Saeed Sajjadi , Akrity Anand , Ana M. Beltrán , Dana Dvoranová , Aldo R. Boccaccini , Dagmar Galusková , David Jaška , Róbert Klement
{"title":"铜掺杂介孔二氧化硅颗粒(Cu-BMS)催化活化过硫酸盐以高效降解亚甲基蓝的研究","authors":"Saeed Sajjadi , Akrity Anand , Ana M. Beltrán , Dana Dvoranová , Aldo R. Boccaccini , Dagmar Galusková , David Jaška , Róbert Klement","doi":"10.1016/j.catcom.2023.106833","DOIUrl":null,"url":null,"abstract":"<div><p>The Cu-doped mesoporous silica-based particles (Cu-BMS) were prepared using an evaporation-induced self-assembly sol-gel procedure as a heterogeneous catalyst for the activation of peroxydisulfate (PDS). The formation of well-organized mesoporous structures with amorphous nature and high surface area of 286 m<sup>2</sup>/g was demonstrated. The catalytic activity of Cu-BMS in the degradation of Methylene Blue (MB) and the effects of operating parameters, including Cu-BMS dosage, initial PDS amount, initial MB concentration, temperature and initial pH, were investigated in details. The Cu-BMS demonstrated a remarkable catalytic activity (93.5% degradation efficiency within 60 min) and good stability.</p></div>","PeriodicalId":263,"journal":{"name":"Catalysis Communications","volume":"186 ","pages":"Article 106833"},"PeriodicalIF":3.4000,"publicationDate":"2024-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1566736723002352/pdfft?md5=e3ea7b0fe88c890fbc62a93fae6e118a&pid=1-s2.0-S1566736723002352-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Investigation of catalytic activation of peroxydisulfate on cu-doped mesoporous silica-based particles (Cu-BMS) for efficient degradation of methylene blue\",\"authors\":\"Saeed Sajjadi , Akrity Anand , Ana M. Beltrán , Dana Dvoranová , Aldo R. Boccaccini , Dagmar Galusková , David Jaška , Róbert Klement\",\"doi\":\"10.1016/j.catcom.2023.106833\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The Cu-doped mesoporous silica-based particles (Cu-BMS) were prepared using an evaporation-induced self-assembly sol-gel procedure as a heterogeneous catalyst for the activation of peroxydisulfate (PDS). The formation of well-organized mesoporous structures with amorphous nature and high surface area of 286 m<sup>2</sup>/g was demonstrated. The catalytic activity of Cu-BMS in the degradation of Methylene Blue (MB) and the effects of operating parameters, including Cu-BMS dosage, initial PDS amount, initial MB concentration, temperature and initial pH, were investigated in details. The Cu-BMS demonstrated a remarkable catalytic activity (93.5% degradation efficiency within 60 min) and good stability.</p></div>\",\"PeriodicalId\":263,\"journal\":{\"name\":\"Catalysis Communications\",\"volume\":\"186 \",\"pages\":\"Article 106833\"},\"PeriodicalIF\":3.4000,\"publicationDate\":\"2024-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S1566736723002352/pdfft?md5=e3ea7b0fe88c890fbc62a93fae6e118a&pid=1-s2.0-S1566736723002352-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Catalysis Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1566736723002352\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Catalysis Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1566736723002352","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Investigation of catalytic activation of peroxydisulfate on cu-doped mesoporous silica-based particles (Cu-BMS) for efficient degradation of methylene blue
The Cu-doped mesoporous silica-based particles (Cu-BMS) were prepared using an evaporation-induced self-assembly sol-gel procedure as a heterogeneous catalyst for the activation of peroxydisulfate (PDS). The formation of well-organized mesoporous structures with amorphous nature and high surface area of 286 m2/g was demonstrated. The catalytic activity of Cu-BMS in the degradation of Methylene Blue (MB) and the effects of operating parameters, including Cu-BMS dosage, initial PDS amount, initial MB concentration, temperature and initial pH, were investigated in details. The Cu-BMS demonstrated a remarkable catalytic activity (93.5% degradation efficiency within 60 min) and good stability.
期刊介绍:
Catalysis Communications aims to provide rapid publication of significant, novel, and timely research results homogeneous, heterogeneous, and enzymatic catalysis.