Fan Zhang , Xiyuan Zhang , Bowen Wang , Haipeng Zhai , Kangcheng Wu , Zixuan Wang , Zhiming Bao , Wanli Tian , Weikang Duan , Bingfeng Zu , Zhengwei Gong , Kui Jiao
{"title":"-基于数据驱动代用模型和多目标优化算法的 PEMFC -30°C 冷启动优化技术","authors":"Fan Zhang , Xiyuan Zhang , Bowen Wang , Haipeng Zhai , Kangcheng Wu , Zixuan Wang , Zhiming Bao , Wanli Tian , Weikang Duan , Bingfeng Zu , Zhengwei Gong , Kui Jiao","doi":"10.1016/j.dche.2024.100144","DOIUrl":null,"url":null,"abstract":"<div><p>Cold start is a critical operating scenario for the proton exchange membrane fuel cell (PEMFC), particularly in the field of transportation. Under sub-freezing temperatures, the water inside the cell will freeze and obstruct gas flow paths as well as cover catalyst reaction sites, resulting in a failed startup. This study proposes an optimization method for the -30°C cold start of PEMFC based on a data-driven surrogate model to improve cold start performance and reduce irreversible damage to the cell. A validated PEMFC cold start mechanism model is utilized as the basis for developing an extreme learning machine (ELM) based data-driven surrogate model, which is trained using data collected from the mechanism model and has higher computational efficiency compared with the original model. In addition, the NSGA-II multi-objective optimization algorithm is employed to optimize the current loading strategies and operating parameters using the surrogate model as fitness function. The objectives are to enhance the minimum voltage and reduce startup duration time. Moreover, experimental validation confirms the effectiveness of the proposed method. The test results demonstrate that a cold start from -30°C is achieved within 97 s, with the minimum voltage reaching 0.44 V. Notably, there is a reduction in startup time by 26 s and an increase in the minimum voltage by 0.06 V compared to the base case. This study establishes a foundation for researchers to adjust operating settings during cold start based on diverse applications and requirements.</p></div>","PeriodicalId":72815,"journal":{"name":"Digital Chemical Engineering","volume":"10 ","pages":"Article 100144"},"PeriodicalIF":3.0000,"publicationDate":"2024-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2772508124000061/pdfft?md5=e12420b70e8952fb11b8c8b1052f6837&pid=1-s2.0-S2772508124000061-main.pdf","citationCount":"0","resultStr":"{\"title\":\"-30°C cold start optimization of PEMFC based on a data-driven surrogate model and multi-objective optimization algorithm\",\"authors\":\"Fan Zhang , Xiyuan Zhang , Bowen Wang , Haipeng Zhai , Kangcheng Wu , Zixuan Wang , Zhiming Bao , Wanli Tian , Weikang Duan , Bingfeng Zu , Zhengwei Gong , Kui Jiao\",\"doi\":\"10.1016/j.dche.2024.100144\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Cold start is a critical operating scenario for the proton exchange membrane fuel cell (PEMFC), particularly in the field of transportation. Under sub-freezing temperatures, the water inside the cell will freeze and obstruct gas flow paths as well as cover catalyst reaction sites, resulting in a failed startup. This study proposes an optimization method for the -30°C cold start of PEMFC based on a data-driven surrogate model to improve cold start performance and reduce irreversible damage to the cell. A validated PEMFC cold start mechanism model is utilized as the basis for developing an extreme learning machine (ELM) based data-driven surrogate model, which is trained using data collected from the mechanism model and has higher computational efficiency compared with the original model. In addition, the NSGA-II multi-objective optimization algorithm is employed to optimize the current loading strategies and operating parameters using the surrogate model as fitness function. The objectives are to enhance the minimum voltage and reduce startup duration time. Moreover, experimental validation confirms the effectiveness of the proposed method. The test results demonstrate that a cold start from -30°C is achieved within 97 s, with the minimum voltage reaching 0.44 V. Notably, there is a reduction in startup time by 26 s and an increase in the minimum voltage by 0.06 V compared to the base case. This study establishes a foundation for researchers to adjust operating settings during cold start based on diverse applications and requirements.</p></div>\",\"PeriodicalId\":72815,\"journal\":{\"name\":\"Digital Chemical Engineering\",\"volume\":\"10 \",\"pages\":\"Article 100144\"},\"PeriodicalIF\":3.0000,\"publicationDate\":\"2024-02-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S2772508124000061/pdfft?md5=e12420b70e8952fb11b8c8b1052f6837&pid=1-s2.0-S2772508124000061-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Digital Chemical Engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2772508124000061\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Digital Chemical Engineering","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2772508124000061","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
-30°C cold start optimization of PEMFC based on a data-driven surrogate model and multi-objective optimization algorithm
Cold start is a critical operating scenario for the proton exchange membrane fuel cell (PEMFC), particularly in the field of transportation. Under sub-freezing temperatures, the water inside the cell will freeze and obstruct gas flow paths as well as cover catalyst reaction sites, resulting in a failed startup. This study proposes an optimization method for the -30°C cold start of PEMFC based on a data-driven surrogate model to improve cold start performance and reduce irreversible damage to the cell. A validated PEMFC cold start mechanism model is utilized as the basis for developing an extreme learning machine (ELM) based data-driven surrogate model, which is trained using data collected from the mechanism model and has higher computational efficiency compared with the original model. In addition, the NSGA-II multi-objective optimization algorithm is employed to optimize the current loading strategies and operating parameters using the surrogate model as fitness function. The objectives are to enhance the minimum voltage and reduce startup duration time. Moreover, experimental validation confirms the effectiveness of the proposed method. The test results demonstrate that a cold start from -30°C is achieved within 97 s, with the minimum voltage reaching 0.44 V. Notably, there is a reduction in startup time by 26 s and an increase in the minimum voltage by 0.06 V compared to the base case. This study establishes a foundation for researchers to adjust operating settings during cold start based on diverse applications and requirements.