方程(双温模型),该模型没有考虑声子分布函数的非热性质。在这项工作中,我们使用了一个微观模型,该模型通过声子分布函数的动力学方程来描述金属纳米棒和金属球形纳米粒子的电子-声子系统的动力学。我们的重点是纳米粒子向介电基体传热时的尺寸效应。如果纳米粒子的尺寸远大于声子-电子平均自由路径,则热量传递由纳米粒子和基体之间的界面特性决定。在相反的情况下,热量的带走完全由金属纳米粒子中电子-声子相互作用的参数决定。此外,还考虑了纳米粒子的冷却动力学,并得出了电子温度与时间的关系。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Phonon heat removal from metal nano-particles and dynamics of nano-particle cooling at low temperatures
The theoretical analysis of the energy relaxation of an electron-phonon system of metal nanoparticles embedded in a dielectric matrix is usually based on semiphenomenological dynamic equations for electron and phonon temperatures (two-temperature model), which does not take into account the non-thermal nature of the phonon distribution function. In this work, we use a microscopic model that describes the dynamics of the electron-phonon system of metal nanorods and metal spherical nanoparticles in terms of the kinetic equation for the phonon distribution function. We focus on the size effect in the transfer of heat from a nanoparticle to a dielectric matrix. If the dimensions of the nanoparticle are much larger than the phonon-electron mean free path, then the heat transfer is determined by the properties of the interface between the nanoparticle and the matrix. In the opposite case, heat removal is determined solely by the parameters of the electron-phonon interaction in a metal nanoparticle. The dynamics of cooling of nanoparticles is also considered and the dependence of the electron temperature on time is obtained.
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