{"title":"评估 Partector Pro 在城市背景场地进行大气粒径分布和数量浓度测量的情况","authors":"C. Asbach, A. Todea, Heinz Kaminski","doi":"10.5194/ar-2-1-2024","DOIUrl":null,"url":null,"abstract":"Abstract. Particle number size distributions, total number concentrations and mean particle sizes have been measured for 70 d at an urban background site in Mülheim-Styrum, Germany, with a handheld Partector Pro of the first generation and a TSI mobility particle size spectrometer (MPSS). The aim of the study was to evaluate the performance of the Partector Pro against the MPSS. The results show that the size distributions, measured with the Partector Pro, agree with the MPSS mostly within ± 25 % for particle sizes between 10 and 113.5 nm, whereas higher, systematic differences were observed for larger particles. The measurement accuracy was shown to be dependent on the geometric mean diameter and the geometric standard deviation of the aerosol. Best results were found for the most abundant size distributions with geometric mean particle diameters ≥ 30 nm and geometric standard deviations larger than 1.8. The total number concentration, measured by the Partector Pro, was found to be in excellent agreement with the MPSS with a slope of the linear fit of 0.9977 and a regression coefficient of R2=0.9956. The agreement of the geometric mean particle diameter, determined with the Partector Pro and the MPSS was good but moderately dependent on the particle size distribution. For mean particle sizes between 20 and 50 nm, the bias was within ±15 %. Higher deviations of up to 30 % were observed when the geometric mean particle sizes exceeded 70 nm and when the geometric standard deviations exceeded approximately 2.7.\n","PeriodicalId":511317,"journal":{"name":"Aerosol Research","volume":" 7","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2024-01-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Evaluation of a Partector Pro for atmospheric particle number size distribution and number concentration measurements at an urban background site\",\"authors\":\"C. Asbach, A. Todea, Heinz Kaminski\",\"doi\":\"10.5194/ar-2-1-2024\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Abstract. Particle number size distributions, total number concentrations and mean particle sizes have been measured for 70 d at an urban background site in Mülheim-Styrum, Germany, with a handheld Partector Pro of the first generation and a TSI mobility particle size spectrometer (MPSS). The aim of the study was to evaluate the performance of the Partector Pro against the MPSS. The results show that the size distributions, measured with the Partector Pro, agree with the MPSS mostly within ± 25 % for particle sizes between 10 and 113.5 nm, whereas higher, systematic differences were observed for larger particles. The measurement accuracy was shown to be dependent on the geometric mean diameter and the geometric standard deviation of the aerosol. Best results were found for the most abundant size distributions with geometric mean particle diameters ≥ 30 nm and geometric standard deviations larger than 1.8. The total number concentration, measured by the Partector Pro, was found to be in excellent agreement with the MPSS with a slope of the linear fit of 0.9977 and a regression coefficient of R2=0.9956. The agreement of the geometric mean particle diameter, determined with the Partector Pro and the MPSS was good but moderately dependent on the particle size distribution. For mean particle sizes between 20 and 50 nm, the bias was within ±15 %. Higher deviations of up to 30 % were observed when the geometric mean particle sizes exceeded 70 nm and when the geometric standard deviations exceeded approximately 2.7.\\n\",\"PeriodicalId\":511317,\"journal\":{\"name\":\"Aerosol Research\",\"volume\":\" 7\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-01-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Aerosol Research\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.5194/ar-2-1-2024\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Aerosol Research","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.5194/ar-2-1-2024","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
摘要
摘要。使用第一代手持式 Partector Pro 和 TSI 移动式粒度光谱仪(MPSS),在德国米尔海姆-施特鲁姆的一个城市背景场地测量了 70 天的粒数粒径分布、总粒数浓度和平均粒径。研究的目的是评估 Partector Pro 和 MPSS 的性能。结果表明,用 Partector Pro 测得的粒度分布与 MPSS 测得的粒度分布基本吻合,粒度在 10 至 113.5 nm 之间时,吻合度在± 25 %以内,而粒度较大时,系统性差异较大。测量精度取决于气溶胶的几何平均直径和几何标准偏差。几何平均粒径≥ 30 nm、几何标准偏差大于 1.8 的最丰富粒度分布的测量结果最佳。用 Partector Pro 测量的总数量浓度与 MPSS 非常吻合,线性拟合斜率为 0.9977,回归系数 R2=0.9956。用 Partector Pro 和 MPSS 测定的几何平均粒径的一致性很好,但在一定程度上取决于粒度分布。平均粒径在 20 至 50 nm 之间时,偏差在 ±15 % 范围内。当几何平均粒径超过 70 nm 和几何标准偏差超过约 2.7 时,偏差较大,可达 30%。
Evaluation of a Partector Pro for atmospheric particle number size distribution and number concentration measurements at an urban background site
Abstract. Particle number size distributions, total number concentrations and mean particle sizes have been measured for 70 d at an urban background site in Mülheim-Styrum, Germany, with a handheld Partector Pro of the first generation and a TSI mobility particle size spectrometer (MPSS). The aim of the study was to evaluate the performance of the Partector Pro against the MPSS. The results show that the size distributions, measured with the Partector Pro, agree with the MPSS mostly within ± 25 % for particle sizes between 10 and 113.5 nm, whereas higher, systematic differences were observed for larger particles. The measurement accuracy was shown to be dependent on the geometric mean diameter and the geometric standard deviation of the aerosol. Best results were found for the most abundant size distributions with geometric mean particle diameters ≥ 30 nm and geometric standard deviations larger than 1.8. The total number concentration, measured by the Partector Pro, was found to be in excellent agreement with the MPSS with a slope of the linear fit of 0.9977 and a regression coefficient of R2=0.9956. The agreement of the geometric mean particle diameter, determined with the Partector Pro and the MPSS was good but moderately dependent on the particle size distribution. For mean particle sizes between 20 and 50 nm, the bias was within ±15 %. Higher deviations of up to 30 % were observed when the geometric mean particle sizes exceeded 70 nm and when the geometric standard deviations exceeded approximately 2.7.