低能电子显微镜中的角度分辨光电子能谱学

Alexander Neuhaus, Pascal Dreher, Florian Schütz, Helder Marchetto, Torsten Franz, Frank Meyer zu Heringdorf
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引用次数: 0

摘要

光谱光发射显微镜是研究表面电子结构的一种成熟方法。在现代光发射显微镜中,根据透镜的设置,电子光学可以对像平面、动量平面或色散平面进行成像。此外,光圈还可以对能量空间、实际空间和动量空间进行过滤。在这里,我们将介绍如何在标准分光低能电子显微镜的半球形分析器入口处增加一个狭缝,以实现具有微米空间选择性的角度和能量分辨光发射模式。我们采用摄影测量校准法来纠正分析仪后面投影系统的图像失真,并以 Au(111)上记录的光谱为基准。我们的方法使能量-动量空间的数据采集更加高效,而这正是基于激光的泵探光电发射显微镜飞秒时间分辨率所必需的。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Angle-resolved photoelectron spectroscopy in a low-energy electron microscope
Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes, the electron optics allow imaging of the image plane, momentum plane, or dispersive plane, depending on the lens setting. Furthermore, apertures allow filtering of energy-, real-, and momentum space. Here, we describe how a standard spectroscopic and low-energy electron microscope can be equipped with an additional slit at the entrance of the already present hemispherical analyzer to enable an angle- and energy-resolved photoemission mode with micrometer spatial selectivity. We apply a photogrammetric calibration to correct for image distortions of the projective system behind the analyzer and present spectra recorded on Au(111) as a benchmark. Our approach makes data acquisition in energy–momentum space more efficient, which is a necessity for laser-based pump–probe photoemission microscopy with femtosecond time resolution.
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