Afshin Ebrahimi , Kun-Yi Andrew Lin , Malihe Moazeni
{"title":"在过一硫酸盐存在下通过合成的异质纳米催化剂分解三氯生的比较研究","authors":"Afshin Ebrahimi , Kun-Yi Andrew Lin , Malihe Moazeni","doi":"10.1016/j.catcom.2023.106820","DOIUrl":null,"url":null,"abstract":"<div><p>Advanced oxidation (AOPs) utilizing peroxymonosulfate (PMS) are efficient processes for the degradation of organic pollutants. This study aimed to synthesize and characterize cobalt ferrite (CoFe<sub>2</sub>O<sub>4</sub>), graphene oxide (GO), MIL-101(Fe), and their composite structures. The nanomaterials were applied as catalysts by PMS for triclosan (TCS) decomposition. The maximum removal rates of TCS were 49.29, 66.13, 84.04, 89.73, and 100% for PMS alone, CoFe<sub>2</sub>O<sub>4</sub>, GO, MIL-101(Fe), and CoFe<sub>2</sub>O<sub>4</sub>/MIL-101(Fe)/GO with PMS, respectively. Metal ions leaching declined in CoFe<sub>2</sub>O<sub>4</sub>/MIL-101(Fe)/GO/PMS compared with others. Hence, the composite nanomaterials appear to be effective catalysts for the degradation of organic pollutants by PMS activation.</p></div>","PeriodicalId":263,"journal":{"name":"Catalysis Communications","volume":"186 ","pages":"Article 106820"},"PeriodicalIF":3.4000,"publicationDate":"2023-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1566736723002224/pdfft?md5=73cbd088c23e77d8b80b84759bb2ac15&pid=1-s2.0-S1566736723002224-main.pdf","citationCount":"0","resultStr":"{\"title\":\"A comparative investigation on the decomposition of triclosan via synthesized heterogeneous nano-catalysts in the presence of peroxymonosulfate\",\"authors\":\"Afshin Ebrahimi , Kun-Yi Andrew Lin , Malihe Moazeni\",\"doi\":\"10.1016/j.catcom.2023.106820\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Advanced oxidation (AOPs) utilizing peroxymonosulfate (PMS) are efficient processes for the degradation of organic pollutants. This study aimed to synthesize and characterize cobalt ferrite (CoFe<sub>2</sub>O<sub>4</sub>), graphene oxide (GO), MIL-101(Fe), and their composite structures. The nanomaterials were applied as catalysts by PMS for triclosan (TCS) decomposition. The maximum removal rates of TCS were 49.29, 66.13, 84.04, 89.73, and 100% for PMS alone, CoFe<sub>2</sub>O<sub>4</sub>, GO, MIL-101(Fe), and CoFe<sub>2</sub>O<sub>4</sub>/MIL-101(Fe)/GO with PMS, respectively. Metal ions leaching declined in CoFe<sub>2</sub>O<sub>4</sub>/MIL-101(Fe)/GO/PMS compared with others. Hence, the composite nanomaterials appear to be effective catalysts for the degradation of organic pollutants by PMS activation.</p></div>\",\"PeriodicalId\":263,\"journal\":{\"name\":\"Catalysis Communications\",\"volume\":\"186 \",\"pages\":\"Article 106820\"},\"PeriodicalIF\":3.4000,\"publicationDate\":\"2023-12-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S1566736723002224/pdfft?md5=73cbd088c23e77d8b80b84759bb2ac15&pid=1-s2.0-S1566736723002224-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Catalysis Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1566736723002224\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Catalysis Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1566736723002224","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
A comparative investigation on the decomposition of triclosan via synthesized heterogeneous nano-catalysts in the presence of peroxymonosulfate
Advanced oxidation (AOPs) utilizing peroxymonosulfate (PMS) are efficient processes for the degradation of organic pollutants. This study aimed to synthesize and characterize cobalt ferrite (CoFe2O4), graphene oxide (GO), MIL-101(Fe), and their composite structures. The nanomaterials were applied as catalysts by PMS for triclosan (TCS) decomposition. The maximum removal rates of TCS were 49.29, 66.13, 84.04, 89.73, and 100% for PMS alone, CoFe2O4, GO, MIL-101(Fe), and CoFe2O4/MIL-101(Fe)/GO with PMS, respectively. Metal ions leaching declined in CoFe2O4/MIL-101(Fe)/GO/PMS compared with others. Hence, the composite nanomaterials appear to be effective catalysts for the degradation of organic pollutants by PMS activation.
期刊介绍:
Catalysis Communications aims to provide rapid publication of significant, novel, and timely research results homogeneous, heterogeneous, and enzymatic catalysis.